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arXiv:2107.14459 · PRX Quantum

Microwave Engineering of Programmable X X Z Hamiltonians in Arrays of Rydberg Atoms

Pascal Scholl, H. J. Williams, Guillaume Bornet, Florian Wallner, Daniel Barredo, Loïc Henriet, Adrien Signoles, Clément Hainaut, Titus Franz, S. Geier, Annika Tebben, Andre Salzinger, G. Zürn, Thierry Lahaye, Matthias Weidemüller, Antoine Browaeys

Published Apr 5, 2022• 172 citations
arXivHTMLPDF

Abstract

We use the resonant dipole-dipole interaction between Rydberg atoms and a periodic external microwave field to engineer XXZ spin Hamiltonians with tunable anisotropies.The atoms are placed in one-dimensional (1D) and two-dimensional (2D) arrays of optical tweezers.As illustrations, we apply this engineering to two iconic situations in spin physics: the Heisenberg model in square arrays and spin transport in 1D.We first benchmark the Hamiltonian engineering for two atoms and then demonstrate the freezing of the magnetization on an initially magnetized 2D array.Finally, we explore the dynamics of 1D domain-wall systems with both periodic and open boundary conditions.We systematically compare our data with numerical simulations and assess the residual limitations of the technique as well as routes for improvement.The geometrical versatility of the platform, combined with the flexibility of the simulated Hamiltonians, opens up exciting prospects in the fields of quantum simulation, quantum information processing, and quantum sensing.

DOI
10.1103/prxquantum.3.020303

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We use the resonant dipole-dipole interaction between Rydberg atoms and a periodic external microwave field to engineer XXZ spin Hamiltonians with tunable anisotropies.The atoms are placed in one-dimensional (1D) and two-dimensional (2D) arrays of optical tweezers.As illustrations, we apply this engineering to two iconic situations in spin physics: the Heisenberg model in square arrays and spin transport in 1D.We first benchmark the Hamiltonian engineering for two atoms and then demonstrate the freezing of the magnetization on an initially magnetized 2D array.Finally, we explore the dynamics of 1D domain-wall systems with both periodic and open boundary conditions.We systematically compare our data with numerical simulations and assess the residual limitations of the technique as well as routes for improvement.The geometrical versatility of the platform, combined with the flexibility of the simulated Hamiltonians, opens up exciting prospects in the fields of quantum simulation, quantum information processing, and quantum sensing.
We report the observation of electron spin interactions between Rydberg atoms, which are driven by spin-orbit coupling through second-order dipole perturbation and exhibit a spatial anisotropy governed by the atomic configuration. Specifically, we observe coherent electron spin exchange dynamics, with the measured coupling strength agreeing well with both numerical calculations and theoretical models. Furthermore, we show that global microwave dressing enables active engineering and dynamical freezing of the spin exchange by introducing a differential AC Stark shift between the participating states. Additionally, we achieve tunability of the interaction by applying a stronger magnetic field, which effectively modifies the energy contributions of the underlying spin-orbit coupling channels. Finally, measuring spin dynamics in one-dimensional multi-atom chains aligned parallel or perpendicular to the magnetic field provides a self-consistent validation of the anisotropic XXZ framework. This electron spin interaction natively features spin-position coupling and enables a natural mapping onto the Heisenberg-Kitaev model. Our findings reveal a new class of electron spin-spin interactions among Rydberg atoms, expanding the scope of quantum simulation with Rydberg atom arrays.
A major application of analog quantum hardware is quantum simulation, where a system evolves over time according to a given Hamiltonian. One challenge when implementing the Hamiltonian on a programmable quantum simulator is the availability of distinct coupling types, many of which go beyond the conventional ZZ-couplings found in Ising Hamiltonians that are naturally implemented by various platforms. In prior work, we have developed a method based on domain wall encoding to simulate one-dimensional spin chains using only Ising Hamiltonians, which would otherwise require XX+YY-couplings as well. Here, we implement the method on a commercially accessible Rydberg atom quantum device, and simulate the time evolution of the Heisenberg XXZ model with various anisotropies. We successfully probe the XY and Ising phases of the model and reproduce the qualitative behavior of several one- and two-body observables in both phases, as well as at the critical point. Our work augments the toolbox to simulate canonical quantum many-body systems on analog quantum simulators.
A frontier challenge in quantum science and technology is the construction of scalable quantum systems which can operate in regimes beyond classical simulatability. Such systems can be used as tools for simulating and exploring complex phenomena in quantum physics; they can also be used to benchmark and test quantum algorithms. Several experimental platforms, based on a variety of quantum mechanical building blocks, are currently being pursued with these goals in mind, with state-of-the-art systems capable of controlling up to around fifty particles. In this thesis, we present the development of a new platform based on individually controlled neutral atoms. In this approach, hundreds of individual atoms are trapped in an array of optical tweezers, and they are sorted in real-time into programmable geometries in one and two dimensions. After initialization of an array, atom interactions are switched on by coherent excitation to highly excited Rydberg states, resulting in a rich spin Hamiltonian. We experimentally advance several key aspects of this platform, developing new tools for controlling strongly interacting atom arrays and probing novel quantum phases and non-equilibrium dynamics. We additionally utilize Rydberg interactions to entangle atoms, demonstrating high fidelity universal quantum logic gates as well as the preparation of fully entangled Schrödinger cat states. This work highlights the prospects for scalable quantum simulation and quantum information processing beyond the limit of classical computation using neutral atom arrays.
Analog quantum simulations with Rydberg atoms in optical tweezers routinely address strongly correlated many-body problems due to the hardware-efficient implementation of the Hamiltonian. Yet, their generality is limited, and flexible Hamiltonian-design techniques are needed to widen the scope of these simulators. Here we report on the realization of spatially tunable interactions for XYZ models implemented by two-color near-resonant coupling to Rydberg pair states. Our results demonstrate the unique opportunities of Rydberg dressing for Hamiltonian design in analog quantum simulators.
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We investigate the magnetic-field dependence of the interaction between two Rydberg atoms, ∣nS1/2,mJ⟩|nS_{1/2}, m_J\rangle∣nS1/2​,mJ​⟩ and ∣(n+1)S1/2,mJ⟩|(n+1)S_{1/2}, m_J\rangle∣(n+1)S1/2​,mJ​⟩. In this setting, the effective spin-1/2 Hamiltonian takes the form of an {\it XXZ} model. We show that the anisotropy parameter of the {\it XXZ} model can be tuned by applying a magnetic field and, in particular, that it changes drastically near the Förster resonance points. Based on this result, we propose experimental realizations of spin-1/2 and spin-1 Heisenberg-type quantum spin models in Rydberg atom quantum simulators, without relying on Floquet engineering. Our results provide guidance for future experiments of Rydberg atom quantum simulators and offer insight into quantum many-body phenomena emerging in the Heisenberg model.