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arXiv:2107.12236 · Communications Physics

Quantum Floquet engineering with an exactly solvable tight-binding chain in a cavity

Christian Eckhardt, Giacomo Passetti, Moustafa Othman, Christoph Karrasch, Fabio Cavaliere, Michael A. Sentef, Dante Marvin Kennes

Published May 19, 2022• 52 citations
arXivHTMLPDF

Abstract

Abstract Recent experimental advances enable the manipulation of quantum matter by exploiting the quantum nature of light. However, paradigmatic exactly solvable models, such as the Dicke, Rabi or Jaynes-Cummings models for quantum-optical systems, are scarce in the corresponding solid-state, quantum materials context. Focusing on the long-wavelength limit for the light, here, we provide such an exactly solvable model given by a tight-binding chain coupled to a single cavity mode via a quantized version of the Peierls substitution. We show that perturbative expansions in the light-matter coupling have to be taken with care and can easily lead to a false superradiant phase. Furthermore, we provide an analytical expression for the groundstate in the thermodynamic limit, in which the cavity photons are squeezed by the light-matter coupling. In addition, we derive analytical expressions for the electronic single-particle spectral function and optical conductivity. We unveil quantum Floquet engineering signatures in these dynamical response functions, such as analogs to dynamical localization and replica side bands, complementing paradigmatic classical Floquet engineering results. Strikingly, the Drude weight in the optical conductivity of the electrons is partially suppressed by the presence of a single cavity mode through an induced electron-electron interaction.

DOI
10.1038/s42005-022-00880-9

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Abstract Recent experimental advances enable the manipulation of quantum matter by exploiting the quantum nature of light. However, paradigmatic exactly solvable models, such as the Dicke, Rabi or Jaynes-Cummings models for quantum-optical systems, are scarce in the corresponding solid-state, quantum materials context. Focusing on the long-wavelength limit for the light, here, we provide such an exactly solvable model given by a tight-binding chain coupled to a single cavity mode via a quantized version of the Peierls substitution. We show that perturbative expansions in the light-matter coupling have to be taken with care and can easily lead to a false superradiant phase. Furthermore, we provide an analytical expression for the groundstate in the thermodynamic limit, in which the cavity photons are squeezed by the light-matter coupling. In addition, we derive analytical expressions for the electronic single-particle spectral function and optical conductivity. We unveil quantum Floquet engineering signatures in these dynamical response functions, such as analogs to dynamical localization and replica side bands, complementing paradigmatic classical Floquet engineering results. Strikingly, the Drude weight in the optical conductivity of the electrons is partially suppressed by the presence of a single cavity mode through an induced electron-electron interaction.
We formulate Floquet Green's functions for noninteracting single-band lattice electrons driven by a reservoir-stabilized single-mode Gaussian quantum light source. The source is prescribed externally and is not updated by the many-electron polarization, while an active electronic probe still conditions the source evolution through the Peierls coupling. The two time arguments of a Green's function share one source history: the lesser and greater components are obtained by convolving a shared-history four-endpoint kernel with the continuous bath kernels before the final source trace, while the bath canonical anticommutation relation yields an equal-time covariance that seeds the retarded and advanced one-leg propagations. The Peierls coupling is treated nonperturbatively within the prescribed-source model, and classical Floquet theory is recovered in the appropriate limit. Numerical calculations on a minimal one-dimensional model show finite-coupling quantum-source corrections beyond a prescribed classical drive, together with spectral reconstruction and occupancy redistribution for squeezed vacuum and squeezed coherent sources. The squeezing parameter and phase provide additional control knobs, beyond classical amplitude modulation, for both sideband structure and occupied weight. This work provides a theoretical framework for quantum Floquet engineering of condensed matter with an externally prescribed quantum light source.
Floquet engineering and cavity quantum electrodynamics represent two complementary descriptions of light-matter interaction, yet their precise connection beyond the small-coupling regime remains subtle. Here, by representing the cavity field in a large-photon-number phase basis, we show that the time-dependent Schrödinger equation of a classically driven system emerges directly from the fully quantized problem, without replacing the field by a classical trajectory or assuming a mean-field decoupling. This establishes a one-to-one correspondence between quasienergies and photon-sector-shifted quantum energies, while providing a direct quantum interpretation of the Floquet mean energy and Anandan phase. Because gauge invariance is exactly preserved at the level of the quantum Hamiltonian, the quantum-to-classical correspondence remains valid beyond perturbative and small-coupling regimes. We further show that light--matter entanglement is encoded in matter--harmonic correlations of the corresponding Floquet mode, thus identifying a semiclassical limit in which Floquet physics emerges without requiring the quantum field itself to approach a coherent classical state.
We investigate classes of interacting quantum spin systems in a single-mode cavity with a Dicke coupling, as a paradigmatic example of strongly correlated light-matter systems. Coming from the limit of weak light-matter couplings and large number of matter entities, we map the relevant low-energy sector of a broad class of models in the non-superradiant phases onto the exactly solvable Dicke model. We apply the outcomes to the Dicke-Ising model as a paradigmatic example [Phys. Rev. Res. 2, 023131 (2020), Sci. Rep. 4, 4083 (2014)], in agreement with results obtained by mean-field theory [Sci. Rep. 4, 4083 (2014)]. We further accompany and verify our findings with finite-size calculations, using exact diagonalization and the series expansion method pcst ^{++} + + [Phys. Rev. A 108, 013323 (2023)]
We demonstrate the emergence of a non-equilibrium superradiant phase in the dissipative Rabi-Dicke model. This phase is characterized by a photonic steady state that oscillates with a frequency close to the cavity frequency, in contrast to the constant photonic steady state of the equilibrium superradiant phase in the Dicke model. We relate this superradiant phase to the population inversion of Floquet states by introducing a Schwinger representation of the driven two-level systems in the cavity. This inversion is depleted near Floquet energies that are resonant with the cavity frequency to sustain a coherent light-field. In particular, our model applies to solids within a two-band approximation, in which the electrons act as Schwinger fermions. We propose to use this Floquet-assisted superradiant phase to obtain controllable optical gain for a laser-like operation.
Quantum simulation with ultracold atoms provides a versatile platform to emulate condensed-matter models. In particular, momentum-space lattices enable the realization of programmable tight-binding Hamiltonians. Here, we generalize this approach by exploiting quantum resonances of a periodically driven (shaken) rotor within the Floquet framework. Using first-order time-dependent perturbation theory, we derive analytical relations between the lattice modulation and the effective tight-binding parameters, and identify explicit solutions for several resonances. We further apply optimal-control techniques to enhance the multi-period Floquet fidelity and extend the accessible parameter regimes. Experimentally, we implement this scheme with a Bose-Einstein condensate of rubidium-87 atoms in a dynamically modulated optical lattice. We demonstrate the simulation of the Rice-Mele model, including band-structure measurements and topological edge states, as well as momentum Bloch oscillations, and superlattice configurations with controlled periodicity. Our results establish quantum resonances as a powerful resource for Floquet engineering of tight-binding models in momentum space.
The ultrastrong coupling regime has emerged as a fascinating and distinctive phenomenon in cavity-QED and light-matter interactions, where the occupation of virtual excitations (e.g., photons) is possible in vacuum, which is a consequence of counter-rotating wave effects and breaking U(1) symmetry. However, an ongoing challenge is how to convert these virtual photons into real photons. We will first discuss how to “Floquet engineer” the quantum Rabi model for a two-level system coupled to a quantized cavity mode, under periodic modulation of the cavity-dipole coupling rate, leading to rich Floquet states. Exploiting the quantum vacuum, in the ultrastrong coupling regime, we show how purely mechanical driving can produce real photons. These periodic driving schemes are promising for the coherent manipulation of hybrid quantum systems and quantum vacuum effects, with applications for quantum state engineering and the study of nonequilibrium quantum phenomena.