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arXiv:2107.10769 · Physical Review A

Effects of photon statistics in wave mixing on a single qubit

W. V. Pogosov, A. Yu. Dmitriev, O. V. Astafiev

Published Aug 5, 2021• 8 citations
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Abstract

We theoretically consider wave mixing under the irradiation of a single qubit by two photon fields. The first signal is a classical monochromatic drive, while the second one is a nonclassical light. Particularly, we address two examples of a nonclassical light: (i) a broadband squeezed light and (ii) a periodically excited quantum superposition of Fock states with 0 and 1 photons. The mixing of classical and nonclassical photon fields gives rise to side peaks due to the elastic multiphoton scattering. We show that a side peaks structure is distinct from the situation when two classical fields are mixed. The most striking feature is that some peaks are absent. The analysis of peak amplitudes can be used to probe photon statistics in the nonclassical mode.

DOI
10.1103/physreva.104.023703

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We theoretically consider wave mixing under the irradiation of a single qubit by two photon fields. The first signal is a classical monochromatic drive, while the second one is a nonclassical light. Particularly, we address two examples of a nonclassical light: (i) a broadband squeezed light and (ii) a periodically excited quantum superposition of Fock states with 0 and 1 photons. The mixing of classical and nonclassical photon fields gives rise to side peaks due to the elastic multiphoton scattering. We show that a side peaks structure is distinct from the situation when two classical fields are mixed. The most striking feature is that some peaks are absent. The analysis of peak amplitudes can be used to probe photon statistics in the nonclassical mode.
We develop a theoretical description of quantum wave mixing (QWM) in a cascaded waveguide-QED system of two superconducting qubits, where the probe is driven by an external coherent tone and by the resonance fluorescence of a strongly driven source qubit. Starting from the field correlation functions of the source emission, we derive an effective master-equation treatment for the probe and identify the regime in which the incident fluorescence is characterized by anomalous correlations. When the coherent Rayleigh component of the source spectrum is suppressed, the probe equations of motion become equivalent to those for a qubit driven by a coherent tone and broadband squeezed light, although the ligt emitted by the source is non-Gaussian and antibunched. This equivalence implies a selection rule for the peaks of the QWM spectrum, with a strong suppression of sidebands associated with processes involving an odd number of photons taken from the source field. Numerical simulations of the full cascaded two-qubit model for different ratios of radiative decay rates unambiguously confirm the participation of correlated photon pairs in QWM processes. The current research illustrates that the analysis of peak amplitudes can be used to probe photon statistics in the incident nonclassical field.
A cascade of two-level superconducting artificial atoms---a source and a probe---strongly coupled to a semi-infinite waveguide is a promising tool for observing nontrivial phenomena in quantum nonlinear optics. The probe atom can scatter an antibunched radiation emitted from the source, thereby generating a field with specific properties. We experimentally demonstrate wave mixing between nonclassical light from the coherently cw-pumped source and another coherent wave acting on the probe. We observe unique features in the wave mixing stationary spectrum which differs from the mixing spectrum of two classical waves on the probe. These features are well described by adapting the theory of Gardiner et al. [Phys. Rev. A 50, 1792 (1994)] for a strongly coupled cascaded system of two atoms. We further analyze the theory to predict nonclassical mixing spectra for various ratios of atoms' radiative constants. Both experimental and numerical results confirm the domination of the multiphoton scattering process with only a single photon from the source. We evaluate entanglement of atoms in the quasistationary state and illustrate the connection between the expected second-order correlation function of the source field and wave mixing side peaks corresponding to a certain number of scattered photons.
A superconducting qubit in a waveguide behaves as a point-like nonlinear element. If irradiated with nearly resonant microwave pulses, the qubit undergoes quantum evolution and generates coherent fields at sideband frequencies due to elastic scattering. This effect is called Quantum Wave Mixing (QWM), and the number of emerged side components depends on the number of interacting photons. By driving a superconducting qubit with short pulses with alternating carrier frequencies, we control the maximal number of photons simultaneously interacting with a two-level system by varying the number and duration of applied pulses. Increasing the number of pulses results in consecutive growth of the order of non-linearity, which manifests in additional coherent side peaks appearing in the spectrum of scattered radiation while the whole spectrum maintains its asymmetry.
Superconducting quantum systems (artificial atoms) have been recently successfully used to demonstrate on-chip effects of quantum optics with single atoms in the microwave range. In particular, a well-known effect of four wave mixing could reveal a series of features beyond classical physics, when a non-linear medium is scaled down to a single quantum scatterer. Here we demonstrate the phenomenon of quantum wave mixing (QWM) on a single superconducting artificial atom. In the QWM, the spectrum of elastically scattered radiation is a direct map of the interacting superposed and coherent photonic states. Moreover, the artificial atom visualises photon-state statistics, distinguishing coherent, one- and two-photon superposed states with the finite (quantised) number of peaks in the quantum regime. Our results may give a new insight into nonlinear quantum effects in microwave optics with artificial atoms.
Superradiance in an ensemble of atoms leads to the collective enhancement of radiation in a particular mode shared by the atoms in their spontaneous decay from an excited state. The quantum aspects of this phenomenon are highlighted when such collective enhancement is observed in the emission of a single quantum of light. Here we report a further step in exploring experimentally the nonclassical features of superradiance by implementing the process not only with single excitations, but also in a two-excitation state. Particularly, we measure and theoretically model the wave packets corresponding to superradiance in both the single-photon and two-photon regimes. Such progress opens the way to the study and future control of the interaction of nonclassical light modes with collective quantum memories at higher photon numbers.
Single atom cavity quantum electrodynamics grants access to nonclassical photon statistics, while electromagnetically induced transparency exhibits a dark state of long coherence time. The combination of the two produces a new light field via four-wave mixing that shows long-lived quantum statistics. We observe the new field in the emission from the cavity as a beat with the probe light that together with the control beam and the cavity vacuum is driving the four-wave mixing process. Moreover, the control field allows us to tune the new light field from antibunching to bunching, demonstrating our all-optical control over the photon-pair emission.