The dynamics of open quantum systems is often modeled using master equations, which describe the expected outcome of an experiment (i.e., the average over many realizations of the same dynamics). Quantum trajectories, instead, model the outcome of ideal single experiments---the ``clicks'' of a perfect detector due to, e.g., spontaneous emission. The correct description of quantum jumps, which are related to random events characterizing a sudden change in the wave function of an open quantum system, is pivotal to the definition of quantum trajectories. In this article, we extend the formalism of quantum trajectories to open quantum systems with ultrastrong coupling (USC) between light and matter by properly defining jump operators in this regime. In such systems, exotic higher-order quantum-state and energy transfer can take place without conserving the total number of excitations in the system. The emitted field of such USC systems bears signatures of these higher-order processes, and significantly differs from similar processes at lower coupling strengths. Notably, the emission statistics must be taken at a single quantum trajectory level, since the signatures of these processes are washed out by the ``averaging'' of a master equation. We analyze the impact of the chosen unraveling (i.e., how one collects the output field of the system) for the quantum trajectories and show that these effects of the higher-order USC processes can be revealed in experiments by constructing histograms of detected quantum jumps. We illustrate these ideas by analyzing the excitation of two atoms by a single photon [Garziano et al., Phys. Rev. Lett. 117, 043601 (2016)]. For example, quantum trajectories reveal that keeping track of the quantum jumps from the atoms allows one to reconstruct both the oscillations between one photon and two atoms as well as emerging Rabi oscillations between the two atoms.
The dynamics of open quantum systems is often modeled using master equations, which describe the expected outcome of an experiment (i.e., the average over many realizations of the same dynamics). Quantum trajectories, instead, model the outcome of ideal single experiments---the clicks'' of a perfect detector due to, e.g., spontaneous emission. The correct description of quantum jumps, which are related to random events characterizing a sudden change in the wave function of an open quantum system, is pivotal to the definition of quantum trajectories. In this article, we extend the formalism of quantum trajectories to open quantum systems with ultrastrong coupling (USC) between light and matter by properly defining jump operators in this regime. In such systems, exotic higher-order quantum-state and energy transfer can take place without conserving the total number of excitations in the system. The emitted field of such USC systems bears signatures of these higher-order processes, and significantly differs from similar processes at lower coupling strengths. Notably, the emission statistics must be taken at a single quantum trajectory level, since the signatures of these processes are washed out by the averaging'' of a master equation. We analyze the impact of the chosen unraveling (i.e., how one collects the output field of the system) for the quantum trajectories and show that these effects of the higher-order USC processes can be revealed in experiments by constructing histograms of detected quantum jumps. We illustrate these ideas by analyzing the excitation of two atoms by a single photon [Garziano et al., Phys. Rev. Lett. 117, 043601 (2016)]. For example, quantum trajectories reveal that keeping track of the quantum jumps from the atoms allows one to reconstruct both the oscillations between one photon and two atoms as well as emerging Rabi oscillations between the two atoms.
In the last decades, the experimental and theoretical study of light-matter interactions in confined quantum systems has allowed to considerably widen and deepen our understanding of the quantum world.The simplest fully-quantized light-matter interaction is the quantum Rabi model (QRM), where a two-level system is coupled to a single bosonic mode.The implementation of quantum-optical systems in which the interaction strength overcomes losses brought a revolution to this research area.Under this condition, dubbed strong coupling (SC) regime, quantum processes can be observed at the single-photon level, and even exploited to perform Quantum Information tasks.Recent developments in solid-state Quantum Technologies have made possible to push the line further, achieving the ultrastrong coupling (USC) regime of the QRM, in which the interaction strength is comparable with the bare frequencies of the interacting systems.In the USC regime of the QRM, light and matter degrees of freedom merge into collective bound states called polaritons, the system ground state is not the vacuum and excitations are not conserved.The growing interest in USC-related phenomena is mainly motivated by the fundamental counterintuitive modifications to light-matter interactions entailed by this regime.At the same time, the USC regime is also expected to provide computational benefits in terms of operational speed, coherence time, and noise protection.In this Thesis, we theoretically analyze novel quantum phenomena emerging in the USC regime, which can be observed using nowadays technology and can motivate foreseeable improvements.The results here presented have been derived using two conceptually different approaches.On one side, we have analyzed interesting models that can be implemented in superconducting circuits, a quantum platform where the USC regime can be naturally achieved.In particular, we focused on excitation transfer across USC impurities, entanglement generation via modulation of electrical boundary conditions and quantum state engineering in ultrastrongly-coupled systems.On the other hand, we have developed methods to reproduce the physics of light-matter interactions in the USC regime, by tailoring the Hamiltonian of atomic systems, like trapped ions and cold atoms.These proposals take profit of the specific features of such quantum platforms, in order to implement regimes and measurements that are not directly accessible.We believe that this Thesis will contribute to develop a thorough understanding of quantum phenomena related to the USC regime of light-matter interaction, and that it will foster the dialog between experimental and theoretical research in this area.I would like to thank first my PhD supervisor Prof. Enrique Solano, for his constant support and invaluable guidance.Countless thought-provoking discussions held with him during my PhD studies have contributed to develop my critical skills, and his advice has covered all facets of nowadays top-level research.
We introduce jump-time unraveling as a distinct description of open quantum systems. As our starting point, we consider quantum jump trajectories, which emerge, physically, from continuous quantum measurements, or, formally, from the unraveling of Markovian quantum master equations. If the stochastically evolving quantum trajectories are ensemble-averaged at specific times, the resulting quantum states are solutions to the associated quantum master equation. We demonstrate that quantum trajectories can also be ensemble-averaged at specific jump counts. The resulting jump-time-averaged quantum states are then solutions to a discrete, deterministic evolution equation, with time replaced by the jump count. This jump-time evolution represents a trace-preserving quantum dynamical map if and only if the associated open system does not exhibit dark states. In the presence of dark states, on the other hand, jump-time-averaged states may decay into the dark states and the jump-time evolution may eventually terminate. Jump-time-averaged quantum states and the associated jump-time evolution are operationally accessible in continuous measurement schemes, when quantum jumps are detected and used to trigger the readout measurements. We illustrate the jump-time evolution with the examples of a two-level system undergoing relaxation or dephasing, a damped harmonic oscillator, and a free particle exposed to collisional decoherence.
In the quantum trajectory approach an open quantum system is represented by a stochastic pure-state wave function. The mixed-state density operator that satisfies the usual master equation is recovered from the quantum trajectories by performing either an ensemble average or, for stationary systems, an average over time. This unraveling of the master equation dynamics into pure-state trajectories provides new insight into the decay of quantum coherence in systems that are open to the environment. Under some conditions macroscopic superposition states are preserved as macroscopic superposition states along individual trajectories, but are reduced to mixtures by the trajectory average. Under other conditions one of the states in a macroscopic superposition becomes dominant (in amplitude) over the other along each quantum trajectory. We discuss the mechanisms that produce these dynamics and assess the implications for the observation of Schrodinger cat states in optics experiments. We present results for some specific examples of macroscopic superposition states generated by a cavity QED system. The system involves a small collection of atoms in an optical cavity driven by a coherent laser field. Under strong-coupling conditions this system produces a variety of Schrodinger cat states whose precise form depends on the number of atoms, the method of excitation (through a cavity mirror or from the side), the initial state of the atoms, and the position of the atoms in the cavity.
We study the stochastic dynamics of the electromagnetic field in a lossless cavity interacting with a beam of two-level atoms, given that the atomic states are measured after they have crossed the cavity. The atoms first interact at the exit of the cavity with a classical laser field ℰ and then enter into a detector which measures their states. Each measurement disentangles the field and the atoms and changes in a random way the state |ψ(t)〉 of the cavity field. For weak atom-field coupling, the evolution of |ψ(t)〉 when many atoms cross the cavity and the detector is characterized by a succession of quantum jumps occurring at random times, separated by quasi-Hamiltonian evolutions, both of which depend on the laser field ℰ. For ℰ=0, the dynamics is the same as in the Monte Carlo wave function model of Dalibard et al. [Phys. Rev. Lett. 68, 580 (1992)] and Carmichael, An Open System Approach to Quantum Optics, Lecture Notes in Physics Vol. 18 (Springer, Berlin, 1991)]. The density matrix of the quantum field, obtained by averaging the projector |ψ(t)〉〈ψ(t)| over all results of the measurements, is independent of ℰ and follows the master equation of the damped harmonic oscillator at finite temperature. We provide numerical evidence showing that for large ℰ, an arbitrary initial field state |ψ(0)〉 evolves under the monitoring of the atoms and the measurements toward squeezed states |α,re2iφ〉, moving in the α-complex plane but with almost constant squeezing parameters r and φ. The values of r and φ are determined analytically. On the other hand, for ℰ=0, the dynamics transforms the initial state into Fock states |n〉 with fluctuating numbers of photons n, as shown in Kist et al. [J. Opt. B: Quantum Semiclassical Opt. 1, 251 (1999)]. In the last part, we derive the quantum jump dynamics from the linear quantum jump model proposed in Spehner and Bellissard [J. Stat. Phys. 104, 525 (2001)], for arbitrary open quantum systems having a Lindblad-type evolution. A careful derivation of the infinite jump rates limit, where the dynamics can be approximated by a diffusion process of the quantum state, is also presented.
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) they appear to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurrence of light-matter decoupling in the deep strong-coupling regime and show how all of the obtained results are gauge invariant.
The Gorini-Kossakowski-Sudarshan-Lindblad master equation (ME) governs the density matrix of open quantum systems (OQSs). When an OQS is subjected to weak continuous measurement, its state evolves as a stochastic quantum trajectory, whose statistical average solves the ME. The ensemble of such trajectories is termed an unraveling of the ME. We propose a method to operationally distinguish unravelings produced by the same ME in different measurement scenarios, using nonlinear averages of observables over trajectories. We apply the method to the paradigmatic quantum nonlinear system of resonance fluorescence in a two-level atom. We compare the Poisson-type unraveling, induced by direct detection of photons scattered from the two-level emitter, and the Wiener-type unraveling, induced by phase-sensitive detection of the emitted field. We show that a quantum-trajectory-averaged variance is able to distinguish these measurement scenarios. We evaluate the performance of the method, which can be readily extended to more complex OQSs, under a range of realistic experimental conditions. Published by the American Physical Society 2024