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arXiv:2107.06346

Driven dissipative preparation of few-body Laughlin states of Rydberg polaritons in twisted cavities

Kristina R. Colladay, Erich J. Mueller

Published Jul 13, 2021• 1 citation
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Abstract

We present a driven dissipative protocol for creating an optical analog of the Laughlin state in a system of Rydberg polaritons in a twisted optical cavity. We envision resonantly driving the system into a 4-polariton state by injecting photons in carefully selected modes. The dissipative nature of the polariton-polariton interactions leads to a decay into a two-polariton analog of the Laughlin state. Generalizations of this technique could be used to explore fractional statistics and anyon based quantum information processing. We also model recent experiments that attempt to coherently drive into this same state.

DOI
10.48550/arxiv.2107.06346

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We present a driven dissipative protocol for creating an optical analog of the Laughlin state in a system of Rydberg polaritons in a twisted optical cavity. We envision resonantly driving the system into a 4-polariton state by injecting photons in carefully selected modes. The dissipative nature of the polariton-polariton interactions leads to a decay into a two-polariton analog of the Laughlin state. Generalizations of this technique could be used to explore fractional statistics and anyon based quantum information processing. We also model recent experiments that attempt to coherently drive into this same state.
We study the propagation of strongly interacting Rydberg polaritons through an atomic medium in a one-dimensional optical lattice. We derive an effective single-band Hubbard model to describe the dynamics of the dark-state polaritons under realistic assumptions. Within this model, we analyze the driven-dissipative transport of polaritons through the system by considering a coherent drive on one side and by including the spontaneous emission of the metastable Rydberg state. Using a variational approach to solve the many-body problem, we find strong antibunching of the outgoing photons despite the losses from the Rydberg state decay.
Designing materials with specific properties has been a long-time goal of the physics community. Optical photons have recently emerged as a promising candidate for such metamaterials due to their fast dynamics and available manipulation toolkit. In conjunction with carefully engineered optical resonators, it is possible to precisely control the properties of individual photons through the resonator Hamiltonian. The only missing ingredient to photonic materials is strong photon-photon interactions. This thesis describes the characterization of cavity Rydberg polaritons and the emergence of strong interactions in such a system. Electromagnetically induced transparency (EIT) is used to create quasiparticles that inherit the properties of both photons and Rydberg atoms: fast dynamics and trapping from the photons and long-range dipole-dipole interactions from the Rydberg atoms. The emergent polaritonic properties are characterized and controlled through the dark-state rotation angle and agree very well with theoretical predictions. We then expand upon this understanding of polaritons by putting them inside a zerodimensional quantum dot. Confining the polaritons in such an object allows for strong interparticle interactions to manifest. We observe these interactions through the temporal auto-correlation intensity function g2(t) and verify the dimensionality of the quantum dot itself by measure the polariton Rabi oscillations. With the experimental demonstration of strong photonic interactions, a complete understanding of Rydberg atoms and polaritons is needed to allow for better control of the system. To this effect, the properties of Rydberg atoms are analytically and numerically understood and the full formalism needed to describe resonator Rydberg polaritons is developed, along with their interactions and various sources of decoherence. Furthermore, a renormalized effective field theory for single mode cavities is developed and tested against full numerical models, paving the way for the simulation of the physical phenomena of manybody states in multi-mode cavities. Strongly interacting cavity polaritons can be utilized in quantum gate and repeater protocols for quantum information processing. Furthermore, combining the experimental and theoretical work here with non-planar resonators presents a clear path to non-trivial topological synthetic materials and strongly correlated quantum states.
Synthetic quantum materials offer an exciting opportunity to explore quantum many-body physics and novel states of matter under controlled conditions. In particular, they provide an avenue to exchange the short length scales and large energy scales of the solid state for an engineered system with better control over the system Hamiltonian, more accurate state preparation, and higher fidelity state readout. Here we propose a unique platform to study quantum phases of strongly interacting photons. We introduce ideas for controlling the dynamics of individual photons by manipulating the geometry of a multimode optical cavity, and combine them with recently established techniques to mediate strong interactions between photons using Rydberg atoms. We demonstrate that this approach gives rise to crystalline- and fractional quantum Hall- states of light, opening the door to studies of strongly correlated quantum many-body physics in a photonic material.
The Bose-Hubbard model (BHM) describes bosons hopping across sites and interacting on-site. Inspired by the success of BHM simulators with atoms in optical lattices, proposals for implementing the BHM with photons in coupled nonlinear cavities have recently emerged. Two coupled semiconductor microcavities constitute a model system where the hopping, interaction and decay of exciton polaritons-mixed light-matter quasiparticles-can be engineered in combination with site-selective coherent driving to implement the driven-dissipative two-site optical BHM. Here we explore the interplay of interference and nonlinearity in this system, in a regime where three distinct density profiles can be observed under identical driving conditions. We demonstrate how the phase acquired by polaritons hopping between cavities can be controlled through polariton-polariton interactions. Our results open new perspectives for synthesizing density-dependent gauge fields using polaritons in two-dimensional multicavity systems.
We propose a scheme for realizing fractional quantum Hall states of light. In our scheme, photons of two polarizations are coupled to different atomic Rydberg states to form two flavors of Rydberg polaritons that behave as an effective spin. An array of optical cavity modes overlapping with the atomic cloud enables the realization of an effective spin-1/21/21/2 lattice. We show that the dipolar interaction between such polaritons, inherited from the Rydberg states, can be exploited to create a flat, topological band for a single spin-flip excitation. At half filling, this gives rise to a photonic (or polaritonic) fractional Chern insulator---a lattice-based, fractional quantum Hall state of light.
Abstract Photonic materials are an emerging platform to explore quantum matter (Carusotto and Ciuti 2013 Rev. Mod. Phys. 85 299; Sommer et al 2015 arXiv: 1506.00341 ) and quantum dynamics (Peyronel et al 2012 Nature 488 57). The development of Rydberg electromagnetically induced transparency (Weatherill et al 2008 J. Phys. B: At. Mol. Opt. Phys. 41 201002; Petrosyan et al 2011 Phys. Rev. Lett. 107 213601) provided a clear route to strong interactions between individual optical photons. In conjunction with carefully designed optical resonators, it is now possible to achieve extraordinary control of the properties of individual photons, introducing tunable gauge fields (Schine et al 2016 Nature 534 671) whilst imbuing the photons with mass and embedding them on curved spatial manifolds (Sommer et al 2016 New J. Phys. 18 035008). Building on work formalizing Rydberg mediated interactions between propagating photons (Gorshkov et al 2011 Phys. Rev. Lett. 107 133602; Gullans et al 2016 Phys. Rev. Lett. 117 113601), we develop a theory of interacting Rydberg polaritons in multimode optical resonators, where the strong interactions are married with tunable single particle properties to build and probe exotic matter. In the presence of strong coupling between the resonator field and a Rydberg-dressed atomic ensemble, a quasiparticle called the ‘cavity Rydberg polariton’ emerges. We investigate its properties, finding that it inherits both the fast dynamics of its photonic constituents and the strong interactions of its atomic constituents. We develop tools to properly renormalize the interactions when polaritons approach each other, and investigate the impact of atomic motion on the coherence of multi-mode polaritons, showing that most channels for atom-polariton cross-thermalization are strongly suppressed. Finally, we propose to harness the repeated diffraction and refocusing of the optical resonator to realize interactions which are local in momentum-space. This work points the way to efficient modeling of polaritonic quantum materials in properly renormalized strongly interacting effective theories, thereby enabling experimental studies of photonic fractional quantum Hall fluids and crystals (Sommer et al 2015 arXiv: 1506.00341 ; Umucalılar et al 2014 Phys. Rev. A 89 023803; Grusdt and Fleischhauer 2013 Phys. Rev. A 87 043628), plus photonic quantum information processors and repeaters (Jaksch et al 2000 Phys. Rev. Lett. 85 2208; Saffman et al 2010 Rev. Mod. Phys. 82 2313; Han et al 2010 Phys. Rev. A 81 , 052311).