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arXiv:2106.09596 · Optics Letters

Effective super-bandwidth in laser pulses

Enrique G. Neyra, Demian A. Biasetti, Pablo Vaveliuk, Gustavo Adrian Torchia, Marcelo F. Ciappina, Fabián A. Videla, Lorena Rebón

Published Aug 25, 2021• 3 citations
arXivHTMLPDF

Abstract

We present here a theoretical analysis of the interaction between an ideal two-level quantum system and a super-oscillatory pulse, like the one proposed and successfully synthesized in [J. Opt.23, 075604 (2021)JOOPDB0150-536X10.1088/2040-8986/abfedf; arXiv:2106.09192 (2021)]. As a prominent feature, these pulses present a high efficiency of the central super-oscillatory region in relation to unavoidable sidelobes. Our study shows an increase in the effective bandwidth of the pulse in the super-oscillatory region, and not only the appearance of a local frequency higher than its highest Fourier-frequency component, as in the usual description of the phenomenon of super-oscillations. Beyond introducing the concept of effective super-bandwidth, the presented results could be relevant for experimental applications and opening new perspectives for laser-matter interaction.

DOI
10.1364/ol.434531

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We present here a theoretical analysis of the interaction between an ideal two-level quantum system and a super-oscillatory pulse, like the one proposed and successfully synthesized in [J. Opt.23, 075604 (2021)JOOPDB0150-536X10.1088/2040-8986/abfedf; arXiv:2106.09192 (2021)]. As a prominent feature, these pulses present a high efficiency of the central super-oscillatory region in relation to unavoidable sidelobes. Our study shows an increase in the effective bandwidth of the pulse in the super-oscillatory region, and not only the appearance of a local frequency higher than its highest Fourier-frequency component, as in the usual description of the phenomenon of super-oscillations. Beyond introducing the concept of effective super-bandwidth, the presented results could be relevant for experimental applications and opening new perspectives for laser-matter interaction.
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Abstract Super-oscillation is a counterintuitive phenomenon describing localized fast variations of functions and fields that happen at frequencies higher than the highest Fourier component of their spectra. The physical implications of this effect have been studied in information theory and optics of classical fields, and have been used in super-resolution imaging. As a general phenomenon of wave dynamics, super-oscillations have also been predicted to exist in quantum wavefunctions. Here we report the experimental demonstration of super-oscillatory behavior of a single-quantum object, a photon. The super-oscillatory behavior is demonstrated by tight localization of the photon wavefunction after focusing with an appropriately designed slit mask to create an interference pattern with a sub-diffraction hotspot (~0.45 λ). Such quantum super-oscillation can be used for low-intensity far-field super-resolution imaging techniques even down to single-photon counting regime, which would be of interest to quantum physics and non-invasive and label-free biological studies.
The spectrum evolution of a few-cycle optical pulse in a resonant two-level atom medium is studied theoretically by using the full Maxwell-Bloch equations. On the propagating pulse, significantly much faster oscillation components separated with the main pulse appear due to strong self-phase modulation and pulse reshaping. In this case, ideal self-induced transparency cannot occur for a 2π pulse. The spectrum of the 4π pulse shows an evident oscillatory feature because of the continuum interference of the separate pulses. For larger pulse areas, continuum generation from near ultraviolet to infrared occurs.
Dynamic multiphoton resonances in ultra-short super-intense laser pulses consisting of 50-200 field periods are considered numerically for a two-level system. The impact of non-resonant (Bloch-Siegert) and carrier-envelope effects on the dynamics of a two-level system was studied numerically, and conditions for complete population inversion were derived. The widths of multiphoton resonances increase with the increasing of the laser field. Results do not depend practically on the pulse duration. Effective resonance frequencies for multiphoton resonances increases strongly in a super-intense field. Multiphoton resonances are shifted and unified with each other in super-intense laser fields.
The absorption of a single photon that excites a quantum system from a low to a high energy level is an elementary process of light-matter interaction, and a route towards realizing pure single-photon absorption has both fundamental and practical implications in quantum technology. Due to nonlinear optical effects, however, the probability of pure single-photon absorption is usually very low, which is particularly pertinent in the case of strong ultrafast laser pulses with broad bandwidth. Here we demonstrate theoretically a counterintuitive coherent single-photon absorption scheme by eliminating nonlinear interactions of ultrafast laser pulses with quantum systems. That is, a completely linear response of the system with respect to the spectral energy density of the incident light at the transition frequency can be obtained for all transition probabilities between 0 and 100% in multilevel quantum systems. To that end, a multiobjective optimization algorithm is developed to find an optimal spectral phase of an ultrafast laser pulse, which is capable of eliminating all possible nonlinear optical responses while maximizing the probability of single-photon absorption between quantum states. This work not only deepens our understanding of light-matter interactions, but also offers a way to study photophysical and photochemical processes in the ``absence'' of nonlinear optical effects.
We experimentally broke the temporal Fourier focusing limit of an ultra-short optical pulse and used it to demonstrate temporal super-resolution detection of a temporal event [1]. The envelope function of the pulse is synthesized in the form of a Super-Oscillating Beat (SOB) signal, made of pairs of optical modes (i.e. beat modes) centered around a common carrier frequency. The mathematical form for the synthesis of the SOB signal is based on a known super-oscillatory function [2]. Suited with the right amplitude and phases these beat modes interfere to create a lobe in the temporal waveform of the field’s envelope which can be arbitrarily narrow, at the cost of reduced amplitude at the fast oscillation. In our case, we achieved a temporal feature that is approximately three times shorter than the duration of a transform-limited Gaussian pulse having a comparable bandwidth while maintaining 30% visibility of the super-oscillating feature. We then used this SOB signal to demonstrate experimentally temporal super-resolution. Specifically, the SOB signal was used to resolve the existence of a temporal double-slit, a pair of adjacent pulses which are detected as a single temporal event by a transform-limited Gaussian pulse having the same bandwidth. Formally, this experiment constitutes a temporal analogue to super resolution imaging by using a super oscillating point-spread-function [3,4]. Numerical simulations analyse in which cases the SOB signal outperform transform-limited signals for detection of short temporal events. [1] Y. Eliezer, L. Hareli, L. Lobachinsky, S. Froim and A. Bahabad, “Breaking the Temporal Resolution Limit by Superoscillating Optical Beats”, Physical Review Letters, 119, 043903 (2017). [2] M. V Berry and S. Popescu, "Evolution of Quantum Superoscillations and Optical Supperresolution without Evanescent Waves," J. Phys. A. Math. Gen. 39, 6965 (2006). [3] A. M. H. Wong and G. V Eleftheriades, "An Optical Super-microscope for Far-field, Real-time Imaging Beyond the Diffraction Limit" Sci. Rep. 3, (2013). [4] E. T. F. Rogers, J. Lindberg, T. Roy, S. Savo, J. E. Chad, M. R. Dennis, and N. I. Zheludev, "A Super-oscillatory Lens Optical Microscope for Subwavelength Imaging," Nat. Mater. 11, 432 (2012).