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arXiv:2106.05179 · Physical Review Research

Intrinsic mechanisms for drive-dependent Purcell decay in superconducting quantum circuits

Ryo Hanai, Alexander McDonald, Aashish A. Clerk

Published Dec 30, 2021• 20 citations
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Abstract

We develop an approach to understanding intrinsic mechanisms that cause the ${T}_{1}$-decay rate of a multilevel superconducting qubit to depend on the photonic population of a coupled, detuned cavity. Our method yields simple analytic expressions for both the coherently driven or thermally excited cases, which are in good agreement with full master equation numerics, and also facilitates direct physical intuition. It also predicts several interesting phenomena. In particular, we find that in a wide range of settings, the cavity-qubit detuning controls whether a nonzero photonic population increases or decreases qubit Purcell decay. Our method combines insights from a Keldysh treatment of the system, and Lindblad perturbation theory.

DOI
10.1103/physrevresearch.3.043228

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We develop an approach to understanding intrinsic mechanisms that cause the T1{T}_{1}T1​-decay rate of a multilevel superconducting qubit to depend on the photonic population of a coupled, detuned cavity. Our method yields simple analytic expressions for both the coherently driven or thermally excited cases, which are in good agreement with full master equation numerics, and also facilitates direct physical intuition. It also predicts several interesting phenomena. In particular, we find that in a wide range of settings, the cavity-qubit detuning controls whether a nonzero photonic population increases or decreases qubit Purcell decay. Our method combines insights from a Keldysh treatment of the system, and Lindblad perturbation theory.
We analyze the Purcell relaxation rate of a superconducting qubit coupled to a resonator, which is coupled to a transmission line and pumped by an external microwave drive. Considering the typical regime of the qubit measurement, we focus on the case when the qubit frequency is significantly detuned from the resonator frequency. Surprisingly, the Purcell rate decreases when the strength of the microwave drive is increased. This suppression becomes significant in the nonlinear regime. In the presence of the microwave drive, the loss of photons to the transmission line also causes excitation of the qubit; however, the excitation rate is typically much smaller than the relaxation rate. Our analysis also applies to a more general case of a two-level quantum system coupled to a cavity.
The dynamics of a weakly anharmonic superconducting qubit in a complex electromagnetic environment is generally well described by an effective multimode Kerr Hamiltonian at sufficiently weak excitation. This Hamiltonian can be embedded in a master equation with losses determined by the details of the electromagnetic environment. Recent experiments indicate, however, that when a superconducting circuit is driven with microwave signals populating the system with sufficiently high excitations, the observed relaxation rates appear to be substantially different from expectations based on the electromagnetic environment of the qubit alone. This issue is a limiting factor in the optimization of superconducting qubit readout schemes. We claim here that an effective master equation with drive-power-dependent parameters is an efficient approach to model such quantum dynamics. In this sequence of papers, we derive effective master equations, whose parameters exhibit nonlinear dependence on the excitation level of the circuit as well as the electromagnetic environment of the qubit. We show that the number nonconserving terms in the qubit nonlinearity generally lead to a renormalization of dissipative parameters of the effective master equation, while the number conserving terms give rise to a renormalization of the system frequencies. Here, in Paper I, we consider the excitation-relaxation dynamics of a transmon qubit that is prepared in a certain initial state, but is not driven otherwise. A unitary transformation technique is introduced to study the renormalization of (i) qubit relaxation due to coupling to a generic bath and (ii) Purcell decay. Analytic expressions are provided for the dependence of the nonlinear dissipative terms on the details of the electromagnetic environment of the qubit. The perturbation technique based on unitary transformations developed here is generalized to the continuously driven case in Paper II [A. Petrescu et al., Phys. Rev. B 101, 134510 (2020)].
One of the defining features of pulsed dynamical decoupling is its suppression of a driven qubit's sensitivity to static detuning errors between the drive field and qubit resonance. In this paper, we show that dissipation, in the form of excited-state decay, can change this behavior entirely, producing an interference signal with a strong detuning dependence. This signal arises from decay during driven evolution and relies on coherence retained by the qubit after such a decay event. We develop analytical and numerical models that capture the underlying mechanism and observe this same dissipation-induced detuning dependence experimentally in both a free-space strontium atom interferometer and a superconducting transmon qubit system. We also use this dissipation-induced detuning dependence as the basis for a new spectroscopic technique called Dissipative Carr-Purcell Spectroscopy (DCPS) and compare it with a traditional Ramsey sequence. Our results establish a regime of pulsed dynamical decoupling in which dissipation reshapes, rather than merely degrades, coherent control, and we expect these dynamics to be relevant to a wide range of quantum systems.
Decoherence due to radiative decay remains an important consideration in scaling superconducting quantum processors. We introduce a passive, interference-based methodology for suppressing radiative decay using only the intrinsic multi-mode structured environment of superconducting circuits. By taking into account the full electromagnetic mode-mode couplings within the device, we derive analytic conditions that enable destructive interference. These conditions are realized by introducing controlled geometric asymmetries -- such as localized perturbations to the transmon capacitor -- which increase mode hybridization and activate interference between multiple decay pathways. We validate this methodology using perturbation theory, full-wave electromagnetic simulations, and experimental measurements of a symmetry-broken transmon qubit with improved coherence times.
The speed and fidelity of dispersive readout of superconducting qubits should improve by increasing the amplitude of the measurement drive. Experiments show, however, that beyond some drive amplitude there is always a saturation or drop in fidelity, often associated with a decrease in qubit energy relaxation time T1T_1T1​. A simple Lindblad master equation does not capture the latter effect. More involved approaches based on effective master equations rely on strong assumptions about the spectra of the system and the bath and only partially agree with observations. Here, we perform a first-principles simulation of the full unitary dynamics of dispersive readout by considering the circuit QED Hamiltonian coupled to a microscopic model for the measurement transmission line, allowing for its arbitrary spectrum, including filters. Our access to the dynamics of the bath degrees of freedom allows us to investigate the emission spectrum of the system as a function of drive power. We show how the dependence of qubit T1T_1T1​ on readout drive amplitude is sensitive to the details of the bath spectrum. In particular, we find that T1T_1T1​ drops with increasing drive amplitude when a Purcell notch filter is placed at the qubit frequency, and that the Lindblad master equation shows general qualitative defects compared to the first-principles model.
Driven-dissipative qubit-resonator dynamics, which are the basis of most dispersive superconducting qubit measurement schemes, are often modeled with Lindblad master equations built from subsystem local jump operators, even when the qubit and resonator are appreciably hybridized. In this work we revisit this setting using a microscopic Bloch-Redfield approach, where dissipation is constructed in the eigenbasis of the coupled qubit-resonator Hamiltonian with a complete, frequency dependent, open system description of the transmission line environment. Here, we show that the Lindblad and Bloch-Redfield decay rates can be quantitatively different in the absence of driving, while in the driven case we demonstrate that the time-independent Redfield dissipator and its time-dependent generalization can show qualitatively different behaviors as a function of driving strength. Finally, we investigate the effects of driving in structured spectral densities, recovering the suppression of measurement-induced relaxation in the presence of a so called Purcell filter.