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arXiv:2106.02042 · Nature Communications

Universality of Dicke superradiance in arrays of quantum emitters

Stuart J. Masson, Ana Asenjo-Garcı́a

Published Apr 27, 2022• 166 citations
arXivHTMLPDF

Abstract

Dicke superradiance is an example of emergence of macroscopic quantum coherence via correlated dissipation. Starting from an initially incoherent state, a collection of excited atoms synchronizes as they decay, generating a macroscopic dipole moment and emitting a short and intense pulse of light. While well understood in cavities, superradiance remains an open problem in extended systems due to the exponential growth of complexity with atom number. Here we show that Dicke superradiance is a universal phenomenon in ordered arrays. We present a theoretical framework - which circumvents the exponential complexity of the problem - that allows us to predict the critical distance beyond which Dicke superradiance disappears. This critical distance is highly dependent on the dimensionality and atom number. Our predictions can be tested in state of the art experiments with arrays of neutral atoms, molecules, and solid-state emitters and pave the way towards understanding the role of many-body decay in quantum simulation, metrology, and lasing.

DOI
10.1038/s41467-022-29805-4

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Dicke superradiance is an example of emergence of macroscopic quantum coherence via correlated dissipation. Starting from an initially incoherent state, a collection of excited atoms synchronizes as they decay, generating a macroscopic dipole moment and emitting a short and intense pulse of light. While well understood in cavities, superradiance remains an open problem in extended systems due to the exponential growth of complexity with atom number. Here we show that Dicke superradiance is a universal phenomenon in ordered arrays. We present a theoretical framework - which circumvents the exponential complexity of the problem - that allows us to predict the critical distance beyond which Dicke superradiance disappears. This critical distance is highly dependent on the dimensionality and atom number. Our predictions can be tested in state of the art experiments with arrays of neutral atoms, molecules, and solid-state emitters and pave the way towards understanding the role of many-body decay in quantum simulation, metrology, and lasing.
Many-body superradiance in ordered atomic arrays is a phenomenon where atomic synchronization gives rise to a burst in photon emission. This superradiant burst only occurs if there is one -- or just a few -- dominant decay channels. We demonstrate that superradiance exists in arrays of any dimensionality, as interference in photon emission leads to the preeminence of certain channels over others. In atomic chains superradiance occurs only below a critical interatomic distance, which we derive analytically. Increasing the array dimensionality leads to a critical distance that scales with system size: sub-logarithmically for 2D, and seemingly faster than that for 3D lattices. We perform calculations for both infinite and finite systems, the latter by employing a highly-efficient algorithm with a computational complexity that scales only linearly with system size, which enables us to study very large arrays. Our results provide a guide to explore this many-body phenomenon in state-of-the art experimental setups.
Dicke superradiance in ordered atomic arrays is a phenomenon where atomic synchronization gives rise to a burst in photon emission. This superradiant burst only occurs if there is one---or just a few---dominant decay channels. For a fixed atom number, this happens only below a critical interatomic distance. Here we show that array dimensionality is the determinant factor that drives superradiance. In two-dimensional (2D) and three-dimensional (3D) arrays, superradiance occurs due to constructive interference, which grows stronger with atom number. This leads to a critical distance that scales sublogarithmically with atom number in 2D, and as a power law in 3D. In one-dimensional arrays, superradiance occurs due to destructive interference that effectively switches off certain decay channels, yielding a critical distance that saturates with atom number. Our results provide a guide to explore many-body decay in state-of-the art experimental setups.
In inverted atomic ensembles, photon-mediated interactions give rise to Dicke superradiance, a form of many-body decay that results in a rapid release of energy as a photon burst. While originally studied in pointlike ensembles, this phenomenon persists in extended ordered systems if the interparticle distance is below a certain bound. Here, we investigate Dicke superradiance in a realistic experimental setting using ordered arrays of alkaline-earth(-like) atoms, such as strontium and ytterbium. Such atoms offer exciting new opportunities for light-matter interactions, as their internal structure allows for trapping at short interatomic distances compared to their long-wavelength transitions, providing the potential for collectively enhanced dissipative interactions. Despite their intricate electronic structure, we show that two-dimensional arrays of these atomic species should exhibit many-body superradiance for achievable lattice constants. Moreover, superradiance effectively “closes” transitions, such that multilevel atoms become more two-level like. This occurs because the avalanchelike decay funnels the emission of most photons into the dominant transition, overcoming the single-atom decay ratios dictated by their fine structure and Zeeman branching. Our work represents an important step in harnessing alkaline-earth atoms as quantum optical sources and as platforms to explore many-body dissipative dynamics. Published by the American Physical Society 2024
Superradiance is an extensive cooperative spontaneous emission phenomenon, exhibited by some atomic collective-spin states. However, distinct initial states differ in their decay dynamics. Dicke states ∣j,m⟩|j,m\rangle∣j,m⟩ with distinct numbers of excitations n=m+jn=m+jn=m+j, driven by vacuum fluctuations, have their peak emission intensity shifted in time. Rotating Dicke states relative to the decay axis introduces an interesting parity structure that affects the pulse profile and photon correlations. Squeezed-bath prepared states undergo a squeezing-controlled crossover to the rotated Dicke states, making the emission character dependent on the amount of squeezing transferred from light to the atomic state. For semiclassical states with a macroscopic dipole moment, like the atomic coherent state, the emission intensity depends on their polarization. We present detailed results on the superradiant dynamics of a representative selection of states expanded in Dicke states to highlight the initial state as an independent dynamical control parameter. For large-NNN, we are able to predict fairly accurately the pulse profile in each case using the mean-field approximation, an approach based on the Fokker--Planck equation. We also present comparative results on the intensity correlation function, quantify the coherent and incoherent contributions of the emission, and contrast between small and large ensembles.
Spontaneous collective decay in incoherently driven atomic ensembles can generate macroscopic coherence in the steady state, as exemplified by steady-state superradiance in single-mode cavities. Whether spontaneous order persists beyond the Dicke limit, where competing collective decay channels and light propagation might preclude an ordered phase, remains an open question. We address it by analyzing incoherently pumped atoms coupled to one-dimensional electromagnetic baths through two models: a ring cavity with two bright decay channels, and a bidirectional waveguide where propagation additionally induces Hamiltonian dipole-dipole interactions. We find that both systems sustain steady-state phase order with intensity scaling as N2N^2N2, but that the order takes two qualitatively distinct forms, neither described by a single macroscopic dipole. In the ring cavity, individual trajectories spontaneously break mirror symmetry, locking the atomic phases and the emitted field to one of two chiral orders. In the waveguide, coherent interactions instead enforce a phase-separated steady state in which the two chiral orders coexist, each dominating one end of the array. Our results show how competition and propagation shape emergent order beyond the Dicke limit.
Recent advances in generating well controlled dense arrangements of individual atoms in free space have generated interest in understanding how the extended nature of these systems influences superradiance phenomena. Here, we provide an in-depth analysis on how space-dependent light shifts and decay rates induced by dipole-dipole interactions modify the steady-state properties of coherently driven arrays of quantum emitters. We characterize the steady-state phase diagram, with particular focus on the radiative properties in the steady state. Interestingly, we find that diverging from the well-established Dicke paradigm of equal all-to-all interactions significantly modifies the emission properties. In particular, the prominent quadratic scaling of the radiated light intensity with particle number in the steady state—a hallmark of steady-state Dicke superradiance—is entirely suppressed, resulting in only linear scaling with particle number. We show that this breakdown of steady-state superradiance occurs due to the emergence of additional dissipation channels that populate not only superradiant states but also subradiant ones. The additional contribution of subradiant dark states in the dynamics leads to a divergence in the time scales needed to achieve steady states. Building on this, we further show that measurements taken at finite times for extended atom ensembles reveal properties closely mirroring the idealized Dicke scenario. Published by the American Physical Society 2024