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arXiv:2106.01945 · Journal of High Energy Physics

Droplet-mediated long-range interfacial correlations. Exact field theory for entropic repulsion effects

Alessio Squarcini, Antonio Tinti

Published Mar 17, 2023• 7 citations
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Abstract

Abstract We consider near-critical two-dimensional statistical systems at phase coexistence on the half plane with boundary conditions leading to the formation of a droplet separating coexisting phases. General low-energy properties of two-dimensional field theories are used in order to find exact analytic results for one- and two-point correlation functions of both the energy density and order parameter fields. The subleading finite-size corrections are also computed and interpreted within an exact probabilistic picture in which interfacial fluctuations are characterized by the probability density of a Brownian excursion. The explicit analysis of the closed-form expression for order parameter correlations reveals the long-ranged character of interfacial correlations and their confinement within the interfacial region. The analysis of correlations is then carried out in momentum space through the notion of interface structure factor, which we extend to the case of systems bounded by a flat wall. The presence of the wall and its associated entropic repulsion leads to a specific term in the interface structure factor which we identify.

DOI
10.1007/jhep03(2023)123

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Abstract We consider near-critical two-dimensional statistical systems at phase coexistence on the half plane with boundary conditions leading to the formation of a droplet separating coexisting phases. General low-energy properties of two-dimensional field theories are used in order to find exact analytic results for one- and two-point correlation functions of both the energy density and order parameter fields. The subleading finite-size corrections are also computed and interpreted within an exact probabilistic picture in which interfacial fluctuations are characterized by the probability density of a Brownian excursion. The explicit analysis of the closed-form expression for order parameter correlations reveals the long-ranged character of interfacial correlations and their confinement within the interfacial region. The analysis of correlations is then carried out in momentum space through the notion of interface structure factor, which we extend to the case of systems bounded by a flat wall. The presence of the wall and its associated entropic repulsion leads to a specific term in the interface structure factor which we identify.
Abstract We consider near-critical two-dimensional statistical systems with boundary conditions inducing phase separation on the strip. By exploiting low-energy properties of two-dimensional field theories, we compute arbitrary n-point correlation of the order parameter field. Finite-size corrections and mixed correlations involving the stress tensor trace are also discussed. As an explicit illustration of the technique, we provide a closed-form expression for a three-point correlation function and illustrate the explicit form of the long-ranged interfacial fluctuations as well as their confinement within the interfacial region.
A long-standing problem in condensed matter physics concerns the nature of the critical wetting phase transition in the Ising model or, more generally, in 3D systems with short-ranged forces.This is of fundamental interest because 3D corresponds to the upper critical dimension of the transition and it is not clear a priori whether the behaviour of the system will be mean-field-like or fluctuation-dominated.Renormalization group studies of the standard coarse-grained effective interfacial Hamiltonian model famously predict strong non-universal critical exponents which depend on the value of the so-called wetting parameter ω.However, these predictions are at odds with extensive Monte Carlo simulations of wetting in the Ising model, due to Binder, Landau and coworkers, which appear to be more mean-field-like.Further amendments to the interfacial Hamiltonian, which included the presence of a position-dependent stiffness, worsened the problem by paradoxically predicting fluctuation-induced first-order wetting behaviour.Here we show from re-analysis of a microscopic Landau-Ginzburg-Wilson model of 3D short-ranged wetting that correlation functions are characterized by two diverging parallel length scales, not one, as previously thought.This has a simple diagrammatic explanation using a non-local interfacial Hamiltonian and yields a thermodynamically consistent theory of wetting in keeping with exact sum rules.The non-local model crucially contains long-ranged two-body interfacial interactions, characterized by the new length scale, which were missing in earlier treatments.For critical wetting the second length cuts off the spectrum of interfacial fluctuations determining the repulsion from the wall.We show how this corrects previous renormalization group predictions for fluctuation effects, based on local interfacial Hamiltonians.In particular, lowering the cut-off leads to a substantial reduction in the effective value of the wetting parameter controlling the non-universality and also prevents the transition being driven first-order.Quantitative comparison with the Ising model simulation studies is also made.
We consider two-dimensional (d = 2) systems with short-ranged microscopic interactions, where interface unbinding (wetting) transitions occur in the limit of vanishing temperature T .For T = 0 the transition is characterized by non-universal critical properties analogous to those established for thermal wetting transitions in d = 3, albeit with a redefined capillary parameter ω.Within a functional renormalization-group treatment of an effective interfacial model, we compute the finite-temperature phase diagram, exhibiting a line of interface unbinding transitions, terminating at T = 0 with an interfacial quantum-critical point.We identify distinct scaling regimes, reflecting the interplay between quantum and thermal interfacial fluctuations.A crossover line marking the onset of the quantum-critical regime is described by the d = 3 interfacial correlationlength exponent ν || .This potentially opens another way to investigate the non-universal character of ν || .On the other hand, the emergent interfacial quantum-critical regime shows no signatures of non-universality.
We consider variational (density functional) models of fluids confined in parallel-plate geometries (with walls situated in the planes z = 0 and z = L respectively) and focus on the structure of the pair correlation function . We show that for local variational models there exist two non-trivial identities relating both the transverse Fourier transform and the zeroth moment at different positions and . These relations form an algebra which severely restricts the possible form of the function . For the common situations in which the equilibrium one-body (magnetization/number density) profile exhibits an odd or even reflection symmetry in the plane, the algebra simplifies considerably, and is used to relate the correlation function to the finite-size excess free energy . We rederive non-trivial scaling expressions for the finite-size contribution to the free energy at bulk criticality and for systems where large-scale interfacial fluctuations are present. Extensions to non-planar geometries are also considered.