This thesis covers different subjects of nonlinear and quantum optics, studied in systems with scales smaller or com-parable to the wavelength of interest. The manuscript is divided into two parts. The first part of the manuscript dealswith several applications of optical nanofibers as a platform for light-matter interaction. In particular we will explore: thecoupling between a dipole placed on the surface of the nanofiber; the coupling between two parallel nanofibers; as well asthe mechanical properties of an optical nanofiber. In the second part of the manuscript, we will focus on solving two mainchallenges when working with emitters: one is the quantum efficiency of photoluminescence, the other is the attenuationduring transport of the photons generated in fiber telecom networks.
This thesis covers different subjects of nonlinear and quantum optics, studied in systems with scales smaller or com-parable to the wavelength of interest. The manuscript is divided into two parts. The first part of the manuscript dealswith several applications of optical nanofibers as a platform for light-matter interaction. In particular we will explore: thecoupling between a dipole placed on the surface of the nanofiber; the coupling between two parallel nanofibers; as well asthe mechanical properties of an optical nanofiber. In the second part of the manuscript, we will focus on solving two mainchallenges when working with emitters: one is the quantum efficiency of photoluminescence, the other is the attenuationduring transport of the photons generated in fiber telecom networks.
Abstract Recent advances in the coherent control of single quanta of light, photons , is a topic of prime interest, and is discussed under the banner of quantum photonics . In the last decade, the subwavelength diameter waist of a tapered optical fiber, referred to as an optical nanofiber , has opened promising new avenues in the field of quantum optics, paving the way toward a versatile platform for quantum photonics applications. The key feature of the technique is that the optical field can be tightly confined in the transverse direction while propagating over long distances as a guided mode and enabling strong interaction with the surrounding medium in the evanescent region. This feature has led to surprising possibilities to manipulate single atoms and fiber-guided photons, e.g. the efficient channeling of emission from single atoms and solid-state quantum emitters into the fiber-guided modes, high optical depth with a few atoms around the nanofiber, trapping atoms around a nanofiber, and atomic memories for fiber-guided photons. Furthermore, implementing a moderate longitudinal confinement in nanofiber cavities has enabled the strong coupling regime of cavity quantum electrodynamics to be reached, and the long-range dipole–dipole interaction between quantum emitters mediated by the nanofiber offers a platform for quantum nonlinear optics with an ensemble of atoms. In addition, the presence of a longitudinal component of the guided field has led to unique capabilities for chiral light–matter interactions on nanofibers. In this article, we review the key developments of the nanofiber technology toward a vision for quantum photonics on an all-fiber interface.
Optical nanofibers provide a versatile platform for exploring strong light-matter interactions at the single-quantum level, a central goal of quantum optics. Their subwavelength diameter supports tightly confined guided modes with strong evanescent fields, enabling efficient coupling between photons and nearby atoms. By incorporating fiber Bragg gratings, nanofibers can form fully fiber-integrated high-finesse cavities, combining strong atom-photon coupling with efficient and low-loss optical input-output interfacing in the setting of cavity quantum electrodynamics (QED). In parallel, nanofiber systems naturally realize waveguide QED, where atoms interact strongly with propagating photons in a one-dimensional geometry. In this review, we introduce the underlying physical principles, summarize key experimental techniques and representative phenomena, and discuss prospects for applications in quantum information processing, quantum networks, and related quantum technologies.
The study of atom-light interaction is a key element of quantum optics and a central part of atomic physics. Systems composed of atoms interacting with each other through the electromagnetic field can be used for studies from fundamental research to practical applications. Experimental realizations of these systems benefit from three distinct attributes: large atom-light coupling, trapping and control of atomic ensembles, and engineering and manipulation of the electromagnetic field. Optical waveguides provide a platform that achieves these three goals. In particular, optical nanofibers are an excellent candidate. They produce a high confinement of the electromagnetic field that improves atom-light coupling, guiding the field that mediates the interactions between atoms, while allowing trapping of the atoms close to it. This thesis describes the uses of an optical nanofiber for quantum optics experiments, demonstrating its possibilities for enabling special atom-light interactions. We trap atoms near the optical nanofiber surface, and characterize the trap in a non-destructive manner. We show how the presence of the nanofiber modifies the fundamental atomic property of spontaneous emission, by altering the electromagnetic environment of the atom. Finally, we use the nanofiber to prepare collective states of atoms around it. These states can radiate faster or slower than a single atom (superradiance and subradiance). The observation of subradiance of a few atoms, a rather elusive effect, evidences nanofibers as a strong candidate for future quantum optics experiments. Moreover, we show how the guided field mediates interaction between atoms hundreds of wavelengths apart, creating macroscopically delocalized collective states.
We study the interaction of emitters with a composite waveguide formed from two parallel optical nanofibers in regimes of experimental importance for atomic gases or solid-state emitters. Using the exact dyadic Green's function we comprehensively investigate the coupling efficiency and the fiber-induced Lamb shift accounting for variations in emitter positions and fiber configurations. This reveals coupling efficiencies and Purcell factors that are enhanced considerably beyond those using a single fiber waveguide, and robustness in the figures of merit. We finally investigate resonant dipole-dipole interactions and the generation of entanglement between two emitters mediated through the composite waveguide under excitation. We show that the concurrence can be enhanced for two fiber systems, such that entanglement may be present even in cases where it is zero for a single fiber. All-fiber systems are simple in construction and benefit from a wealth of existing telecommunications technologies, while enjoying strong couplings to emitters and offering interesting light-matter functionalities specific to slot waveguides. Published by the American Physical Society 2024
While a great amount of attention is being given to the development of nanodevices, both through academic research and private industry, the field is still on the verge. Progress hinges upon the development of tools and components that can precisely control the interaction between light and matter, and that can be efficiently integrated into nano-devices. Nanofibers are one of the most promising candidates for such purposes. However, in order to fully exploit their potential, a more intimate knowledge of how nanofibers interact with single neutral atoms must be gained. As we learn more about the properties of nanofiber modes, and the way they interface with atoms, and as the technology develops that allows them to be prepared with more precisely known properties, they become more and more adaptable and effective. The work presented in this thesis touches on many topics, which is testament to the broad range of applications and high degree of promise that nanofibers hold. For immediate use, we need to fully grasp how they can be best implemented as sensors, filters, detectors, and switches in existing nano-technologies. Areas of interest also include how they might be best exploited for probing atom-surface interactions, single-atom detection and single photon generation. Nanofiber research is also motivated by their potential integration into fundamental cold atom quantum experiments, and the role they can play there. Combining nanofibers with existing optical and quantum technologies is a powerful strategy for advancing areas like quantum computation, quantum information processing, and quantum communication. In this thesis I present a variety of theoretical work, which explores a range of the applications listed above. The first work presented concerns the use of the evanescent fields around a nanofiber to manipulate an existing trapping geometry and therefore influence the centre-of-mass dynamics of the atom. The second work presented explores interesting trapping geometries that can be achieved in the vicinity of a fiber in which just four modes are allowed to propagate. In a third study I explore the use of a nanofiber as a detector of small numbers of photons by calculating the rate of emission into the fiber modes when the fiber is moved along next to a regularly separated array of atoms. Also included are some results from a work in progress, where I consider the scattered field that appears along the nanofiber axis when a small number of atoms trapped along that axis are illuminated orthogonally; some interesting preliminary results are outlined. Finally, in contrast with the rest of the thesis, I consider some interesting physics that can be done in one of the trapping geometries that can be created around the fiber, here I explore the ground states of a phase separated two-component superfluid Bose-Einstein condensate trapped in a toroidal potential.
Waveguide-coupled nano-emitters for non-linear and quantum optics Cette thèse couvre différents sujets de l’optique non linéaire et quantique, étudiés dans des systèmes avec des échelles plus petites ou comparables à la longueur d’onde d’intérêt. Le manuscrit est divisé en deux parties. La première partie du manuscrit traite de plusieurs applications des nanofibres optiques en tant que plateforme d’interaction lumière-matière. En particulier, nous explorerons : le couplage entre d’un dipôle posé à la surface de la nanofibre ; le couplage entre deux nanofibres parallèles ; ainsi que les propriétés mécaniques d’une nanofibre optique. Dans la deuxième partie du manuscrit, nous nous concentrerons sur la résolution de deux principaux défis lorsque l’on travaille avec des émetteurs : l’un est le rendement quantique de photoluminescence, l’autre est l’atténuation lors du transport des photons générés dans les réseaux télécom fibrés.