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arXiv:2105.02105 · Physical Review A

Spin dynamical decoupling for generating macroscopic superpositions of a free-falling nanodiamond

Benjamin D. Wood, Sougato Bose, Gavin W. Morley

Published Jan 31, 2022• 23 citations
arXivHTMLPDF

Abstract

Levitated nanodiamonds containing negatively charged nitrogen-vacancy centers $({\text{NV}}^{\ensuremath{-}})$ have been proposed as a platform to generate macroscopic spatial superpositions. Requirements for this include having a long ${\text{NV}}^{\ensuremath{-}}$ spin coherence time, which necessitates formulating a dynamical decoupling strategy in which the regular spin flips do not cancel the growth of the superposition through the Stern-Gerlach effect in an inhomogeneous magnetic field. Here, we propose a scheme to place a $250\text{\ensuremath{-}}\mathrm{n}\mathrm{m}$-diameter diamond in a superposition with spatial separation of over $250\phantom{\rule{0.16em}{0ex}}\mathrm{n}\mathrm{m}$, while incorporating dynamical decoupling. We achieve this by letting a diamond fall for $2.4\phantom{\rule{0.16em}{0ex}}\mathrm{m}$ through a magnetic structure, including $1.13\phantom{\rule{0.16em}{0ex}}\mathrm{m}$ in an inhomogeneous region generated by magnetic teeth.

DOI
10.1103/physreva.105.012824

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Levitated nanodiamonds containing negatively charged nitrogen-vacancy centers (NV\ensuremath−)({\text{NV}}^{\ensuremath{-}})(NV\ensuremath−) have been proposed as a platform to generate macroscopic spatial superpositions. Requirements for this include having a long NV\ensuremath−{\text{NV}}^{\ensuremath{-}}NV\ensuremath− spin coherence time, which necessitates formulating a dynamical decoupling strategy in which the regular spin flips do not cancel the growth of the superposition through the Stern-Gerlach effect in an inhomogeneous magnetic field. Here, we propose a scheme to place a 250\ensuremath-nm250\text{\ensuremath{-}}\mathrm{n}\mathrm{m}250\ensuremath-nm-diameter diamond in a superposition with spatial separation of over 250nm250\phantom{\rule{0.16em}{0ex}}\mathrm{n}\mathrm{m}250nm, while incorporating dynamical decoupling. We achieve this by letting a diamond fall for 2.4m2.4\phantom{\rule{0.16em}{0ex}}\mathrm{m}2.4m through a magnetic structure, including 1.13m1.13\phantom{\rule{0.16em}{0ex}}\mathrm{m}1.13m in an inhomogeneous region generated by magnetic teeth.
A free-falling nanodiamond containing a nitrogen vacancy centre in a spin superposition should experience a superposition of forces in an inhomogeneous magnetic field. We propose a practical design that brings the internal temperature of the diamond to under 10 K. This extends the expected spin coherence time from 2 ms to 500 ms, so the spatial superposition distance could be increased from 0.05 nm to over 1 μμμm, for a 1 μμμm diameter diamond and a magnetic inhomogeneity of only 104^44 T/m. The low temperature allows single-shot spin readout, reducing the number of nanodiamonds that need to be dropped by a factor of 10,000. We also propose solutions to a generic obstacle that would prevent such macroscopic superpositions.
There is significant interest in potential experimental tests of macroscopic quantum effects, both to test potential modifications to quantum theory and to probe the quantum nature of gravity. A proposed platform with which to generate the required macroscopic quantum spatial superposition is a nanodiamond containing a negatively charged nitrogen vacancy (NV-) centre. In this review, methods to fabricate nanodiamonds containing NV­suitable for these quantum applications are discussed. The proposed probes of the macroscopic limits of quantum theory are presented along with the spin physics of the NV- centre relevant to those tests.
We propose a current-carrying-chip scheme for generating spatial quantum superpositions using a levitating nanodiamond with a built-in nitrogen-vacancy (NV) centre defect. Our setup is quite versatile and we aim to create the superposition for a mass range of 10−19 kg<m<10−15 kg10^{-19}~{\rm kg}< m< 10^{-15}~{\rm kg}10−19 kg<m<10−15 kg and a superposition size O(10)μm<Δx<O(1)nm{\cal O}(10) {\rm μm} < Δx < {\cal O}(1){\rm nm}O(10)μm<Δx<O(1)nm, respectively, in t≤0.1t\leq 0.1t≤0.1s, depending on the position we launch from the center of the diamagnetic trap. We provide an in-depth analysis of two parallel chips that can create levitation and spatial superposition along the xxx-axis, while producing a very tight trap in the yyy direction, and the direction of gravity, i.e., the zzz direction. Numerical simulations demonstrate that our setup can create a one-dimensional spatial superposition state along the x-axis. Throughout this process, the particle is stably levitated in the z-direction, and its motion is effectively confined in the y-direction for a Gaussian initial condition. This setup presents a viable platform for a diamagnetically levitated nanoparticle for a table-top experiment exploring the possibility of creating a macroscopic Schrödinger Cat state to test the quantum gravity induced entanglement of masses (QGEM) protocol.
We extend the concept of dynamical decoupling from spin to mechanical degrees of freedom of macroscopic objects, for application in interferometry. In this manner, the superposition of matter waves can be made resilient to many important sources of noise when these are driven along suitable paths in space. As a concrete implementation, we present the case of levitated (or free falling) nanodiamonds hosting a color center in a magnetic field gradient. We point out that these interferometers are inherently affected by diamagnetic forces, which restrict the separation of the superposed states to distances that scale with the inverse of the magnetic field gradient. Periodic forcing of the mechanical degree of freedom is shown to overcome this limitation, achieving a linear-in-time growth of the separation distance independent of the magnetic field gradient, while simultaneously protecting the coherence of the superposition from environmental perturbations.
A large spatial quantum superposition of size $O(1\text{--}10)\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\text{m}$ for mass $m\ensuremath{\sim}{10}^{\ensuremath{-}17}\text{--}{10}^{\ensuremath{-}14}$ kg is required to probe the foundations of quantum mechanics and test the classical and quantum nature of gravity via entanglement in a laboratory. In this paper, we will show that it is possible to accelerate the two spin states of a macroscopic nanocrystal sourced by the inhomogeneous nonlinear magnetic field in a Stern-Gerlach-type setup. We will assume that the electronic spin can be embedded at the center of the nanocrystal, such as the nitrogen-vacancy (NV) center of diamond. Our analysis will be generic to any dopant or any material. We will show that we can create a desired superposition size within 1–21\text{--}21–2 s by catapulting the trajectories of the two spin states with a modest magnetic field gradient and then recombine the trajectories for a coherent interference. We will show the demanding nature of the precision required in the magnetic field to recover a 9999%99 spin coherence confidence level at the moment of interference.
Nitrogen-vacancy (NV) centers in nanodiamond offer a promising platform for quantum information processing due to their room-temperature spin coherence and optical addressability. However, scalable quantum processors remain limited by the challenge of achieving strong, controllable interactions between distant NV spins. Here, we propose a scalable architecture utilizing optically levitated nanodiamond arrays, where torsional vibrations mediate the coherent coupling between the embedded NV centers. By optimizing the shape of ellipsoidal nanoparticles, we achieve a light-induced coupling strength exceeding 119 kHz between torsional modes of the distant levitated nanodiamonds, which are two orders of magnitude larger than the typical decoherence rates in this system. This strong interaction, combined with magnetic-field-enabled spin-torsion coupling, establishes an effective interaction between the spatially separated NV centers in the distant nanodiamonds. Numerical simulations confirm that dynamic decoupling can suppress both thermal noise and spin dephasing, enabling two-qubit gates with fidelity exceeding 99%. This work provides a foundation for reconfigurable quantum hybrid systems, with potential applications in rotational sensing and programmable quantum processing.