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arXiv:2105.02075 · Physical Review Letters

Quantum Entanglement from Classical Trajectories

Johan E. Runeson, Jeremy O. Richardson

Published Dec 15, 2021• 17 citations
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Abstract

A long-standing challenge in mixed quantum-classical trajectory simulations is the treatment of entanglement between the classical and quantal degrees of freedom. We present a novel approach that describes the emergence of entangled states entirely in terms of independent and deterministic Ehrenfest-like classical trajectories. For a two-level quantum system in a classical environment, this is derived by mapping the quantum system onto a path-integral representation of a spin 1/2. We demonstrate that the method correctly accounts for coherence and decoherence and thus reproduces the splitting of a wave packet in a nonadiabatic scattering problem. This discovery opens up a new class of simulations as an alternative to stochastic surface-hopping, coupled-trajectory, or semiclassical approaches.

DOI
10.1103/physrevlett.127.250403

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A long-standing challenge in mixed quantum-classical trajectory simulations is the treatment of entanglement between the classical and quantal degrees of freedom. We present a novel approach that describes the emergence of entangled states entirely in terms of independent and deterministic Ehrenfest-like classical trajectories. For a two-level quantum system in a classical environment, this is derived by mapping the quantum system onto a path-integral representation of a spin 1/2. We demonstrate that the method correctly accounts for coherence and decoherence and thus reproduces the splitting of a wave packet in a nonadiabatic scattering problem. This discovery opens up a new class of simulations as an alternative to stochastic surface-hopping, coupled-trajectory, or semiclassical approaches.
A long-standing challenge in mixed quantum-classical trajectory simulations is the treatment of entanglement between the classical and quantal degrees of freedom. We present a novel approach which describes the emergence of entangled states entirely in terms of independent and deterministic Ehrenfest-like classical trajectories. For a two-level quantum system in a classical environment, this is derived by mapping the quantum system onto a path-integral representation of a spin-1/2. We demonstrate that the method correctly accounts for coherence and decoherence and thus reproduces the splitting of a wavepacket in a nonadiabatic scattering problem. This discovery opens up a new class of simulations as an alternative to stochastic surface-hopping, coupled-trajectory or semiclassical approaches.
We study the semiclassical Ehrenfest trajectories in open quantum systems. We first give a self-contained derivation of the Fokker--Planck equation that governs the time evolution of the mixing measure for a Gaussian mixture. Then, we embed the generalized Ehrenfest theorem recently obtained for open quantum systems into this phase-space picture to study the time evolution of the expectations of observables with respect to the Gaussian mixture. We show how the coherent and irreversible contributions are separated in the frictionless harmonic regime relevant to the semiclassical approximation. Our work provides a transparent phase-space interpretation of the emergence of classical trajectories in open quantum dynamics.
We present a novel quantum-classical approach to nonadiabatic dynamics, deduced from the coupled electronic and nuclear equations in the framework of the exact factorization of the electron-nuclear wave function. The method is based on the quasiclassical interpretation of the nuclear wave function, whose phase is related to the classical momentum and whose density is represented in terms of classical trajectories. In this approximation, electronic decoherence is naturally induced as an effect of the coupling to the nuclei and correctly reproduces the expected quantum behavior. Moreover, the splitting of the nuclear wave packet is captured as a consequence of the correct approximation of the time-dependent potential of the theory. This new approach offers a clear improvement over Ehrenfest-like dynamics. The theoretical derivation presented in this Letter is supported by numerical results that are compared to quantum mechanical calculations.
We study a general bipartite quantum system consisting of a spin interacting with a bosonic field, with the initial state prepared as the product of a spin coherent state and a canonical coherent state. Our goal is to develop a semiclassical framework to describe the entanglement dynamics between these two subsystems. Using appropriate approximations, we derive a semiclassical expression for the entanglement entropy that depends exclusively on the trajectories of the underlying classical description. By analytically extending the classical phase space into the complex domain, we identify additional complex trajectories that significantly improve the accuracy of the semiclassical description. The inclusion of these complex trajectories allows us to capture the entanglement dynamics with remarkable precision, even well beyond the Ehrenfest time. The approach is illustrated with a representative example, where the role of real and complex trajectories in reproducing the quantum entanglement entropy is explicitly demonstrated.
We present a formulation for the emergence of classical dynamics in a quantum world using a path integral approach that incorporates continuous measurements. Our approach complements decoherence and coarse-grained quantum-to-classical transition frameworks. The path-integral formulation provides the joint statistics of a sequence of measurements, with each Feynman path picking up an additional random phase. Its magnitude is proportional to the measurement strength, and we give conditions under which the dominant contribution to the probability amplitude comes from trajectories near classical paths. Information proliferates across the environment, a key feature of quantum Darwinism, via plane-wave probe scattering. Extending to repeated measurements, we show that in the continuous limit each system trajectory picks up an additional phase due to momentum kicks from the probes--the origin of the back-action force. We provide conditions under which measurements yield enough ``which-path'' information while keeping the wave packet localized. This allows the quantum-to-classical transition to be described from individual measurement records, complementing the ensemble description from density matrices. We further show that the same scattering that decoheres a trajectory heats it, tying decoherence and measurement back-action together. This bounds how redundantly an individual classical trajectory can be recorded before back-action randomises it into Brownian motion. For a trapped particle, the ceiling is fixed by the resolution measured in units of the zero-point motion. It is not restrictive for macroscopic systems; it collapses to a single record where the semiclassical description of a trajectory fails, delimiting the regime in which objective classical trajectories exist. The deterministic-to-Brownian crossover is accessible in levitated optomechanics.
Abstract We consider the dynamics of interacting quantum and classical systems in the Heisenberg representation. Unlike the usual construction in standard quantum mechanics, mixed quantum-classical systems involve the interplay of unitary operators acting on the quantum observables and the Lagrangian trajectories sweeping the classical degrees of freedom. This interplay reflects an intricate structure which is made particularly challenging by the backreaction excerpted on the classical trajectories by the quantum degrees of freedom. While the backreaction is underestimated in the common Ehrenfest model, more recent methodologies succeed in capturing this important effect by resorting to Koopman wavefunctions in classical mechanics. Luckily, both Ehrenfest and Koopman models enjoy a variational framework which is exploited here to unfold the geometric structure underlying quantum-classical coupling. A special role is played by the action of the diffeomorphic Lagrangian paths on a non-Abelian pure-gauge potential which comprises statistical correlations. After presenting the treatment in the simple case of Ehrenfest dynamics, we move on to the Koopman model and present the role of the backreaction terms therein. Finally, we compare both models in the context of pure-dephasing systems.