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arXiv:2104.06712 · Physical review. B./Physical review. B

Coexistence of vortex arrays and surface capillary waves in spinning prolate superfluid He4 nanodroplets

Martí Pi, José María Escartín, Francesco Ancilotto, M. Barranco

Published Sep 9, 2021• 11 citations
arXivHTMLPDF

Abstract

Within density functional theory, we have studied the interplay between vortex arrays and capillary waves in spinning prolate $^{4}\mathrm{He}$ droplets made of several thousand helium atoms. Surface capillary waves are ubiquitous in prolate superfluid $^{4}\mathrm{He}$ droplets, and depending on the size and angular momentum of the droplet, they may coexist with vortex arrays. We have found that the equilibrium configuration of small prolate droplets is vortex free, evolving towards vortex hosting as the droplet size increases. This result is in agreement with a recent experiment [O'Connell et al., Phys. Rev. Lett. 124, 215301 (2020)] that disclosed that vortex arrays and capillary waves coexist in the equilibrium configuration of very large drops. In contrast to viscous droplets executing rigid-body rotation, the stability phase diagram of spinning $^{4}\mathrm{He}$ droplets cannot be universally described in terms of dimensionless angular momentum and angular velocity variables: Instead, the rotational properties of superfluid helium droplets display a clear dependence on the droplet size and the number of vortices they host.

DOI
10.1103/physrevb.104.094509

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Within density functional theory, we have studied the interplay between vortex arrays and capillary waves in spinning prolate 4He^{4}\mathrm{He}4He droplets made of several thousand helium atoms. Surface capillary waves are ubiquitous in prolate superfluid 4He^{4}\mathrm{He}4He droplets, and depending on the size and angular momentum of the droplet, they may coexist with vortex arrays. We have found that the equilibrium configuration of small prolate droplets is vortex free, evolving towards vortex hosting as the droplet size increases. This result is in agreement with a recent experiment [O'Connell et al., Phys. Rev. Lett. 124, 215301 (2020)] that disclosed that vortex arrays and capillary waves coexist in the equilibrium configuration of very large drops. In contrast to viscous droplets executing rigid-body rotation, the stability phase diagram of spinning 4He^{4}\mathrm{He}4He droplets cannot be universally described in terms of dimensionless angular momentum and angular velocity variables: Instead, the rotational properties of superfluid helium droplets display a clear dependence on the droplet size and the number of vortices they host.
The angular momentum of rotating superfluid droplets originates from quantized vortices and capillary waves, the interplay between which remains to be uncovered. Here, the rotation of isolated submicrometer superfluid ^{4}He droplets is studied by ultrafast x-ray diffraction using a free electron laser. The diffraction patterns provide simultaneous access to the morphology of the droplets and the vortex arrays they host. In capsule-shaped droplets, vortices form a distorted triangular lattice, whereas they arrange along elliptical contours in ellipsoidal droplets. The combined action of vortices and capillary waves results in droplet shapes close to those of classical droplets rotating with the same angular velocity. The findings are corroborated by density functional theory calculations describing the velocity fields and shape deformations of a rotating superfluid cylinder.
Helium nanodroplets are considered ideal model systems to explore quantum hydrodynamics in self-contained, isolated superfluids. However, exploring the dynamic properties of individual droplets is experimentally challenging. In this work, we used single-shot femtosecond x-ray coherent diffractive imaging to investigate the rotation of single, isolated superfluid helium-4 droplets containing ~10(8) to 10(11) atoms. The formation of quantum vortex lattices inside the droplets is confirmed by observing characteristic Bragg patterns from xenon clusters trapped in the vortex cores. The vortex densities are up to five orders of magnitude larger than those observed in bulk liquid helium. The droplets exhibit large centrifugal deformations but retain axially symmetric shapes at angular velocities well beyond the stability range of viscous classical droplets.
We address the collision of two superfluid 4He droplets at non-zero initial relative velocities and impact parameters within the framework of liquid 4He time-dependent density functional theory at zero temperature. Despite the small size of these droplets (1000 He atoms in the merged droplet) imposed by computational limitations, we have found that quantized vortices may be readily nucleated for reasonable collision parameters. At variance with head-on collisions, where only vortex rings are produced, collisions with a non-zero impact parameter produce linear vortices that are nucleated at indentations appearing on the surface of the deformed merged droplet. Whereas for equal-size droplets, vortices are produced in pairs, an odd number of vortices can appear when the colliding droplet sizes are different. In all cases, vortices coexist with surface capillary waves. The possibility for collisions to be at the origin of vortex nucleation in experiments involving very large droplets is discussed. An additional surprising result is the observation of the drops coalescence even for grazing and distal collisions at relative velocities as high as 80 and 40 m/s, respectively, induced by the long-range van der Waals attraction between the droplets.
Mixed $^{3}\mathrm{He}\ensuremath{-}^{4}\mathrm{He}$ droplets may acquire angular momentum during their passage through the nozzle of the experimental apparatus, cooling down and undergoing isotopic segregation, developing a 3He^{3}\mathrm{He}3He crust surrounding a superfluid 4He^{4}\mathrm{He}4He core. Within density functional theory, we investigate their stability and the relations between their angular momenta and their shapes. We uncover a variety of behaviors where the interplay between the superfluid 4He^{4}\mathrm{He}4He core and the normal-fluid 3He^{3}\mathrm{He}3He coating leads to a scenario that both bears analogies with viscous rotating drops and displays new features such as configurations with a fissioned or three-lobed 4He^{4}\mathrm{He}4He core, or with multiply charged vortices.
Within density functional theory, we investigate stationary many-vortex structures in a rotating 4He^{4}\mathrm{He}4He nanocylinder at zero temperature. We compute the stability diagram and compare our results with the classical model of vortical lines in an inviscid and incompressible fluid. Scaling the results to millimeter-size buckets, they can be compared with experiments on vortex arrays conducted in the past. Motivated by recent experiments that have used atomic impurities as a means of visualizing vortices in superfluid 4He^{4}\mathrm{He}4He droplets, we have also considered the formation of chains of xenon atoms along a vortex line and the interaction between xenon atoms inside the same vortex and on different neighboring vortex lines.
Helium nanodroplets are considered ideal model systems to explore quantum hydrodynamics in self-contained, isolated superfluids. Rotation of a superfluid droplet is manifested as a collection of quantum vortices. Here, the authors use single-shot femtosecond X-ray coherent diffractive imaging to investigate the shapes and vorticity of rotating superfluid 4{}^{4}4He droplets. They find that most of the diffraction contours exhibit noticeable ellipticity. A smaller but still significant number of distorted diffraction contours are marked by regions of high intensity concentrated along the direction of the long axis in the diffraction image, indicating the presence of extremely deformed 4{}^{4}4He droplets. Forward modeling of the diffraction images shows that the shapes of superfluid 4{}^{4}4He droplets are very similar to their classical counterparts. In particular, the existence of both axially symmetric (oblate) and, for higher angular momenta, two-lobed (triaxial prolate) droplets is revealed. The latter shapes are strongly deformed compared to the spheroidal bodies that are expected for smaller rotational speeds. The observed shapes provide direct access to the droplet angular momenta, angular velocities, and estimated number of quantum vortices inside the droplets.