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arXiv:2104.05748 · New Journal of Physics

Observation of phase synchronization and alignment during free induction decay of quantum spins with Heisenberg interactions

Patrick Vorndamme, Heinz–Jürgen Schmidt, Christian Schröder, Jürgen Schnack

Published Jul 29, 2021• 7 citations
arXivHTMLPDF

Abstract

Abstract Equilibration of observables in closed quantum systems that are described by a unitary time evolution is a meanwhile well-established phenomenon apart from a few equally well-established exceptions. Here we report the surprising theoretical observation that integrable as well as non-integrable spin rings with nearest-neighbor or long-range isotropic Heisenberg interaction not only equilibrate but moreover also synchronize the directions of the expectation values of the individual spins. We highlight that this differs from spontaneous synchronization in quantum dissipative systems. Here, we observe mutual synchronization of local spin directions in closed systems under unitary time evolution. In our numerical simulations, we investigate the free induction decay of an ensemble of up toN= 25 quantum spins withs= 1/2 each by solving the time-dependent Schrödinger equation numerically exactly. Our findings are related to, but not fully explained by conservation laws of the system. Even if we cannot provide a full understanding of the phenomenon, it is very robust against for instance random fluctuations of the Heisenberg couplings and inhomogeneous magnetic fields. The observed synchronization is independent of whether the interaction is ferro- or antiferromagnetic. Synchronization is not observed with strong enough symmetry-breaking interactions such as the dipolar interaction. We also compare our results to closed-system classical spin dynamics which does not exhibit phase synchronization due to the lack of entanglement and since the fixed magnitude of individual classical spins effectively acts like additionalNconservation laws.

DOI
10.1088/1367-2630/ac18df

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Abstract Equilibration of observables in closed quantum systems that are described by a unitary time evolution is a meanwhile well-established phenomenon apart from a few equally well-established exceptions. Here we report the surprising theoretical observation that integrable as well as non-integrable spin rings with nearest-neighbor or long-range isotropic Heisenberg interaction not only equilibrate but moreover also synchronize the directions of the expectation values of the individual spins. We highlight that this differs from spontaneous synchronization in quantum dissipative systems. Here, we observe mutual synchronization of local spin directions in closed systems under unitary time evolution. In our numerical simulations, we investigate the free induction decay of an ensemble of up toN= 25 quantum spins withs= 1/2 each by solving the time-dependent Schrödinger equation numerically exactly. Our findings are related to, but not fully explained by conservation laws of the system. Even if we cannot provide a full understanding of the phenomenon, it is very robust against for instance random fluctuations of the Heisenberg couplings and inhomogeneous magnetic fields. The observed synchronization is independent of whether the interaction is ferro- or antiferromagnetic. Synchronization is not observed with strong enough symmetry-breaking interactions such as the dipolar interaction. We also compare our results to closed-system classical spin dynamics which does not exhibit phase synchronization due to the lack of entanglement and since the fixed magnitude of individual classical spins effectively acts like additionalNconservation laws.
Isotropic but otherwise largely arbitrary Heisenberg models in the presence of a homogeneous magnetic field are considered, including various integrable, nonintegrable, as well as disordered examples, and not necessarily restricted to one dimension or short-range interactions. Taking for granted that the nonequilibrium initial condition and the spectrum of the field-free model satisfy some very weak requirements, expectation values of generic observables are analytically shown to exhibit permanent long-time oscillations, thus ruling out equilibration. If the model (but not necessarily the initial condition) is translationally invariant, the long-time oscillations are moreover shown to exhibit synchronization in the long run, meaning that they are invariant under arbitrary translations of the observable. Analogous long-time oscillations are also recovered for temporal correlation functions when the system is already at thermal equilibrium from the outset, thus realizing a so-called time crystal.
Abstract In nature, instances of synchronisation abound across a diverse range of environments. In the quantum regime, however, synchronisation is typically observed by identifying an appropriate parameter regime in a specific system. In this work we show that this need not be the case, identifying conditions which, when satisfied, guarantee that the individual constituents of a generic open quantum system will undergo completely synchronous limit cycles which are, to first order, robust to symmetry-breaking perturbations. We then describe how these conditions can be satisfied by the interplay between several elements: interactions, local dephasing and the presence of a strong dynamical symmetry—an operator which guarantees long-time non-stationary dynamics. These elements cause the formation of entanglement and off-diagonal long-range order which drive the synchronised response of the system. To illustrate these ideas we present two central examples: a chain of quadratically dephased spin-1s and the many-body charge-dephased Hubbard model. In both cases perfect phase-locking occurs throughout the system, regardless of the specific microscopic parameters or initial states. Furthermore, when these systems are perturbed, their nonlinear responses elicit long-lived signatures of both phase and frequency-locking.
ABSTRACT Quantum synchronization, characterized by correlated dynamics in coupled quantum systems, is an active field with profound implications for quantum technologies. This work investigates near‐perfect spontaneous quantum phase synchronization (QPS) within a spin‐1/2 Heisenberg chain system, a cornerstone in the study of quantum magnetism, enhancing both fundamental insights and technological prospects. We explore the dependencies of synchronization time on interaction strength and system size. Moreover, our analysis confirms the resilience of QPS against random frequency and interaction fluctuations. Intriguingly, we reveal that dephasing can enhance spontaneous QPS, presenting a paradoxical avenue for synchronization improvement. We demonstrate that QPS can attain Heisenberg‐limit precision and discuss practical implementations using superconducting quantum circuits. Our results enrich the understanding of quantum synchronization mechanisms and highlight their potential in enhancing the functionality of quantum systems, essential for both natural and engineered systems.
An important step towards a comprehensive understanding of far-from-equilibrium dynamics of quantum many-body systems is the identification of unifying features that are independent of microscopic details of the system. We experimentally observe such robust features in the magnetization relaxation dynamics of disordered Heisenberg XX, XXZ, and Ising Hamiltonians. We realize these Heisenberg spin models with tunable anisotropy parameter and power-law interactions in an ensemble of Rydberg atoms by encoding the spin in suitable Rydberg state combinations. We consistently observe stretched-exponential relaxation of magnetization for all considered spin models, collapsing onto a single curve after appropriate rescaling of time. This robust short-time relaxation behavior is explained by a perturbative treatment that exploits the strong disorder in pairwise couplings, which leads to a description in terms of approximately independent pairs of spins. In numerical simulations of small systems, we show that these pairs of spins constitute approximate local integrals of motion, which remain at least partially conserved on a timescale exceeding the duration of the relaxation dynamics of the magnetization. Published by the American Physical Society 2024
We study the out-of-equilibrium dynamics of one-dimensional quantum Ising-like systems, arising from sudden quenches of the Hamiltonian parameter ggg driving quantum transitions between disordered and ordered phases. In particular, we consider quenches to values of ggg around the critical value gc{g}_{c}gc​, and mainly address the question whether, and how, the quantum transition leaves traces in the evolution of the transverse and longitudinal magnetizations during such a deep out-of-equilibrium dynamics. We shed light on the emergence of singularities in the thermodynamic infinite-size limit, likely related to the integrability of the model. Finite systems in periodic and open boundary conditions develop peculiar power-law finite-size scaling laws related to revival phenomena, but apparently unrelated to the quantum transition, because their main features are generally observed in quenches to generic values of ggg. We also investigate the effects of dissipative interactions with an environment, modeled by a Lindblad equation with local decay and pumping dissipation operators within the quadratic fermionic model obtainable by a Jordan-Wigner mapping. Dissipation tends to suppress the main features of the unitary dynamics of closed systems. We finally address the effects of integrability breaking, due to further lattice interactions, such as in anisotropic next-to-nearest-neighbor Ising (ANNNI) models. We show that some qualitative features of the post-quench dynamics persist, in particular, the different behaviors when quenching to quantum ferromagnetic and paramagnetic phases, and the revival phenomena due to the finite size of the system.
We develop an excited-state real-space renormalization group (RSRG-X) formalism to describe the dynamics of conserved densities in randomly interacting spin-12\frac{1}{2}21​ systems. Our formalism is suitable for systems with U(1)\textrm{U}(1)U(1) and Z2\mathbb{Z}_2Z2​ symmetries, and we apply it to chains of randomly positioned spins with dipolar XX+YYXX+YYXX+YY interactions, as arise in Rydberg quantum simulators and other platforms. The formalism generates a sequence of effective Hamiltonians which provide approximate descriptions for dynamics on successively smaller energy scales. These effective Hamiltonians involve ``superspins'': two-level collective degrees of freedom constructed from (anti)aligned microscopic spins. Conserved densities can then be understood as relaxing via coherent collective spin flips. For the well-studied simpler case of randomly interacting nearest-neighbor XX+YYXX+YYXX+YY chains, the superspins reduce to single spins. Our formalism also leads to a numerical method capable of simulating the dynamics up to an otherwise inaccessible combination of large system size and late time. Focusing on disorder-averaged infinite-temperature autocorrelation functions, in particular the local spin survival probability Sp‾(t)\overline{S_p}(t)Sp​​(t), we demonstrate quantitative agreement in results between our algorithm and exact diagonalization (ED) at low but nonzero frequencies. Such agreement holds for chains with nearest-neighbor, next-nearest-neighbor, and long-range dipolar interactions. Our results indicate decay of Sp‾(t)\overline{S_p}(t)Sp​​(t) slower than any power law and feature no significant deviation from the ∼1/log⁡2(t)\sim 1/ \log^2(t)∼1/log2(t) asymptote expected from the infinite-randomness fixed-point of the nearest-neighbor model. We also apply the RSRG-X formalism to two-dimensional long-range systems of moderate size and find slow late-time decay of Sp‾(t)\overline{S_p}(t)Sp​​(t).