Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multiphoton events. We propose a scheme to overcome this purity-yield trade-off by suppressing multiphoton events in a cavity-enhanced SPDC via the photon-blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon yield to larger than $90\mathrm{%}$, while keeping the purity high, towards on-demand generation of single photons through the SPDC process. Our quasi-on-demand SPDC sources may boost single-photon-based quantum-information technology.
Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multiphoton events. We propose a scheme to overcome this purity-yield trade-off by suppressing multiphoton events in a cavity-enhanced SPDC via the photon-blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon yield to larger than 90\mathrm{%}, while keeping the purity high, towards on-demand generation of single photons through the SPDC process. Our quasi-on-demand SPDC sources may boost single-photon-based quantum-information technology.
Single-photon sources that emit only one photon at a time with high yield are important for security and efficiency in quantum communication and computation, respectively. One method to develop the desired single-photon source is through entangled single-photon pairs from spontaneous parametric down-conversion (SPDC) crystals where detection of idler photons “heralds” the presence of signal photons. If the SPDC crystal is pumped with weak intensity laser, high purity heralded single photons can be produced at the cost of low yield. Increasing the yield by using stronger laser intensity inevitably decreases the purity due to the presence of multiple photons. Here, we propose a conceptual method to overcome this trade-off between single-photon purity and single-photon yield. Our setup consists of a weakly pumped SPDC crystal seeded with strong coherent states (CS) at the idler mode. Clicks on a click detector at the idler mode conditionally prepare a superposition state of zero-, one-, and two-photon Fock states (FS) at the signal mode. By employing repeated processes of infinitesimal displacement (ID) and two-photon elimination (PE), we can obtain a final state of one-photon FS. Based on the heralding probability (single-photon yield) and single-photon fidelity (single-photon purity), we found that our method transforms the initial state with high heralding probability but low single-photon fidelity (near minimum) to a final state with high heralding probability and high single-photon fidelity (maximum). Furthermore, we discussed the conditions required for the experimental implementations of the processes. Thus, our work paves the way to producing heralded single photons with high purity and yield in SPDC sources.
Cavity-enhanced spontaneous parametric down-conversion (SPDC) can be used to implement heralded single-photon sources with narrow bandwidth down to tens of megahertz, thus compatible with atom-based quantum memories. In this work, we propose and study the cavities that are either singly resonant at the frequency of only one of the generated photons or doubly resonant at the frequency of one generated photon and for the pump field. We derive analytical expressions for the generation rate and the spectral brightness as a function of the main structure parameters. Our analysis shows that by exploiting counterpropagating SPDC inside a cavity with properly designed distributed Bragg reflectors, pure narrow-band heralded single photons can be generated. In particular, when a pulsed pump illuminates a 1-mm-long singly resonant cavity, the bandwidth of the resonant and the nonresonant photons will be 120 MHz and 5.7 GHz, respectively, with heralded single-photon purity as high as 0.993. Due to its small absorption probability inside the cavity, the heralding efficiency can approach unity if the nonresonant partner is used as a heralded single photon. Finally, we also show that continuous-wave excitation of a 1-cm-long cavity resonant for the pump and copropagating fields can provide photon pairs in a narrow bandwidth of 10 MHz with spectral brightness as high as $2\ifmmode\times\else\texttimes\fi{}{10}^{6}$ $({\text{s}\phantom{\rule{4.pt}{0ex}}\text{mW}\phantom{\rule{4.pt}{0ex}}\text{MHz})}^{\ensuremath{-}1}$. This source can efficiently couple with quantum memories and can find applications in quantum information processing and communication.
Photons have proven to be excellent carriers of quantum information, and play essential roles in numerous quantum information processing (QIP) applications. In particular, heralded single- photon sources via spontaneous parametric-down conversion (SPDC) have been a key technology for demonstrating small-scale QIP, yet their low generation efficiency is a critical limitation for further scaling up optical QIP technology. In order to efficiently overcome the probabilistic nature of SPDC, here we demonstrate time multiplexing for up to 30 time slots of a periodically pumped heralded single-photon source, using a switchable low-loss optical storage cavity. We observe a maximum single-photon probability of 38.6% in periodic output time windows, corresponding to 6 times enhancement over a non-multiplexed source, but with no increase in the contribution of unwanted multi-photon events. Combining this time-multiplexing technique with a heralded source producing pure single-photon states should enable larger scale optical QIP systems than ever realized.
This thesis presents experimental progress towards highly efficient generation of cavity- enhanced, narrow-band multiphotons using spontaneous parametric downconversion. It also suggests theoretical proposals for new applications of multiphoton sources in quantum information technology. Photons prepared in Fock states, with a well-defined number of particles, are the essence of the quantum nature of light, and their unique nonclassical properties help us to develop quantum information technology. The generation of Fock states has been most commonly achieved by using spontaneous parametric down-conversion (SPDC) through the χ(2) nonlinearity in bulk crystals. During the SPDC process the nonlinear crystal emits photon-number correlated modes, and a photon-number- resolving measurement in one mode heralds the preparation of the other mode in a Fock state. The fidelity and the success rate of Fock state generation is limited by the multimode nature of SPDC emission. In this thesis, I will investigate the use of cavity-enhanced SPDC modes for higher fidelity photon pair generation, in which the well defined mode of the cavity is enhanced and results in the narrow-band source of the heralded single-photons with up to 80% heralding efficiency. The heralding efficiency is defined as the ratio between number of coincidences and single events on the heralding mode. The photon-number-resolving ability of high-quantum-efficiency transition edge sensors is used for the heralding and detection. We further discuss the feasibility of Fock state generation with higher photon numbers upon improving the data acquisition and analysis techniques. We also demonstrate and implement an interferometry scheme that exploit the phase of the photon and is capable of reading boundless bits of digital information using a single photon. This thesis also introduces new theoretical proposals for using Fock states to obtain quantum advantages for various quantum information applications, here to increase the efficiency in reading out information stored in a classical digital memory and to discriminate optical phases with lower error rates than is feasible with classical protocols.
The high-purity single-photon source plays an important role in the field of quantum information. Usually, it is generated through spontaneous parametric down-conversion process. In this paper, we investigate and summarize a few approaches on obtaining single-photon sources with a high purity using either PPKTP or PPLN nonlinear crystals. Moreover, we present improved schemes to increase the purity based on existing work, corresponding applicable conditions and procedures are discussed and analyzed. Besides, we carry out numerical simulations and show that nearly perfect purity can be reached even without using any filters. Therefore, this work might provide valuable references for the generation and application of high purity single-photon sources.
An on-demand single-photon source is a fundamental building block in quantum science and technology. We experimentally demonstrate the proof of concept for a scheme to generate on-demand single photons via actively multiplexing several heralded photons probabilistically produced from pulsed spontaneous parametric down-conversions (SPDCs). By utilizing a four-photon-pair source, an active feed-forward technique, and an ultrafast single-photon router, we show a fourfold enhancement of the output photon rate. Simultaneously, we maintain the quality of the output single-photon states, confirmed by correlation measurements. We also experimentally verify, via Hong-Ou-Mandel interference, that the router does not affect the indistinguishability of the single photons. Furthermore, we give numerical simulations, which indicate that photons based on multiplexing of four SPDC sources can outperform the heralding based on highly advanced photon-number-resolving detectors. Our results show a route for on-demand single-photon generation and the practical realization of scalable linear optical quantum-information processing.