Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2103.06246 · Nature Physics

Tuning of dipolar interactions and evaporative cooling in a three-dimensional molecular quantum gas

Jun-Ru Li, William G. Tobias, Kyle Matsuda, Calder Miller, Giacomo Valtolina, Luigi De Marco, Reuben R. W. Wang, Lucas Lassablière, Goulven Quéméner, John L. Bohn, Jun Ye

Published Sep 2, 2021• 103 citations
arXivHTMLPDF
DOI
10.1038/s41567-021-01329-6

Related papers

Controlling anisotropic dipolar interaction with shielding resonance in a 3D molecular quantum gas

Jun-Ru Li, W. A. Tobias, Kyle Matsuda +8 more

Bulletin of the American Physical Society•Jun 4, 2021•0 citations

Towards two-dimensional quantum gases of strongly dipolar molecules

Aden Z. Lam, Niccolò Bigagli, Claire Warner +2 more

Bulletin of the American Physical Society•May 31, 2018•0 citations

Controlling anisotropic dipolar interaction with shielding resonance in a three-dimensional molecular quantum gas

Jun-Ru Li, William G. Tobias, Kyle Matsuda +8 more

Ultracold polar molecules possess long-range, anisotropic, and tunable dipolar interactions, providing unique opportunities to probe novel quantum phenomena. However, experimental progress has been hindered by excessive two-body loss, which also limits further cooling via evaporation. Recent work shows the loss can be mitigated by confining molecules in a two-dimensional geometry. However, a general approach for tuning molecular interactions in a full three-dimensional (3D) stable system has been lacking. Here, we demonstrate the use of an electric field-induced shielding resonance to suppress the reactive loss by a factor of 30 while preserving elastic, long-range dipolar interactions in a bulk gas of ultracold 40K87Rb molecules in 3D. The favorable ratio of elastic to inelastic collisions enables direct thermalization, the rate of which depends on the angle between the collisional axis and the dipole orientation controlled by an external electric field. This is a direct manifestation of the anisotropic dipolar interaction. We further achieve dipolar-interaction-mediated evaporative cooling in 3D. This work demonstrates control of a long-lived bulk quantum gas system with tunable long-range interactions, paving the way for the study of collective quantum many-body physics.

•Mar 11, 2021•1 citation

Evaporation of microwave-shielded polar molecules to quantum degeneracy

Andreas Schindewolf, Roman Bause, Xing-Yan Chen +4 more

Abstract Ultracold polar molecules offer strong electric dipole moments and rich internal structure, which makes them ideal building blocks to explore exotic quantum matter 1–9 , implement quantum information schemes 10–12 and test the fundamental symmetries of nature 13 . Realizing their full potential requires cooling interacting molecular gases deeply into the quantum-degenerate regime. However, the intrinsically unstable collisions between molecules at short range have so far prevented direct cooling through elastic collisions to quantum degeneracy in three dimensions. Here we demonstrate evaporative cooling of a three-dimensional gas of fermionic sodium–potassium molecules to well below the Fermi temperature using microwave shielding. The molecules are protected from reaching short range with a repulsive barrier engineered by coupling rotational states with a blue-detuned circularly polarized microwave. The microwave dressing induces strong tunable dipolar interactions between the molecules, leading to high elastic collision rates that can exceed the inelastic ones by at least a factor of 460. This large elastic-to-inelastic collision ratio allows us to cool the molecular gas to 21 nanokelvin, corresponding to 0.36 times the Fermi temperature. Such cold and dense samples of polar molecules open the path to the exploration of many-body phenomena with strong dipolar interactions.

arXiv:2201.05143•Nature•Jul 27, 2022•170 citations

Universal Threshold Laws for Dipolar Evaporation of Molecular Fermi Gases

Kevin B. Xu, John L. Bohn, Reuben R. W. Wang

Fermi statistics suppress the elastic collisions that rethermalize a Fermi gas during evaporative cooling, creating a fundamental low-temperature bottleneck for producing quantum degenerate gases. We show that, for shielded single-component ultracold dipolar molecular Fermi gases in the Wigner threshold regime, this bottleneck is governed by universal threshold laws fixed by the effective dimensionality of the gas. In this regime, Fermi suppression of rethermalization scales quadratically with temperature in 3D but only linearly in 2D. Consequently, the thermalization-to-loss ratio is more favorable in 2D than in 3D, and these results suggest that 2D geometries are better suited for reaching deep degeneracy. We also present ab initio close-coupling calculations that agree well with experimental measurements on Fermi degenerate gases of KRb molecules, supporting our conclusions.

cond-mat.quant-gasCross-listedarXiv:2610.22639•Oct 19, 2026•0 citations

Dipolar evaporation of reactive molecules to below the Fermi temperature

Giacomo Valtolina, Kyle Matsuda, William G. Tobias +3 more

Abstract The control of molecules is key to the investigation of quantum phases, in which rich degrees of freedom can be used to encode information and strong interactions can be precisely tuned1. Inelastic losses in molecular collisions2–5, however, have greatly hampered the engineering of low-entropy molecular systems6. So far, the only quantum degenerate gas of molecules has been created via association of two highly degenerate atomic gases7, 8. Here we use an external electric field along with optical lattice confinement to create a two-dimensional Fermi gas of spin-polarized potassium–rubidium (KRb) polar molecules, in which elastic, tunable dipolar interactions dominate over all inelastic processes. Direct thermalization among the molecules in the trap leads to efficient dipolar evaporative cooling, yielding a rapid increase in phase-space density. At the onset of quantum degeneracy, we observe the effects of Fermi statistics on the thermodynamics of the molecular gas. These results demonstrate a general strategy for achieving quantum degeneracy in dipolar molecular gases in which strong, long-range and anisotropic dipolar interactions can drive the emergence of exotic many-body phases, such as interlayer pairing and p-wave superfluidity.

•Jan 1, 2020•93 citations
Ultracold polar molecules possess long-range, anisotropic, and tunable dipolar interactions, providing unique opportunities to probe novel quantum phenomena. However, experimental progress has been hindered by excessive two-body loss, which also limits further cooling via evaporation. Recent work shows the loss can be mitigated by confining molecules in a two-dimensional geometry. However, a general approach for tuning molecular interactions in a full three-dimensional (3D) stable system has been lacking. Here, we demonstrate the use of an electric field-induced shielding resonance to suppress the reactive loss by a factor of 30 while preserving elastic, long-range dipolar interactions in a bulk gas of ultracold 40K87Rb molecules in 3D. The favorable ratio of elastic to inelastic collisions enables direct thermalization, the rate of which depends on the angle between the collisional axis and the dipole orientation controlled by an external electric field. This is a direct manifestation of the anisotropic dipolar interaction. We further achieve dipolar-interaction-mediated evaporative cooling in 3D. This work demonstrates control of a long-lived bulk quantum gas system with tunable long-range interactions, paving the way for the study of collective quantum many-body physics.
Abstract Ultracold polar molecules offer strong electric dipole moments and rich internal structure, which makes them ideal building blocks to explore exotic quantum matter 1–9 , implement quantum information schemes 10–12 and test the fundamental symmetries of nature 13 . Realizing their full potential requires cooling interacting molecular gases deeply into the quantum-degenerate regime. However, the intrinsically unstable collisions between molecules at short range have so far prevented direct cooling through elastic collisions to quantum degeneracy in three dimensions. Here we demonstrate evaporative cooling of a three-dimensional gas of fermionic sodium–potassium molecules to well below the Fermi temperature using microwave shielding. The molecules are protected from reaching short range with a repulsive barrier engineered by coupling rotational states with a blue-detuned circularly polarized microwave. The microwave dressing induces strong tunable dipolar interactions between the molecules, leading to high elastic collision rates that can exceed the inelastic ones by at least a factor of 460. This large elastic-to-inelastic collision ratio allows us to cool the molecular gas to 21 nanokelvin, corresponding to 0.36 times the Fermi temperature. Such cold and dense samples of polar molecules open the path to the exploration of many-body phenomena with strong dipolar interactions.
Fermi statistics suppress the elastic collisions that rethermalize a Fermi gas during evaporative cooling, creating a fundamental low-temperature bottleneck for producing quantum degenerate gases. We show that, for shielded single-component ultracold dipolar molecular Fermi gases in the Wigner threshold regime, this bottleneck is governed by universal threshold laws fixed by the effective dimensionality of the gas. In this regime, Fermi suppression of rethermalization scales quadratically with temperature in 3D but only linearly in 2D. Consequently, the thermalization-to-loss ratio is more favorable in 2D than in 3D, and these results suggest that 2D geometries are better suited for reaching deep degeneracy. We also present ab initio close-coupling calculations that agree well with experimental measurements on Fermi degenerate gases of KRb molecules, supporting our conclusions.
Abstract The control of molecules is key to the investigation of quantum phases, in which rich degrees of freedom can be used to encode information and strong interactions can be precisely tuned1. Inelastic losses in molecular collisions2–5, however, have greatly hampered the engineering of low-entropy molecular systems6. So far, the only quantum degenerate gas of molecules has been created via association of two highly degenerate atomic gases7, 8. Here we use an external electric field along with optical lattice confinement to create a two-dimensional Fermi gas of spin-polarized potassium–rubidium (KRb) polar molecules, in which elastic, tunable dipolar interactions dominate over all inelastic processes. Direct thermalization among the molecules in the trap leads to efficient dipolar evaporative cooling, yielding a rapid increase in phase-space density. At the onset of quantum degeneracy, we observe the effects of Fermi statistics on the thermodynamics of the molecular gas. These results demonstrate a general strategy for achieving quantum degeneracy in dipolar molecular gases in which strong, long-range and anisotropic dipolar interactions can drive the emergence of exotic many-body phases, such as interlayer pairing and p-wave superfluidity.