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arXiv:2103.04687 · Quantum

Lieb's Theorem and Maximum Entropy Condensates

Joseph Tindall, Frank Schlawin, Michael A. Sentef, Dieter Jaksch

Published Dec 23, 2021• 13 citations
arXivHTMLPDF

Abstract

Coherent driving has established itself as a powerful tool for guiding a many-body quantum system into a desirable, coherent non-equilibrium state. A thermodynamically large system will, however, almost always saturate to a featureless infinite temperature state under continuous driving and so the optical manipulation of many-body systems is considered feasible only if a transient, prethermal regime exists, where heating is suppressed. Here we show that, counterintuitively, in a broad class of lattices Floquet heating can actually be an advantageous effect. Specifically, we prove that the maximum entropy steady states which form upon driving the ground state of the Hubbard model on unbalanced bi-partite lattices possess uniform off-diagonal long-range order which remains finite even in the thermodynamic limit. This creation of a `hot' condensate can occur on any driven unbalanced lattice and provides an understanding of how heating can, at the macroscopic level, expose and alter the order in a quantum system. We discuss implications for recent experiments observing emergent superconductivity in photoexcited materials.

DOI
10.22331/q-2021-12-23-610

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Coherent driving has established itself as a powerful tool for guiding a many-body quantum system into a desirable, coherent non-equilibrium state. A thermodynamically large system will, however, almost always saturate to a featureless infinite temperature state under continuous driving and so the optical manipulation of many-body systems is considered feasible only if a transient, prethermal regime exists, where heating is suppressed. Here we show that, counterintuitively, in a broad class of lattices Floquet heating can actually be an advantageous effect. Specifically, we prove that the maximum entropy steady states which form upon driving the ground state of the Hubbard model on unbalanced bi-partite lattices possess uniform off-diagonal long-range order which remains finite even in the thermodynamic limit. This creation of a `hot' condensate can occur on any driven unbalanced lattice and provides an understanding of how heating can, at the macroscopic level, expose and alter the order in a quantum system. We discuss implications for recent experiments observing emergent superconductivity in photoexcited materials.
Periodic driving has emerged as a powerful tool in the quest to engineer new and exotic quantum phases. While driven many-body systems are generically expected to absorb energy indefinitely and reach an infinite-temperature state, the rate of heating can be exponentially suppressed when the drive frequency is large compared to the local energy scales of the system -- leading to long-lived 'prethermal' regimes. In this work, we experimentally study a bosonic cloud of ultracold atoms in a driven optical lattice and identify such a prethermal regime in the Bose-Hubbard model. By measuring the energy absorption of the cloud as the driving frequency is increased, we observe an exponential-in-frequency reduction of the heating rate persisting over more than 2 orders of magnitude. The tunability of the lattice potentials allows us to explore one- and two-dimensional systems in a range of different interacting regimes. Alongside the exponential decrease, the dependence of the heating rate on the frequency displays features characteristic of the phase diagram of the Bose-Hubbard model, whose understanding is additionally supported by numerical simulations in one dimension. Our results show experimental evidence of the phenomenon of Floquet prethermalization, and provide insight into the characterization of heating for driven bosonic systems.
Periodic driving has emerged as a powerful tool in the quest to engineer new and exotic quantum phases.While driven many-body systems are generically expected to absorb energy indefinitely and reach an infinitetemperature state, the rate of heating can be exponentially suppressed when the drive frequency is large compared to the local energy scales of the system-leading to long-lived "prethermal" regimes.In this work, we experimentally study a bosonic cloud of ultracold atoms in a driven optical lattice and identify such a prethermal regime in the Bose-Hubbard model.By measuring the energy absorption of the cloud as the driving frequency is increased, we observe an exponential-in-frequency reduction of the heating rate persisting over more than 2 orders of magnitude.The tunability of the lattice potentials allows us to explore one-and twodimensional systems in a range of different interacting regimes.Alongside the exponential decrease, the dependence of the heating rate on the frequency displays features characteristic of the phase diagram of the Bose-Hubbard model, whose understanding is additionally supported by numerical simulations in one dimension.Our results show experimental evidence of the phenomenon of Floquet prethermalization and provide insight into the characterization of heating for driven bosonic systems.
Under the action of coherent periodic driving a generic quantum system will undergo Floquet heating and continuously absorb energy until it reaches a featureless thermal state. The phase-space constraints induced by certain symmetries can, however, prevent this and allow the system to dynamically form robust steady states with off-diagonal long-range order. In this work, we take the Hubbard model on an arbitrary lattice with arbitrary filling and, by simultaneously diagonalizing the two possible SU(2) symmetries of the system, we analytically construct the correlated steady states for different symmetry classes of driving. This construction allows us to make verifiable, quantitative predictions about the long-range particle-hole and spin-exchange correlations that these states can possess. In the case when both SU(2) symmetries are preserved in the thermodynamic limit we show how the driving can be used to form a unique condensate which simultaneously hosts particle-hole and spin-wave order.
Periodically driven many-body systems generally heat towards a featureless 'infinite-temperature' state. As an alternative to uniform heating in a clean system, here we establish a Floquet superheating regime, where fast heating nucleates at ''hot spots" generated by rare fluctuations in the local energy with respect to an appropriate effective Hamiltonian. Striking macroscopic consequences include exceptionally long-lived prethermalization and non-ergodic bimodal distributions of macroscopic observables. Superheating is predicated on a heating rate depending strongly on the local fluctuation; in our example, this is supplied by a sharp state-selective spin-echo, where the energy absorption is strongly suppressed for low-energy states, while thermal fluctuations open up excessive heating channels. A simple phenomenological theory is developed to show the existence of a critical droplet size, which incorporates heating by the driving field as well as the heat current out of the droplet. Our results shine light on a new heating mechanism and suggest new routes towards stabilizing non-equilibrium phases of matter in driven systems.
The optical manipulation of phonon degrees of freedom can change the effective interactions in solids and potentially enhance superconductivity. However, heating and nonthermal energy distributions need to be considered to understand the ultimate effects of such a driving on ordered states. Using nonequilibrium dynamical mean field theory in the Kadanoff-Baym and Floquet implementation, the authors systematically discuss the effects of parametric phonon driving on conventional superconductivity. Both the transient dynamics of isolated systems and the nonequilibrium steady states in driven-dissipative systems are considered. While the phonon-mediated attractive interaction can be enhanced in certain driving regimes because of Floquet phonon sidebands, the heating and nonthermal distribution effects dominate and generically result in a suppression of superconductivity.
Periodically-driven (Floquet) quantum systems are ubiquitous in science and technology. For example, when a laser illuminates a material or an AC voltage is applied to a device, the system is well-described by a time-periodic Hamiltonian. In recent years, periodic driving has been proposed, not just as a tool to excite and probe devices, but actually as a mechanism of engineering new phases of matter, some of which have no equilibrium analog. However, with this promise comes a serious problem. Intuitively, if energy is injected into and distributed throughout a system, it is no surprise that it tends to heat up indefinitely to infinite temperature. In this thesis, we study the mechanisms of heating, i.e. the process of thermalization, in Floquet systems and propose methods to control them. Specifically, for non-interacting Floquet systems that are coupled to external bosonic and fermionic baths (e.g. laser-driven electrons in a semiconductor that interact with phonons and an external lead), we classify the relevant scattering processes that contribute to cooling/heating in the Floquet bands and suggest methods to suppress heating via bandwidth-restrictions on the baths. We find that is possible, with appropriate dissipative engineering, to stabilize a controlled incompressible nonequilibrium steady-state resembling a ground state - a state we term the "Floquet insulator." We extend this analysis to include short-range interactions that contribute additional heating processes and show, under the same framework, that heating can be controlled with dissipation. In the process, we develop a simple effective model for the Floquet band densities that captures the essence of all the Floquet scattering processes and that is useful for ballparking experimentally-relevant estimates of heating. Next, we turn our attention to strongly-interacting closed Floquet systems and study how heating emerges through a proliferation of resonances. We find a novel integrable point governing the strong-interaction limit of the Floquet system and examine the breakdown of integrability via the proliferation of resonances. We observe two distinct scaling regimes, attributed to non-thermal and thermal behavior, and discover a power-law scaling of the crossover between them as a function of system size. The lingering ergodicity-breaking effects of the conserved quantities in the vicinity (in parameter space) of the integrable point at finite size is a phenomena we term "near-integrability." These results suggest that small quantum systems, which are accessible currently in many platforms (e.g. trapped ions, cold atoms, superconducting devices), intrinsically host non-thermal states that one may be able to utilize to avoid heating. Furthermore, our results suggest a "dual" interpretation, in the thermodynamic limit, that a periodically-driven system exhibits prethermalization as a power-law in interaction strength.