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arXiv:2103.03484 · Journal of Physics Condensed Matter

Why the Schwinger boson mean field theory fails to describe the spin dynamics of the triangular lattice antiferromagnetic Heisenberg model?

Qiu Zhang, Tao Li

Published Jun 28, 2021• 7 citations

Abstract

We find that the Schwinger boson mean field theory (SBMFT) supplemented with Gutzwiller projection provides an exceedingly accurate description for the ground state of the spin-12triangular lattice antiferromagnetic Heisenberg model (spin-12TLHAF). However, we find the SBMFT fails even qualitatively in the description of the dynamical behavior of the system. In particular, the SBMFT fails to predict the Goldstone mode in the magnetic ordered phase. We show that the coherent peak in the two-spinon continuum in the presence of spinon condensate should not be interpreted as a magnon mode. The SBMFT also predicts incorrectly a gapless longitudinal spin fluctuation mode in the magnetic ordered phase. We show that these failures are related to the following facts: (1) spinon condensation fails to provide a consistent description of the order parameter manifold of the 120 degree ordered phase. (2) There lacks in the SBMFT the coupling between the uncondensed spinon and the spinon condensate, which breaks both the spin rotational and the translational symmetry. (3) There lacks in the SBMFT the rigidity that is related to the no double occupancy constraint on the spinon system. We show that such failures of the SBMFT is neither restricted to the spin-12TLHAF nor to the magnetic ordered phase. We proposed a generalized SBMFT to resolve the first two issues and a new formalism to address the third issue.

DOI: 10.1088/1361-648x/ac0f2d

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We find that the Schwinger boson mean field theory (SBMFT) supplemented with Gutzwiller projection provides an exceedingly accurate description for the ground state of the spin-12triangular lattice antiferromagnetic Heisenberg model (spin-12TLHAF). However, we find the SBMFT fails even qualitatively in the description of the dynamical behavior of the system. In particular, the SBMFT fails to predict the Goldstone mode in the magnetic ordered phase. We show that the coherent peak in the two-spinon continuum in the presence of spinon condensate should not be interpreted as a magnon mode. The SBMFT also predicts incorrectly a gapless longitudinal spin fluctuation mode in the magnetic ordered phase. We show that these failures are related to the following facts: (1) spinon condensation fails to provide a consistent description of the order parameter manifold of the 120 degree ordered phase. (2) There lacks in the SBMFT the coupling between the uncondensed spinon and the spinon condensate, which breaks both the spin rotational and the translational symmetry. (3) There lacks in the SBMFT the rigidity that is related to the no double occupancy constraint on the spinon system. We show that such failures of the SBMFT is neither restricted to the spin-12TLHAF nor to the magnetic ordered phase. We proposed a generalized SBMFT to resolve the first two issues and a new formalism to address the third issue.

The Schwinger boson theory provides a natural path for treating quantum spin systems with large quantum fluctuations. In contrast to semiclassical treatments, this theory allows us to describe a continuous transition between magnetically ordered and spin liquid states, as well as the continuous evolution of the corresponding excitation spectrum. The square lattice Heisenberg antiferromagnet is one of the first models that was approached with the Schwinger boson theory. Here we revisit this problem to reveal several subtle points that were omitted in previous treatments and that are crucial to further develop this formalism. These points include the freedom for the choice of the saddle point (Hubbard-Stratonovich decoupling and choice of the condensate) and the

1/N

expansion in the presence of a condensate. A key observation is that the spinon condensate leads to Feynman diagrams that include contributions of different order in

1/N

, which must be accounted for to get a qualitatively correct excitation spectrum. We demonstrate that a proper treatment of these contributions leads to an exact cancellation of the single-spinon poles of the dynamical spin structure factor, as expected for a magnetically ordered state. The only surviving poles are the ones arising from the magnons (two-spinon bound states), which are the true collective modes of an ordered magnet.

We compute the dynamical structure factor of the spin-½ triangular Heisenberg model using the mean-field Schwinger boson theory. We find that a reconstructed dispersion, resulting from a non-trivial redistribution of the spectral weight, agrees quite well with the spin excitation spectrum recently found with series expansions. In particular, we recover the strong renormalization with respect to linear spin wave theory along with the appearance of roton-like minima. Furthermore, near the roton-like minima the contribution of the two spinon continuum to the static structure factor is about 40% of the total weight. By computing the density-density dynamical structure factor, we identify an unphysical weak signal of the spin excitation spectrum with the relaxation of the local constraint of the Schwinger bosons at the mean-field level. Based on the accurate description obtained for the static and dynamic ground-state properties, we argue that the bosonic spinon theory should be considered seriously as a valid alternative to interpret the physics of the triangular Heisenberg model.

We compute the zero temperature dynamical structure factor

S({\bf q},\omega)

of the triangular lattice Heisenberg model using a Schwinger Boson approach that includes the Gaussian fluctuations (

1/N

correction) of the saddle point solution. While the ground state of this model exhibits a well-known 120

^{\circ}

magnetic ordering, the excitation spectrum revealed by

S({\bf q},\omega)

has a strong quantum character that is not captured by low-order

1/S

expansions. The low-energy magnons consist of two spinon bound states confined by gauge fluctuations of the auxiliary fields, which can produce internal structure of the magnon peaks. In addition, the high-energy continuum of spinon modes extends up to about three times the single-magnon bandwidth.

A non-abelian spin liquid in triangular lattice spin-1 systems was recently formulated in the form of continuum field theory [T. Grover, and T. Senthil, Phys. Rev. Lett. 107, 077203 (2011); Cenke Xu, A.W.W. Ludwig, arXiv:1012.5671]. It has spin-1/2 bosonic spinons coupled to emergent quaternion gauge fields, and can be obtained by quantum disordering a non-collinear spin nematic order hypothesized to describe NiGa_2S_4 [H. Tsunetsugu, and M. Arikawa, J. Phys. Soc. Jpn. 75, 083701 (2006)], However a microscopic lattice description, e.g. the lattice spinon (mean-field) Hamiltonian and the spin wavefunction, has been missing, and it has been noted that the standard Schwinger boson or bosonic triplon representations of spin-1 cannot describe this spin liquid. In this paper a two-orbital Schwinger boson representation for spin-1 systems is developed and used to construct a mean-field description of this quaternion spin liquid. Projecting the mean-field state produces a prototype wavefunction, which is a superposition of close-packed AKLT loop configurations with nontrivial amplitudes. This new formalism and related wavefunctions may be generalized to higher spin systems and can possibly produce spin liquid states with even richer emergent gauge structures.

We present three different methods of finding the critical spin value

1/N

of the quantum phase transition between the spin liquid and the Néel order phase on the mean field triangular Heisenberg antiferromagnet at

T=0

K. These methods are: using the sublattice magnetization as an order parameter, looking at the scaling of the energy difference of topologically degenerate states in different phases, and the quantum fidelity approach. All of these methods are able to pick up the signal of the phase transition, and their estimated numerical values of

S_c

agree for systems where the relative strength of next nearest neighbour interaction compared to the nearest neighbour interaction is small. For the relative interaction strength

j=0

and

j=0.1

, all three methods predict

S_c\\approx0.21

and

S_c\\approx0.25

respectively, while

j=0.2

gives deviating results. This deviation might be caused by the influence of other magnetically ordered states that we have not accounted for in our calculations, and so we restrict the validity of our results to

j<0.125

.