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arXiv:2103.01138 · Communications Physics

Continuous quantum light from a dark atom

Karl Nicolas Tolazzi, Bo Wang, Christopher Ianzano, Jonas Neumeier, Celso Jorge Villas-Boas, Gerhard Rempe

Published Mar 23, 2021• 8 citations
arXivHTMLPDF

Abstract

Abstract Cycling processes are important in many areas of physics ranging from lasers to topological insulators, often offering surprising insights into dynamical and structural aspects of the respective system. Here we report on a quantum-nonlinear wave-mixing experiment where resonant lasers and an optical cavity define a closed cycle between several ground and excited states of a single atom. We show that, for strong atom–cavity coupling and steady-state driving, the entanglement between the atomic states and intracavity photon number suppresses the excited-state population via quantum interference, effectively reducing the cycle to the atomic ground states. The system dynamics then result from transitions within a harmonic ladder of entangled dark states, one for each cavity photon number, and a quantum Zeno blockade that generates antibunching in the photons emitted from the cavity. The reduced cycle suppresses unwanted optical pumping into atomic states outside the cycle, thereby enhancing the number of emitted photons.

DOI
10.1038/s42005-021-00559-7

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Abstract Cycling processes are important in many areas of physics ranging from lasers to topological insulators, often offering surprising insights into dynamical and structural aspects of the respective system. Here we report on a quantum-nonlinear wave-mixing experiment where resonant lasers and an optical cavity define a closed cycle between several ground and excited states of a single atom. We show that, for strong atom–cavity coupling and steady-state driving, the entanglement between the atomic states and intracavity photon number suppresses the excited-state population via quantum interference, effectively reducing the cycle to the atomic ground states. The system dynamics then result from transitions within a harmonic ladder of entangled dark states, one for each cavity photon number, and a quantum Zeno blockade that generates antibunching in the photons emitted from the cavity. The reduced cycle suppresses unwanted optical pumping into atomic states outside the cycle, thereby enhancing the number of emitted photons.
We show an optical wave-mixing scheme that generates quantum light by means of a single three-level atom. The atom couples to an optical cavity and two laser fields that together drive a cycling current within the atom. Weak driving in combination with strong atom-cavity coupling induces transitions in a harmonic ladder of dark states, accompanied by single-photon emission via a quantum Zeno effect and suppression of atomic excitation via quantum interference. For strong driving, the system can generate coherent or Schrödinger cat-like fields with frequencies distinct from those of the applied lasers.
Photon blockade is a dynamical quantum-nonlinear effect in driven systems with an anharmonic energy ladder. For a single atom strongly coupled to an optical cavity, we show that atom driving gives a decisively larger optical nonlinearity than cavity driving. This enhances single-photon blockade and allows for the implementation of two-photon blockade where the absorption of two photons suppresses the absorption of further photons. As a signature, we report on three-photon antibunching with simultaneous two-photon bunching observed in the light emitted from the cavity. Our experiment constitutes a significant step towards multiphoton quantum-nonlinear optics.
We theoretically study the quantum-interference-induced photon blockade and antiblockade phenomenon in an atom-cavity QED system, where the destructive [constructive] interference between two different transition pathways prohibits [enhances] two-photon excitation. To begin with, we study a single-atom--cavity QED system where the atom or cavity is driven by a coherent pump field. We show that the cavity-driven case will lead to the quantum-interference-induced photon blockade under a specific condition, but such an interference-induced photon blockade cannot be realized in the atom-driven case. This is an important consequence of the pathways possible for the two types of drives. Then, we investigate the two-atom case, and find that an additional transition pathway appears in the atom-driven case. We show that this additional transition pathway results in the quantum-interference-induced photon blockade only when the atomic resonant frequency is different from the cavity mode frequency otherwise antiblockade occurs. Moreover, in this case, the condition for realizing the interference-induced photon blockade is independent of the system's intrinsic parameters, which can be used to generate antibunched photons in both weak and strong coupling regimes.
We study the dynamics of a system composed of two coupled cavities, each interacting with a single Rydberg atom. The interplay between Rydberg-Rydberg interaction and photon hopping enables the transition of the atoms from the collective ground state to the double Rydberg excitation state by individually interacting with the optical normal modes and suppressing the upconversion process between them. The atomic transition is accompanied by the two-photon absorption and emission of the normal modes. Since the energy level structure of the atom-cavity system is photon number dependent there is only a pair of states being in the two-photon resonance. Therefore, the system can act as a quantum nonlinear absorption filter through the nonclassical quantum process, converting coherent light field into a nonclassical state. Meanwhile, the vacuum field in the cavity inspires the Rydberg atoms to simultaneously emit two photons into the normal mode, resulting in obvious emission enhancement of the mode.
Photon antibunching based on a single two-level atom strongly coupled to a single-mode optical cavity has been demonstrated in experiments. Here, we put forward an improved version of such an antibunching by introducing a pump field and a microwave field in the coupled atom-cavity system to form both a three-level $\mathrm{\ensuremath{\Delta}}$-type transition and closed-loop coupling. Via calculating the zero-time-delay second-order correlation function g(2)(0){g}^{(2)}(0)g(2)(0) of the single-mode cavity field, we find that a complete photon blockade, namely, g(2)(0)=0{g}^{(2)}(0)=0g(2)(0)=0, can be well achieved without detuning the driving and cavity resonance. In addition, it is clearly shown that this strong photon antibunching effect appears in the weak-coupling regime of light-atom interactions. The enhanced photon antibunching is ascribed to quantum interference between the two transition paths from the three-level $\mathrm{\ensuremath{\Delta}}$ atom weakly coupled to the three involved fields (cavity, pump, and microwave). Our proposal is useful for the single-photon generation by photon blockade, which has applications in quantum information processing.
Although conventional lasers operate with a large number of intracavity atoms, the lasing properties of a single atom in a resonant cavity have been theoretically investigated for more than a decade. Here we report the experimental realization of such a one-atom laser operated in a regime of strong coupling. Our experiment exploits recent advances in cavity quantum electrodynamics that allow one atom to be isolated in an optical cavity in a regime for which one photon is sufficient to saturate the atomic transition. In this regime the observed characteristics of the atom-cavity system are qualitatively different from those of the familiar many atom case. Specifically, we present measurements of intracavity photon number versus pump intensity that exhibit "thresholdless" behavior, and infer that the output flux from the cavity mode exceeds that from atomic fluorescence by more than tenfold. Observations of the second-order intensity correlation function demonstrate that our one-atom laser generates manifestly nonclassical light that exhibits both photon antibunching and sub-Poissonian photon statistics.