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arXiv:2102.11862 · PRX Quantum

Site-Resolved Imaging of Ultracold Fermions in a Triangular-Lattice Quantum Gas Microscope

Jin Yang, Liyu Liu, Jirayu Mongkolkiattichai, Peter Schauß

Published Jun 21, 2021• 76 citations
arXivHTMLPDF

Abstract

Quantum gas microscopes have expanded the capabilities of quantum simulation of Hubbard models by enabling the study of spatial spin and density correlations in square lattices.However, quantum gas microscopes have not been realized for fermionic atoms in frustrated geometries.Here, we demonstrate the single-atom resolved imaging of ultracold fermionic 6 Li atoms in a triangular optical lattice with a lattice constant of 1003 nm.The optical lattice is formed by a recycled narrow-linewidth, high-power laser combined with a light sheet to allow for Raman sideband cooling on the D 1 line.We optically resolve single atoms on individual lattice sites using a high-resolution objective to collect scattered photons while cooling them close to the two-dimensional ground vibrational level in each lattice site.By reconstructing the lattice occupation, we measure an imaging fidelity of approximately 98%.Our triangular lattice microscope platform for fermions clears the path for studying spin-spin correlations, entanglement, and dynamics of geometrically frustrated Hubbard systems which are expected to exhibit exotic emergent phenomena including spin liquids and kinetic frustration.

DOI
10.1103/prxquantum.2.020344

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Quantum gas microscopes have expanded the capabilities of quantum simulation of Hubbard models by enabling the study of spatial spin and density correlations in square lattices.However, quantum gas microscopes have not been realized for fermionic atoms in frustrated geometries.Here, we demonstrate the single-atom resolved imaging of ultracold fermionic 6 Li atoms in a triangular optical lattice with a lattice constant of 1003 nm.The optical lattice is formed by a recycled narrow-linewidth, high-power laser combined with a light sheet to allow for Raman sideband cooling on the D 1 line.We optically resolve single atoms on individual lattice sites using a high-resolution objective to collect scattered photons while cooling them close to the two-dimensional ground vibrational level in each lattice site.By reconstructing the lattice occupation, we measure an imaging fidelity of approximately 98%.Our triangular lattice microscope platform for fermions clears the path for studying spin-spin correlations, entanglement, and dynamics of geometrically frustrated Hubbard systems which are expected to exhibit exotic emergent phenomena including spin liquids and kinetic frustration.
We realize a quantum-gas microscope for fermionic ^{40}K atoms trapped in an optical lattice, which allows one to probe strongly correlated fermions at the single-atom level. We combine 3D Raman sideband cooling with high-resolution optics to simultaneously cool and image individual atoms with single-lattice-site resolution at a detection fidelity above 95%. The imaging process leaves the atoms predominantly in the 3D motional ground state of their respective lattice sites, inviting the implementation of a Maxwell's demon to assemble low-entropy many-body states. Single-site-resolved imaging of fermions enables the direct observation of magnetic order, time-resolved measurements of the spread of particle correlations, and the detection of many-fermion entanglement.
Strongly-correlated electron systems generate some of the richest phenomena and most challenging theoretical problems studied in physics. One approach to understanding these systems is with ultracold fermionic atoms in optical lattices, which can provide a level of control and ways of observing strongly-correlated fermionic systems that are not accessible with conventional materials. This thesis describes the development of an experimental technique where a quantum gas of fermionic 6Li atoms is prepared in a two-dimensional optical lattice and each atom can be frozen in place and imaged with single-site resolution. Combining a vacuum-compatible large numerical aperture microscope with Raman sideband cooling enables site-resolved fluorescence imaging with high fidelity. We observe several phases of the Hubbard model, including band and Mott insulators. The observed in-situ occupation distributions of atoms in the lattice are compared to theory with unprecedented detail and are used to determine the thermodynamic properties of the system. By combining site-resolved imaging with a spin-removal technique, we observe antiferromagnetic correlations in the Hubbard model with single-site resolution. We observe, for the first time in cold atom systems, beyond-nearest-neighbor magnetic correlations, which provide a direct measurement of the correlation length. We also present detailed measurements of the formation of correlations during lattice loading.
Abstract We demonstrate single-site-resolved fluorescence imaging of ultracold 87Rb atoms in a triangular optical lattice by employing Raman sideband cooling. Combining a Raman transition at the D1 line and a photon scattering through an optical pumping of the D2 line, we obtain images with low background noise. The Bayesian optimisation of 11 experimental parameters for fluorescence imaging with Raman sideband cooling enables us to achieve single-atom detection with a high fidelity of (96.3 ± 1.3)%. Single-atom and single-site resolved detection in a triangular optical lattice paves the way for the direct observation of spin correlations or entanglement in geometrically frustrated systems.
This thesis describes the methods used to achieve single-atom and single-site resolved fluorescence imaging of a quantum gas of fermionic atoms held in an optical lattice. This kind of quantum gas microscopy has been previously applied to bosonic atoms in two experiments, and has allowed for extensive studies of many-body quantum systems. Here we detail methods to extend the techniques of quantum gas microscopy to fermionic species of atoms, opening the door to quantum simulation of electronic models of condensed matter physics. We prepare quantum degenerate gases of fermionic 40K through sympathetic cooling with a gas of \Rb. The gas prepared is trapped less than 1 mm away from a thin vacuum window, an experimental geometry which permits interrogation with a large Numerical Aperture microscope objective. The cloud is loaded into a 527 nm-period cubic optical lattice, ideal for quantum simulation of many-body models of fermionic particles such as the Hubbard model. The optical lattice is designed to allow for potential depths up to V/kB = 250 microKelvin, sufficient to strongly confine 40K atoms into individual lattice sites. EIT cooling --- a technique previously demonstrated in ion-trapping experiments --- is used to cool the fermionic atoms deeply towards the ground motional state of the lattice wells. We collect the photons scattered during continuous application of EIT cooling, while atoms are kept pinned in the lattice for many seconds. We strongly suppress all other sources of light with the use of a modulated cooling scheme and a spinning chopper wheel. Collecting the scattered light produced during 2 s of EIT cooling allows us to resolve single atoms in a fluorescence image. We demonstrate that the high resolution of our imaging apparatus also permits atom positions to be precisely identified on the length scale of the optical lattice. Thus we demonstrate the realisation of a quantum gas microscope for fermionic atoms, allowing for precise investigation of the ground states and dynamics of correlated quantum states of fermionic particles.
We demonstrate site-resolved imaging of individual fermionic ^{6}Li atoms in a single layer of a 3D optical lattice. To preserve the density distribution during fluorescence imaging, we simultaneously cool the atoms with 3D Raman sideband cooling. This laser cooling technique, demonstrated here for the first time for ^{6}Li atoms, also provides a pathway to rapid low-entropy filling of an optical lattice. We are able to determine the occupation of individual lattice sites with a fidelity >95%, enabling direct, local measurement of particle correlations in Fermi lattice systems. This ability will be instrumental for creating and investigating low-temperature phases of the Fermi-Hubbard model, including antiferromagnets and d-wave superfluidity.
Geometrically frustrated many-particle quantum systems are notoriously hard to study numerically but are of profound interest because of their unusual properties and emergent phenomena. In these systems energetic constraints cannot be minimized simultaneously, leading to large ground-state degeneracy and a variety of exotic quantum phases. Here, we present a platform that enables unprecedentedly detailed experimental exploration of geometrically frustrated electronic systems on lattices with triangular geometry. We demonstrate the first realization of triangular atomic Hubbard systems, directly image Mott insulators in the triangular geometry with single-atom and single-site resolution, and measure antiferromagnetic spin-spin correlations for all nearest neighbors allowing for thermometry. This platform provides a powerful new approach for studying exotic quantum magnetism and direct detection of quantum spin liquid signatures in Hubbard systems.