Abstract The quantum world distinguishes itself from the classical world by being governed by probability amplitudes rather than probabilities. On a single-particle level, quantum phases can be manipulated leading to observable interference patterns that can be used as a probe e.g. in matter wave microscopy. But the quantum world bears even more fascinating effects when it comes to the interplay between more than one particle. Correlations between quantum particles such as entanglement can be exploited to speed up computational algorithms or enable secure cryptography. Here, we propose and numerically explore a thought experiment to address the question whether quantum correlations between particles can be used in matter wave microscopy. Specifically, we address the following questions: can information be transferred between two mutually spin-correlated free-electron wavepackets? Can Coulomb and exchange correlations be linked to the decoherence and dephasing mechanisms of matter waves? Using a time-dependent Hartree–Fock algorithm, we will show that the exchange term has a substantial role in transferring the information between two mutually spin-correlated electrons, whereas the Hartree potential (or mean-field Coulomb potential) dominates the dephasing on a single-particle level. Our findings might facilitate fermionic matter wave interferometry experiments designed to retrieve information about non-classical correlations and the mechanism of decoherence in open quantum systems.
Abstract The quantum world distinguishes itself from the classical world by being governed by probability amplitudes rather than probabilities. On a single-particle level, quantum phases can be manipulated leading to observable interference patterns that can be used as a probe e.g. in matter wave microscopy. But the quantum world bears even more fascinating effects when it comes to the interplay between more than one particle. Correlations between quantum particles such as entanglement can be exploited to speed up computational algorithms or enable secure cryptography. Here, we propose and numerically explore a thought experiment to address the question whether quantum correlations between particles can be used in matter wave microscopy. Specifically, we address the following questions: can information be transferred between two mutually spin-correlated free-electron wavepackets? Can Coulomb and exchange correlations be linked to the decoherence and dephasing mechanisms of matter waves? Using a time-dependent Hartree–Fock algorithm, we will show that the exchange term has a substantial role in transferring the information between two mutually spin-correlated electrons, whereas the Hartree potential (or mean-field Coulomb potential) dominates the dephasing on a single-particle level. Our findings might facilitate fermionic matter wave interferometry experiments designed to retrieve information about non-classical correlations and the mechanism of decoherence in open quantum systems.
Abstract In quantum mechanics, each particle is described by a complex valued wave-function characterized by amplitude and phase. When many particles interact each other, cooperative phenomena give rise to a quantum many-body state with a specific quantum coherence. What is the interplay between single-particle’s phase coherence and many-body quantum coherence? Over the years, such question has been object of profound analysis in quantum physics. Here, we demonstrate how the time-dependent interference formed by releasing an interacting degenerate Fermi gas from a specific matter-wave circuit in an effective magnetic field can tell apart the two notions. Single-particle phase coherence, indicated by the first-order correlator, and many-body quantum coherence, indicated by the density–density correlator, are displayed as distinct features of the interferogram. Single particle phase coherence produces spiral interference of the Fermi orbitals at intermediate times. Many-body quantum coherence emerges as long times interference. The interplay between single-particle coherence and many-body coherence is reflected in a stepwise dependence of the interference pattern on the effective magnetic field.
We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and for neutral particles with permanent dipole moments. Interference is studied when electrons or atomic systems are coupled to classical or quantum electromagnetic fields. The interaction between the particles and time-dependent fields induces a time-varying Aharonov phase. Averaging over the phase generates a suppression of fringe visibility in the interference pattern. We show that, for suitable experimental conditions, the loss of contrast for dipoles can be almost as large as the corresponding one for coherent electrons and therefore can be observed. We analyse different trajectories in order to show the dependence of the decoherence factor on the velocity of the particles.
Electron beams are a formidable tool for probing nanophotonic systems [1]. Combining electron microscopy with external optical excitation in ultrafast transmission electron microscopes has enabled the mapping of optical near-fields [2] and the bunching of electrons in attosecond pulses [3, 4]. These developments are based on the stimulated inelastic scattering between electrons and light [5, 6], in which the electrons gain energy from or lose energy to the optical field. Recently, the underlying interaction strength of this process has been increased significantly by harnessing resonant enhancement of the optical field and velocity phase matching [7]. Such an increased interaction strength also benefits the spontaneous scattering of electrons with light, thus promising applications like generating complex quantum states of light [8]. In this presentation, we discuss a set of experiments on free electron quantum optics that investigate single-electron-single-photon interactions and probe the resulting entanglement. Specifically, we consider scenarios in which optical waveguide structures are placed inside a transmission electron microscope (TEM) facilitating the interaction. Electrons passing by, for example, an integrated photonic structure (cf. Fig. 1a) can inelastically scatter with the optical mode, leading to the emergence of electron-photon pair states [9]. The resulting correlation between energy-loss electrons and photons, illustrated in Fig. 1b, can be probed employing time- and energy-resolved detection of both particles, revealing a pronounced coincidence peak between their arrival times, schematically shown in Fig. 1c. Extending the photon detection setup by a second detector to allow for Hanbury Brown and Twiss (HBT) measurements, the photon statistics heralded by such energy-loss electrons can be studied [10]. The observed anti-bunching behavior indicates a nonclassical optical state with single-photon properties. The inelastic electron-light scattering underlying the electron-photon pair generation is further expected to induce entanglement in the particle energies [11], however, direct observation of quantum entanglement would be exceedingly difficult given the large number of independent quantum states available in these degrees of freedom. Therefore, we propose experiments based on the quantum eraser scheme to demonstrate this free-electron-photon entanglement in different degrees of freedom [12,13]. Specifically, we consider a double-slit geometry coherently illuminated by an electron beam such that an interference pattern can be observed on a distant screen (cf. Fig. 2a). If electrons passing through the left or right (denoted |Land |R, respectively) slit generate distinct marker photons with vertical (|V)or horizontal (|H) polarization, this interference pattern would disappear due to the entanglement of electron path and photon polarisation (cf. Fig. 2b). However, if this which-path information carried by the marker photon is erased, e.g. by mixing the polarisation states, the interference pattern can be recovered when detecting electrons and photons in coincidence. We describe an extension of this idea to an entanglement test, before discussing possible realistic implementations and presenting preliminary results on several experimental key aspects. In summary, we discuss the inelastic electron-light scattering at integrated photonic structures with applications ranging from coherent electron beam modulation using continuous-wave optical fields to the electron-driven generation of quantum optical states of light. Delving deeper into single electron-single photon interactions, we outline feasible experiments to generate and verify electron-photon entanglement with a potential extension to electron pairs based on entanglement swapping. All this adds to the toolbox of free electron quantum optics, potentially enabling novel sources of quantum light as well as quantum-enhanced sensing in electron microscopy. Generation of correlated electron-photon pairs. (a) Electrons pass over a photonic integrated circuit placed in the sample plane of a TEM, generating photons in the optical waveguides via inelastic scattering. Energy-loss electrons are detected and time-tagged behind an imaging spectrometer in coincidence with photons exiting the waveguide. (b) Inelastic scattering links the electron energy loss (green, right ladder) to the generation of photons (red, left ladder), creating correlations in energy and time. (c) A strong temporal correlation between the loss electrons and detected photons, indicated by the red dot, is observed relative to the uncorrelated zero-loss background electrons (blue line). Free-electron-photon quantum eraser. (a) Coherent electron illumination of a double-slit structure results in interference between the two pathways |Land |R.(b) If the electrons generate distinguishable marker photons, e.g. of orthogonal polarizations |Vand |H, no interference pattern can be observed due to the electron-photon entanglement. (c) Collecting these marker photons and erasing the which-path information, e.g. using a half-wave plate (λ/2), the electron interference can be recovered using electron-photon coincidence detection with single-photon detectors (SPDs) placed behind a polarizing beam splitter (PBS).
Quantum theory is often cited as being one of the most empirically validated theories in terms of its predictive power and precision. These attributes have led to numerous scientific discoveries and technological advancements. However, the precise relationship between quantum and classical physics remains obscure. The prevailing description is known as decoherence theory, where classical physics emerges from a more general quantum theory through environmental interaction. Sometimes referred to as the decoherence program, it does not solve the quantum measurement problem. We believe experiments performed between the microscopic and macroscopic world may help finish the program. The following considers a free electron that interacts with a surface (the environment), providing a controlled decoherence mechanism. There are non-decohering interactions to be examined and quantified before the weaker decohering effects are filtered out. In the first experiment, an electron beam passes over a surface that’s illuminated by low-power laser light. This induces a surface charge redistribution causing the electron deflection. This phenomenon’s parameters are investigated. This system can be well understood in terms of classical electrodynamics, A second experiment tests decoherence theory by introducing a nanofabricated diffraction grating before the surface. The electron undergoes diffraction through the grating, but as the electron passes over the surface it’s predicted by various physical models that the electron will lose its wave interference property. Image charge based models, which predict a larger loss of contrast than what is observed, are falsified (despite experiencing an image charge force). A theoretical study demonstrates how a loss of contrast may not be due to the irreversible process decoherence, but dephasing (a reversible process due to randomization of the wavefunction’s phase). To resolve this ambiguity, a correlation function on an ensemble of diffraction patterns is analyzed after an electron undergoes either process in a path integral calculation. The diffraction pattern is successfully recovered for dephasing, but not for decoherence, thus verifying it as a potential tool in experimental studies to determine the nature of the observed process.
Matter-wave interferometry is a phenomenon which has been utilized and studied in electron microscopy since the early days of electron optics, with the development of phase contrast imaging, electron diffraction, electron holography, etc. When an electron diffracts off of a crystal lattice, it enters a superposition state of eligible Bragg diffraction components; due to momentum conservation, the crystalline sample must receive an equal and opposite superposition of momentum transfers. In theory, this results in an entangled electron-sample state. Typically, however, the sample is extremely large relative to the electron and is held fast in a sample holder, and this reciprocal momentum transfer is unobservable [1]. We present a proposal [2] to establish a system where such momentum kicks would be resolvable, to enable probing of the matter-wave properties of the sample as well as the free electron. A crystalline silicon nanoparticle is levitated in the sample plane, then released from its trap to enter free-fall. A single electron impacts the nanoparticle and undergoes Bragg diffraction. The nanoparticle receives a momentum transfer from the diffraction and is allowed to continue free-falling for a fixed amount of time before recapture and measurement of its position, X. In synchrony, the position of the electron, x, is measured. Assuming perfect measurement resolution, we calculate the resulting interference pattern for a quantum interaction, where the nanoparticle can behave as a quantum wave (Fig. 1a), or for the case where it behaves as a classical grating aperture (Fig. 1b) for different recapture times, t. The quantum scenario presents additional fringes visible at specific recapture times. Such an experiment provides a test of the matter-wave behaviour of high mass nanoparticles, with an efficient duty cycle and a short interference time, and would allow access to electron-sample entanglement in a transmission electron microscope.
In quantum mechanics, each particle is described by a complex valued wave function characterized by amplitude and phase. When many particles interact each other, cooperative phenomena give rise to a quantum many-body state with a specific quantum coherence. What is the interplay between particle's phase coherence and many-body quantum coherence? Over the years, such question has been object of profound analysis in quantum physics. Here, we demonstrate how state of the art quantum technology allows to explore the question operatively. To this end, we study the time-dependent interference formed by releasing an interacting degenerate Fermi-gas from a specific matter-wave circuit in an effective magnetic field. Particle phase coherence, indicated by the first-order correlator, and many-body quantum coherence, indicated by the noise correlator, are displayed as distinct features of the interferogram. Particle phase coherence produces spiral interference of the Fermi orbitals at intermediate times. Many-body quantum coherence emerges at long times. The coupling between particles coherence and many-body coherence is reflected in a specific dependence of the interference pattern on the effective magnetic field.