Collective decays of multiply excited atoms become subradiant and bound in space when they are strongly coupled to the guided modes in an atom-waveguide interface. In this interface, we analyze their average density-density and modified third-order correlations via Kubo cumulant expansions, which can arise, and finite correlations can be sustained for long time. The shape-preserving dimers and trimers of atomic excitations emerge in the most subradiant coupling regime of light-induced dipole-dipole interactions. This leads to a potential application of quantum information processing and quantum storage in the encoded nonreciprocal spin diffusion, where its diffusion speed depends on the initial coherence between the excited atoms and is robust to their relative phase fluctuations. The state-dependent photon routing can be viable as well in this interface.
Collective decays of multiply excited atoms become subradiant and bound in space when they are strongly coupled to the guided modes in an atom-waveguide interface. In this interface, we analyze their average density-density and modified third-order correlations via Kubo cumulant expansions, which can arise, and finite correlations can be sustained for long time. The shape-preserving dimers and trimers of atomic excitations emerge in the most subradiant coupling regime of light-induced dipole-dipole interactions. This leads to a potential application of quantum information processing and quantum storage in the encoded nonreciprocal spin diffusion, where its diffusion speed depends on the initial coherence between the excited atoms and is robust to their relative phase fluctuations. The state-dependent photon routing can be viable as well in this interface.
We investigate theoretically the subradiance dynamics in a nonreciprocal chirally coupled atomic chain, in which infinite-range dipole-dipole interaction emerges in the dissipation. We find that super- and subradiance are both present in the dissipation process following single-photon excitation, and the decay dynamics shows burst emissions from uniform initial excitations, which reflects the influence of atomic ordering on the propagation of light-induced atom-atom correlations. By tuning the nonreciprocal couplings in the chirally coupled atomic system, we show that the subradiance dynamics can be greatly modified. We further study the effect of atomic local disorder and find the occurrence of plateaus on the decay curve dependent on the defect locations, as well as persistent localized excitations induced by disorder. We also discuss the effect of imperfections of systems on the subradiance dynamics. Our results show rich opportunities in the chirally coupled system toward photon storage and routing.
The atom-waveguide interface mediates significant and long-range light-matter interactions through guided modes. In this one-dimensional system, we theoretically investigate the excitation localization of multiple atomic excitations under strong position disorder. Deep in the localization side, we obtain the time evolutions of quantum correlations via Kubo cumulant expansions, which arise initially and become finite and leveled afterward, overtaking those without disorder. This indicates two distinct regimes in time: before the onset of excitation localization, the disorder engage the disturbance of quantum correlations, which is followed by disorder-assisted buildup of quantum correlations that maintain at a later stage owing to the absence of excitations diffusion. The crossing of distinct regimes is pushed further in time for longer-range correlations, which indicates a characteristic timescale needed for disorder to sustain them. We also explore the effect of directionality of couplings and resonant dipole-dipole interactions, which can drive the system toward the delocalized side when it is under chiral couplings or large dipole-dipole interaction strengths. The time-evolved quantum correlations can give insights into the studies of few-body localization phenomenon and nonequilibrium dynamics in open quantum systems.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
An atomic array coupled to a one-dimensional nanophotonic waveguide allows photon-mediated dipole-dipole interactions and nonreciprocal decay channels. Such an array possesses many intriguing quantum phenomena due to its distinctive and emergent quantum correlations. In this atom-waveguide quantum system, we theoretically investigate the atomic excitation dynamics and its transport property, specifically at an interface of dissimilar atomic arrays with different interparticle distances. We find that the atomic excitation dynamics is highly dependent on the interparticle distances of dissimilar arrays and the directionality of nonreciprocal couplings. By tuning these parameters, a dominant excitation reflection can be achieved at the interface of the arrays in the single excitation case. We further study two effects on the transport property—of external drive and of single excitation delocalization over multiple atoms—where we manifest a rich interplay between multisite excitation and the relative phase in determining the transport properties. Finally, we present an intriguing trapping effect of atomic excitation by designing multiple zones of dissimilar arrays. Similar to the single excitations, multiple excitations are reflected from the array interfaces and trapped as well, although complete trapping of many excitations together is relatively challenging at long time due to a faster combined decay rate. Our results can provide insights into nonequilibrium quantum dynamics in dissimilar arrays, and they can shed light on confining and controlling quantum registers useful for quantum information processing. Published by the American Physical Society 2024
The collective interaction of electronic excitations with the electromagnetic field in atomic arrays can lead to reduced decay rates, forming subradiant states with applications in quantum information and memories. By including quantized vibrational excitations, we examine the effects of finite trap strength and light-mediated forces on highly subradiant singly excited states for two, three, and many atoms in a one-dimensional waveguide or free space. For waveguide-coupled and tightly trapped atoms, the recoil energy from photon emission can reach a vibrational quantum, even in the Lamb-Dicke regime. For weakly trapped atoms, the vibrational wave packets are shifted or distorted due to induced forces and uneven decay. These effects lead to a time-dependent decay rate, extra vibrational energy transfer, and mixing of different electronic and vibrational states. The resulting entanglement entropy and infidelity can be mitigated by decreasing the induced forces or increasing trap strength. For quantum information storage, these findings suggest optimal array configurations in geometry and polarization. Our results provide insights for quantum memories and atom array experiments.
Collective excitations in ordered subwavelength atomic arrays can exhibit strongly suppressed radiative decay due to interference between light scattered by neighboring emitters. These so-called subradiant states make these systems a promising platform for storing and manipulating photonic excitations. The external geometry of the array, combined with dynamical control of the atomic dipole orientation, enables localized trapping and coherent transport of these subradiant excitations. Here, we theoretically demonstrate these capabilities in ring-shaped atomic arrays. Specifically, we show adiabatic transport of a localized excitation around a single ring, coherent transfer of a single excitation between two neighboring rings with geometry-controlled selectivity, and interaction-induced conditional phase shifts between two simultaneously trapped excitations in neighboring rings. The latter can be interpreted as effective controlled-phase operations between stored excitations. Together, these results demonstrate the potential of ordered atomic arrays as a platform for coherent photonic quantum information processing with dissipation-protected collective excitations.