Quantum dynamics is of fundamental interest and has implications in quantum information processing. The four-point out-of-time-ordered correlator (OTOC) is traditionally used to quantify quantum information scrambling under many-body dynamics. Due to the OTOC's unusual time ordering, its measurement is challenging. We propose higher-point OTOCs to reveal early-time scrambling behavior, and present protocols to measure any higher-point OTOC using the shadow estimation method. The protocols circumvent the need for time-reversal evolution and ancillary control. They can be implemented in near-term quantum devices with single-qubit readout.
Quantum dynamics is of fundamental interest and has implications in quantum information processing. The four-point out-of-time-ordered correlator (OTOC) is traditionally used to quantify quantum information scrambling under many-body dynamics. Due to the OTOC's unusual time ordering, its measurement is challenging. We propose higher-point OTOCs to reveal early-time scrambling behavior, and present protocols to measure any higher-point OTOC using the shadow estimation method. The protocols circumvent the need for time-reversal evolution and ancillary control. They can be implemented in near-term quantum devices with single-qubit readout.
Out-of-time-order correlator (OTOC), been suggested as a measure of quantum information scrambling in quantum many-body systems, has received enormous attention recently. The experimental measurement of OTOC is quite challenging. The existing theoretical protocols consist in implementing time-reversal operations or using ancillary quantum systems, therefore only a few experiments have been reported. Recently, a new protocol to detect OTOC using statistical correlations between randomized measurements was put forward. In this work, we detect the OTOCs of a kicked-Ising model using this new measurement method on a 4-qubit nuclear magnetic resonance quantum simulator. In experiment, we use random Hamiltonian evolutions to generate the random operations that are required by the randomized OTOC detection protocol. Our experimental results are in good agreement with the theoretical predictions, thus confirming the feasibility of the protocols. Therefore, our work represents a step in exploring realistic quantum chaotic dynamics in complicated quantum systems.
The out-of-time-ordered correlator (OTOC) is a powerful tool for probing quantum information scrambling, a fundamental process by which local information spreads irreversibly throughout a quantum many-body system. Experimentally measuring the OTOC, however, is notoriously challenging due to the need for time-reversed evolution. Here, we present an experimental evaluation of the OTOC on a quantum computer, using three distinct protocols to address this challenge: the rewinding time method (RTM), the weak-measurement method (WMM), and the irreversibility-susceptibility method (ISM). Our experiments investigate the quantum dynamics of an XXZ spin-1/2 chain prepared in a thermal Gibbs state. As a key contribution, we provide the first experimental demonstration of the ISM, using the trapped-ion quantum computer, reimei. We also conduct a detailed comparative analysis of all three methods, revealing method-dependent behaviors in the measured OTOC. This work not only validates these protocols as practical tools for exploring quantum chaos on near-term hardware but also offers crucial insights into their respective advantages and limitations, providing a practical framework for future experimental investigations.
Out-of-time-ordered correlation functions (OTOCs) play a crucial role in the study of thermalization, entanglement, and quantum chaos, as they quantify the scrambling of quantum information due to complex interactions. As a consequence of their out-of-time-ordered nature, OTOCs are difficult to measure experimentally. Here we propose an OTOC measurement protocol that does not rely on the reversal of time evolution and is easy to implement in a range of experimental settings. The protocol accounts for both pure and mixed initial states, and is applicable to systems that interact with environmental degrees of freedom. We demonstrate the application of our protocol by the characterization of scrambling in a periodically driven spin that exhibits quantum chaos.
Out-of-time-order correlators (OTOCs) are central probes of quantum scrambling, and their generalizations have recently become key primitives for both benchmarking quantum advantage and learning the structure of Hamiltonians. Yet their behavior has lacked a unified algorithmic interpretation. We show that higher-order OTOCs naturally fit within the framework of quantum signal processing (QSP): each OTOC(k) measures the 2k-th Fourier component of the phase distribution associated with the singular values of a spatially resolved truncated propagator. This explains the contrasting sensitivities of time-ordered correlators (TOCs) and higher-order OTOCs to causal-cone structure and to chaotic, integrable, or localized dynamics. Based on this understanding, we further generalize higher-order OTOCs by polynomial transformation of the singular values of the spatially resolved truncated propagator. The resultant signal allows us to construct frequency-selective filters, which we call \emph{OTOC spectroscopy}. This extends conventional OTOCs into a mode-resolved tool for probing scrambling and spectral structure of quantum many-body dynamics.
Out-of-time-order correlators (OTOCs) can be used to probe how quickly a quantum system scrambles information when the initial conditions of the dynamics are changed. In sufficiently large quantum systems, one can extract from the OTOC the quantum analog of the Lyapunov coefficient that describes the timescale on which a classical chaotic system becomes scrambled. OTOCs have been applied only to a very limited number of toy models, such as the Sachdev-Ye-Kitaev model connected with black hole information scrambling, but they could find much wider applicability for information scrambling in quantum systems that allow comparison with experiments. The vibrations of polyatomic molecules are known to undergo a transition from regular dynamics at low energy to facile energy flow at sufficiently high energy. Molecules therefore represent ideal quantum systems to study scrambling in many-body systems of moderate size (here 6 to 36 degrees of freedoms). By computing quantum OTOCs and their classical counterparts we quantify how information becomes ``scrambled'' quantum mechanically in molecular systems. Between early ``ballistic'' dynamics, and late ``saturation'' of the OTOC when the full density of states is explored, there is indeed a regime where a quantum Lyapunov coefficient can be defined for all molecules in this study. Comparison with experimental rate data shows that slow scrambling as measured by the OTOC can reach the timescale of molecular reaction dynamics. Even for the smallest molecules we discuss, the Maldacena bound remains satisfied by regularized OTOCs, but not by unregularized OTOCs, highlighting that the former are more useful for discussing information scrambling in this type of moderate-size quantum system.
This tutorial article introduces the physics of quantum information scrambling in quantum many-body systems. The goals are to understand how to precisely quantify the spreading of quantum information and how causality emerges in complex quantum systems. We introduce a general framework to study the dynamics of quantum information, including detection and decoding. We show that the dynamics of quantum information is closely related to operator dynamics in the Heisenberg picture, and, under certain circumstances, can be precisely quantified by the so-called out-of-time-ordered correlator (OTOC). The general behavior of the OTOC is discussed based on several toy models, including the Sachdev-Ye-Kitaev model, random circuit models, and Brownian models, in which the OTOC is analytically tractable. We introduce numerical methods, including exact diagonalization and tensor network methods, to calculate the OTOC for generic quantum many-body systems. We also survey current experimental schemes for measuring the OTOC in various quantum simulators. Published by the American Physical Society 2024