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arXiv:2101.10945 · Physical Review Letters

Supermagnonic Propagation in Two-Dimensional Antiferromagnets

Giammarco Fabiani, M. D. Bouman, Johan H. Mentink

Published Aug 25, 2021• 22 citations
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Abstract

We investigate the propagation of magnons after ultrashort perturbations of the exchange interaction in the prototype two-dimensional Heisenberg antiferromagnet. Using the recently proposed neural quantum states, we predict highly anisotropic spreading in space constrained by the symmetry of the perturbation. Interestingly, the propagation speed at the shortest length scale and timescale is up to 40% higher than the highest magnon velocity. We argue that the enhancement stems from extraordinary strong magnon-magnon interactions, suggesting new avenues for manipulating information transfer on ultrashort length scales and timescales.

DOI
10.1103/physrevlett.127.097202

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We investigate the propagation of magnons after ultrashort perturbations of the exchange interaction in the prototype two-dimensional Heisenberg antiferromagnet. Using the recently proposed neural quantum states, we predict highly anisotropic spreading in space constrained by the symmetry of the perturbation. Interestingly, the propagation speed at the shortest length scale and timescale is up to 40% higher than the highest magnon velocity. We argue that the enhancement stems from extraordinary strong magnon-magnon interactions, suggesting new avenues for manipulating information transfer on ultrashort length scales and timescales.
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We numerically study the real space-time dynamics of magnon pairs in the two-dimensional antiferromagnetic Heisenberg model after short perturbations of the exchange interaction. Analogous to the dynamics following quantum quenches in one dimension, we find ultrafast light-cone like spreading of quantum spin correlations. Interestingly, the spreading speed is larger than can be expected from the highest magnon or spinon group velocities. Opposed to results in one dimension, the evolution of entanglement is not directly linked to the spreading and dictated by the coherent dynamics of nearest neighbour correlations. We show that this enables coherent control of both phase and amplitude of entanglement oscillations. All results are obtained with the recently proposed neural quantum states.
We investigate entanglement dynamics in the antiferromagnetic Heisenberg model in two dimensions following a spatially anisotropic quench of the exchange interactions. Opposed to established results in one dimension, the magnon quasiparticles show an initial growth of entanglement dynamics that does not depend on the system size and is governed by the oscillation period of the exchange interaction. We ascribe this to the dominance of the intrinsic entanglement of short wavelength nonpropagating magnon pairs, which also leads to a competition between area-law and volume-law contribution in the entanglement dynamics. Furthermore, by adopting the neural-network quantum states, we provide numerical evidence that this behavior survives even in the presence of strong magnon-magnon interactions, suggesting intriguing avenues for manipulating entanglement dynamics in quantum materials.
In this thesis the elementary excitations of the spin-1=2 Heisenberg antiferromagnet on the square lattice are studied. This fundamental model is a paradigmatic example for long range ordered quantum phases and the spontaneous breaking of a continuous symmetry in condensed matter. The elementary excitations at long wavelengths are well understood by quantized spin waves, i.e., magnons, which are the gapless Goldstone bosons of the broken SU(2) symmetry. However, recent findings reveal an anomalous energy dip at short wavelengths, which cannot be explained by the conventional spin wave theory. The nature of spin waves at short wavelengths remains unclear to this day. A central aim of this thesis is the derivation of an effective magnon description for the square lattice antiferromagnet which is quantitatively valid for all length scales. For this purpose, the method of continuous unitary transformations (CUT) is extended to its use for gapless excitations. CUT methods provide a powerful tool for the derivation of effective quasi-particle descriptions by means of flow equations. However, typical approaches are truncated in real space restricting their scope of application to gapped quantum phases. In order to circumvent these limitations a CUT approach in momentum space is developed. The scaling dimension of operator terms is established as a suitable truncation criterion for gapless quasi-particles. Moreover, a diagrammatic representation of operator terms is introduced which simplifies the derivation and interpretation of flow equations in momentum space. The developed approach is used to transform the Heisenberg Hamiltonian into an effective Hamiltonian which conserves the number of magnons. In addition, effective observables required for the theoretical description of inelastic neutron scattering are derived. The initial magnon operators before the transformation are defined by the Dyson-Maleev representation which leads to a superficially non-hermitian Hamiltonian. As a result, the transformation constitutes a continuous similarity transformation (CST). This formalism enables the formulation of spin wave interactions by means of quartic boson operators. A crucial step of the transformation is the proper renormalization of the spin wave interaction which is achieved by a selfsimilar CST for scaling dimension d = 2. The resulting effective magnon description is consistent at all length scales. In particular, the magnon dispersion exhibits an energy dip at short wavelengths which is in quantitative agreement with recent numerical and experimental data. Further analysis of the spectral properties indicates a strong attraction between spin waves giving rise to a resonance in the longitudinal two-magnon channel. This resonance can be interpreted as the amplitude or Higgs mode of the continuously broken SU(2) symmetry with finite lifetime. The origin of the anomalous dispersion is ascribed to a scattering between the Higgs resonance and single magnon states. The theoretical results are directly compared with experimental data obtained by inelastic neutron scattering and various numerical results which support this view. The quantitative agreement between the effective spin wave approach and numerous numerical and experimental findings shows that magnons are a valid description of the elementary excitations at all length scales. Therefore, this thesis provides a final settlement of the question about the nature of the elementary excitations in the square lattice quantum antiferromagnet.
This thesis investigates two-dimensional quantum antiferromagnets, with a focus on the spin-12\frac{1}{2}21​ antiferromagnetic easy-axis XXZ model on a square and a honeycomb lattice. Describing the excitations and interactions of magnons in these models is of substantial interest, as magnons are the fundamental quasiparticles and can thus explain experimental observations. Already for the paradigmatic antiferromagnetic spin-12\frac{1}{2}21​ Heisenberg model on the square lattice, high-energy features of the magnon dispersion are understood via strong magnon-magnon interactions. Besides that, interesting high-energy features were recently observed in the honeycomb lattice, including a possible decay of the single-magnon mode. The goal of this thesis is to obtain effective descriptions of the aforementioned systems that capture the relevant features of the magnon excitations and their interactions. To study these features, this thesis employs continuous similarity transformations (CSTs), which enables a systematic derivation of an effective quasiparticle picture via so-called flow equations. The approach enables decoupling different magnon sectors and thus for investigating ground-state properties, single-magnon excitations, and multi-magnon bound states. The magnon description is derived from the non-Hermitian Dyson-Maleev representation, which describes fluctuations around a long-range magnetically ordered ground state. The flow equations are set up in momentum space, truncated by the scaling dimension, retaining only operators up to scaling dimension of two, and solved numerically. For the square lattice, a magnon-conserving effective Hamiltonian is obtained across the full anisotropy range by interpolating between the Ising limit and the Heisenberg limit. The ground-state energy, staggered magnetization, dispersion, and critical exponents are in excellent agreement with the literature, supporting the validity of CST also for gapped phases. Two-magnon excitations in the Sz=0S^z=0Sz=0 subspace comprise four bound states, which are tracked across the anisotropy range. Their successive decay into the two-magnon continuum is determined by using the inverse participation ratio. For the honeycomb lattice, the magnon-conserving CST is reliable only up to λ≲0.57\lambda ≲ 0.57λ≲0.57; an adapted CST scheme that decouples only the ground state while preserving couplings between different higher-magnon sectors yields effective descriptions for all λ\lambdaλ and confirms stable long-range order. The low-energy properties determined in this way match the literature values. However, in the Heisenberg limit, the adapted approach fails to capture high-energy features, such as the experimentally observed decay into the multi-particle continuum at corners of the Brillouin zone. A termination of the magnon-conserving flow equations at a finite flow parameter before the divergence reveals a single-magnon decay at high energies, which is connected to a crossing of a two-magnon bound state with the single-magnon mode. The observed energy dip qualitatively agrees with Quantum Monte Carlo results, but magnon–magnon interactions are overestimated, hindering a fully quantitative characterization of the single-magnon dispersion. Analyzing multi-magnon bound states over the anisotropy range unveils that the crossing of a three-magnon bound state with the single-magnon mode accounts for the breakdown of the magnon-conserving CST at higher λ\lambdaλ. This work demonstrates that CST with scaling-dimension truncation provides a powerful framework for studying two-dimensional quantum magnets, capturing low-energy properties and bound states. Nevertheless, challenges remain in accurately describing high-energy features arising from a persistent overlap of magnon sectors due to strong binding effects.
We develop an approach to describe antiferromagnetic magnons on a bipartite lattice supporting the N\'eel state using fractionalized degrees of freedom typically inherent to quantum spin liquids. In particular, we consider a long-range magnetically ordered state of interacting two-dimensional quantum spin-1/21/21/2 XY models using the Chern-Simons (CS) fermion representation of interacting spins. The interaction leads to Cooper instability and pairing of CS fermions, and to CS superconductivity which spontaneously violates the continuous U(1)\mathrm{U}(1)U(1) symmetry generating a linearly dispersing gapless Nambu-Goldstone mode due to phase fluctuations. We evaluate this mode and show that it is in high-precision agreement with magnons of the corresponding N\'eel antiferromagnet irrespective to the lattice symmetry. Using the fermion formulation of the system with frustration, we show that the competing interactions emerge in the form of long-range interaction vertices mediated by the CS gauge field, which are responsible for restoring the continuous symmetry at sufficiently strong frustration. We identify these new interaction vertices and discuss their implications for unconventional phase transitions. We also apply the proposed theory to a model of anyons that can be tuned continuously from fermions to bosons, and discuss the results.