Metasurfaces have recently entered the realm of quantum photonics, enabling manipulation of quantum light using a compact nanophotonic platform. Realizing the full potential of metasurfaces at the deepest quantum level requires the ability to tune coherent light-matter interactions continuously in space and time. Here, we introduce the concept of space-time quantum metasurfaces for arbitrary control of the spectral, spatial, and spin properties of nonclassical light using a compact photonic platform. We show that space-time quantum metasurfaces allow on-demand tailoring of entanglement among all degrees of freedom of a single photon. We also show that spatiotemporal modulation induces asymmetry at the fundamental level of quantum fluctuations, resulting in the generation of steered and vortex photon pairs out of vacuum. Space-time quantum metasurfaces have the potential to enable novel photonic functionalities, such as encoding quantum information into high-dimensional color qudits using designer modulation protocols, sculpting multispectral and multispatial modes in spontaneous emission, and generating reconfigurable hyperentanglement for high-capacity quantum communications.
Metasurfaces have recently entered the realm of quantum photonics, enabling manipulation of quantum light using a compact nanophotonic platform. Realizing the full potential of metasurfaces at the deepest quantum level requires the ability to tune coherent light-matter interactions continuously in space and time. Here, we introduce the concept of space-time quantum metasurfaces for arbitrary control of the spectral, spatial, and spin properties of nonclassical light using a compact photonic platform. We show that space-time quantum metasurfaces allow on-demand tailoring of entanglement among all degrees of freedom of a single photon. We also show that spatiotemporal modulation induces asymmetry at the fundamental level of quantum fluctuations, resulting in the generation of steered and vortex photon pairs out of vacuum. Space-time quantum metasurfaces have the potential to enable novel photonic functionalities, such as encoding quantum information into high-dimensional color qudits using designer modulation protocols, sculpting multispectral and multispatial modes in spontaneous emission, and generating reconfigurable hyperentanglement for high-capacity quantum communications.
Recent progress in meta-optics, particularly the development of metasurfaces, has enabled compact, tunable, and integrable control over the amplitude, phase, polarization, and wavefront of light, thereby allowing a paradigm shift in traditional optical science and engineering. In parallel, the ability to generate and precisely manipulate nonclassical light is central to quantum optics, enabling key functionalities in secure quantum communication, precision measurement, and scalable quantum computation. This review aims to bridge these two rapidly advancing fields by presenting recent progress in the application of structured materials to the manipulation of quantum states of light. We begin by introducing the concept of singular optics, followed by a discussion of various families of spatially and temporally structured beams that form the foundation for many of the phenomena explored in quantum photonics. Next, we revisit the theoretical framework of quantum optics, including the formalism of photon quantization and the principles governing quantum frequency conversion. We then examine how metasurfaces can be engineered to enable highly efficient nonlinear quantum processes, including both up-conversion and down-conversion, thereby offering new approaches for generating and controlling complex quantum states. Furthermore, we discuss the crucial role of structured materials in shaping the properties of quantum light and in applications such as quantum ghost imaging. The review concludes by identifying emerging directions for integrating meta-optical platforms with quantum systems, highlighting their potential for scalable manipulation of nonclassical light at the nanoscale.
All-dielectric optical metasurfaces are a workhorse in nano-optics, because of both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to 2 orders of magnitude, compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons-a new promising platform for quantum optics experiments.
The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.
Hybrid integration of solid-state quantum emitters (QEs) into nanophotonic structures opens enticing perspectives for exploiting multiple degrees of freedom of single-photon sources for on-chip quantum photonic applications. However, the state-of-the-art single-photon sources are mostly limited to two-level states or scalar vortex beams. Direct generation of high-dimensional structured single photons remains challenging, being still in its infancy. Here, we propose a general strategy to design highly entangled high-dimensional spin-orbital single-photon sources by taking full advantage of the spatial freedom to design QE-coupled composite (i.e., Moiré/multipart) metasurfaces. We demonstrate the generation of arbitrary vectorial spin-orbital photon emission in high-dimensional Hilbert spaces, mapping the generated states on hybrid-order Bloch spheres. We further realize single-photon sources of high-dimensional spin-orbital quantum emission and experimentally verify the entanglement of high-dimensional superposition states with high fidelity. We believe that the results obtained facilitate further progress in integrated solutions for the deployment of next-generation high-capacity quantum information technologies.
In recent decades, quantum information technologies have attracted significant attention and experienced rapid development due to their ultrafast processing speeds and high level of information security. A significant trend in this field of study involves the ongoing pursuit of integrating and miniaturizing quantum devices. Metasurfaces, which are artificially designed planar nanostructure arrays with versatile wavefront shaping capabilities, present a promising platform for the development of integrated photonic quantum devices by effectively controlling quantum light in multiple degrees of freedom. In this review, recent advances in the field of quantum photonics facilitated by metasurfaces, encompassing quantum light sources, manipulation and measurement of quantum states, and the intriguing functionalities of quantum metasurfaces, are summarized. Additionally, potential future directions for the advancement of quantum metasurfaces are discussed.
Quantum skyrmions are topological structures that have garnered significant interest due to their demonstrated robustness and versatility across diverse optical platforms. However, existing approaches for their generation are limited to producing pre-determined two dimensional qubit states with a single topology. Here we create multi-dimensional topological states by introducing a non-local interaction between high-dimensional photonic entanglement and a metasurface, where the topological transformation induced by the metasurface is made non-deterministic by the probabilistic nature of the interfacing entangled state. Within this framework, we demonstrate that individual quantum states can host multiple co-existing topologies that are only revealed upon measurement, allowing for their parallel transport within distinct spatial mode channels. We confirm this by revealing the rich topological landscape within our modified Hilbert space while controlling the desired output topology by orbital angular momentum (OAM) projections on one of the entangled photons, producing multiple non-local polarization-OAM entangled states characterized by distinct topological classes, all from a single metasurface device. Our results reveal new capability when structured high-dimensional entanglement is interfaced with structured matter capable of coupling photonic degrees of freedom, establishing a new pathway for the compact generation of complex quantum states.