We elaborate a comprehensive theory of the sharp variations of the four-wave-mixing (FWM) threshold happening with the tuning of the pump frequency along the dispersive tails of the nonlinear resonance in the driven Kerr microresonators with high finesses and high finesse dispersions. Our theory leads to the explicit estimates for the difference in the pump powers required for the excitation of one sideband pair with momenta $\ifmmode\pm\else\textpm\fi{}\ensuremath{\mu}$ and for the simultaneous excitation of the two neighboring pairs with momenta $\ifmmode\pm\else\textpm\fi{}\ensuremath{\mu}, \ifmmode\pm\else\textpm\fi{}(\ensuremath{\mu}+1)$. This power difference also measures the depth of the Arnold tongues in the pump-frequency and pump-power parameter space, associated with the aforementioned power variations. A set of select pump frequencies and powers, where the instabilities of the two sideband pairs come first, forms the threshold of complexity, which is followed by a sequence of conditions specifying critical powers for the simultaneous instabilities of three, four and so on pairs. We formally link finesse dispersion and the density of states notion borrowed from the condensed matter context, and report a value of the finesse dispersion and a critical mode number signaling the transition from the low- to the high-contrast tongue structure. We also demonstrate that the large finesse dispersion makes possible a surprising for the multimode resonators regime of the bistability without FWM.
We elaborate a comprehensive theory of the sharp variations of the four-wave-mixing (FWM) threshold happening with the tuning of the pump frequency along the dispersive tails of the nonlinear resonance in the driven Kerr microresonators with high finesses and high finesse dispersions. Our theory leads to the explicit estimates for the difference in the pump powers required for the excitation of one sideband pair with momenta \ifmmode±\else\textpm\fi\ensuremathμ and for the simultaneous excitation of the two neighboring pairs with momenta \ifmmode±\else\textpm\fi\ensuremathμ,\ifmmode±\else\textpm\fi(\ensuremathμ+1). This power difference also measures the depth of the Arnold tongues in the pump-frequency and pump-power parameter space, associated with the aforementioned power variations. A set of select pump frequencies and powers, where the instabilities of the two sideband pairs come first, forms the threshold of complexity, which is followed by a sequence of conditions specifying critical powers for the simultaneous instabilities of three, four and so on pairs. We formally link finesse dispersion and the density of states notion borrowed from the condensed matter context, and report a value of the finesse dispersion and a critical mode number signaling the transition from the low- to the high-contrast tongue structure. We also demonstrate that the large finesse dispersion makes possible a surprising for the multimode resonators regime of the bistability without FWM.
We have shown previously that two strong laser beams (with the same frequency) counterpropagating in a Kerr nonlinear medium with linear dispersion become un stable when their intensities exceed a certain threshold.1 We demonstrate here that the system exhibits large (theoretically unlimited) amplification of a probe beam when the two pumping beams have their intensities slightly below the threshold. This is in contrast to the conventional phase conjugation due to four-wave mixing in a nondispersive Kerr nonlinear medium. The mechanism of amplification in our system can be explained in terms of positive distributed feedback from the Kerr nonlinear index grating formed by two strong pumping laser beams in the presence of dispersion giving rise to a light-induced distributed-feedback resonator. This feedback is attributed to the fact that the weak beams with both signal frequency, ω + δ, and conjugate frequency, ω − δ, propagate with phase speed different (due to dispersion) from that of a pumping wave with frequency ω, which triggers the exponentially increasing energy exchange between weak and strong beams at the nonlinear index grating (this energy exchange is prohibited in nondispersive media). When the probe frequency approaches a frequency of one of the longitudinal modes of the light-induced distributed resonator, and the pumping intensity approaches the threshold of instability, the resonant amplification increases infinitely; for presently available laser intensity stabilities, amplification as large as 104 is feasible.
The dynamical behavior of Kerr optical frequency combs is very well understood today from the perspective of the semiclassical approximation. These combs are obtained by pumping an ultrahigh-Q whispering-gallery mode resonator with a continuous-wave laser. The long-lifetime photons are trapped within the toruslike eigenmodes of the resonator, where they interact nonlinearly via the Kerr effect. In this article, we use quantum Langevin equations to provide a theoretical understanding of the nonclassical behavior of these combs when pumped below and above threshold. In the configuration where the system is under threshold, the pump field is the unique oscillating mode inside the resonator, and it triggers the phenomenon of spontaneous four-wave mixing, where two photons from the pump are symmetrically up- and down-converted in the Fourier domain. This phenomenon, also referred to as parametric fluorescence, can only be understood and analyzed from a fully quantum perspective as a consequence of the coupling between the field of the central (pumped) mode and the vacuum fluctuations of the various side modes. We analytically calculate the power spectra of the spontaneous emission noise, and we show that these spectra can be either single- or double-peaked depending on the value of the laser frequency, chromatic dispersion, pump power, and spectral distance between the central mode and the side mode of interest. We also calculate as well the overall spontaneous noise power per side mode and propose simplified analytical expressions for some particular cases. In the configuration where the system is pumped above threshold, we investigate the phenomena of quantum correlations and multimode squeezed states of light that can occur in the Kerr frequency combs originating from stimulated four-wave mixing. We show that for all stationary spatiotemporal patterns, the side modes that are symmetrical relative to the pumped mode in the frequency domain display quantum correlations that can lead to squeezed states of light under some optimal conditions that are analytically determined. These quantum correlations can persist regardless the dynamical state of the system (rolls or solitons), regardless of the spectral extension of the comb (number side modes) and regardless of the dispersion regime (normal or anomalous). We also explicitly determine the phase quadratures leading to photon entanglement and analytically calculate their quantum-noise spectra. For both the below- and above-threshold cases, we study with particular emphasis the two principal architectures for Kerr comb generation, namely the add-through and add-drop configurations. It is found that regardless of the configuration, an essential parameter is the ratio between out-coupling and total losses, which plays a key role as it directly determines the efficiency of the detected fluorescence or squeezing spectra. We finally discuss the relevance of Kerr combs for quantum information systems at optical telecommunication wavelengths below and above threshold.
Bichromatically pumped Kerr microresonators exhibit phase bistability and multistability arising from four-wave mixing between pump and generated modes. Here we analyze the symmetry structure of stationary solutions in the coupled-mode description of such systems. We show that the two-pump coupled-mode equations are a particular case of a more general model with pumps placed at equally spaced modes. For this model, any stationary solution generates a finite family of stationary solutions through a discrete phase transformation. This transformation leaves the equations invariant and preserves the stability type of the corresponding stationary states. As a consequence, the possible stationary values of each individual mode form a regular polygon in the complex plane. The number of vertices is determined by the order of the mode index μ in the group Zn, where n is the separation between the pumped modes. Thus, the phase multistability structure depends not only on nonlinear dynamics but also on the arithmetic relation between the mode index and the pump separation. These results provide a simple symmetry-based explanation for the discrete phase structure observed in multimode Kerr resonators under bichromatic pumping.
In optical fibers, nonlinear dispersion due to the same third-order susceptibility as that responsible for parametric mixing significantly alters the squeezing behavior in a traveling wave geometry, giving the squeezed quadrature an intensity dependent phase and reducing the overall squeezing. Phase noise is not squeezed at all. In the case of a fiber ring resonator, the nonlinear susceptibility will also lead to dispersive optical bistability and the squeezing will be strongly dependent on pump and sideband detuning. Yurke1 has analyzed squeezing due to backward four-wave mixing in a cavity, but the pump wave did not circulate in the cavity, and bistability was not dealt with. We have developed a theory of the resonant fiber ring interferometer, where the pump wave is near resonance with an interferometer mode and the circulating power is thereby enhanced. For perfect pump resonance and for frequencies corresponding to sideband resonance, the overall enhancement of the squeezing in the output mode compared to the traveling wave case is proportional to the square of the resonator finesse. The best squeezing in the output mode is always found for this condition of sideband resonance. The phase of the minimum noise quadrature is quite sensitive to both pump and sideband detuning. This feature may provide a means for avoiding excess thermal phase noise due to guided acoustic wave Brillouin scattering in the fiber itself. At the critical points for dispersive optical bistability in such a resonator and for sideband resonance (i.e., noise frequencies which are multiples of the resonator free spectral range), perfect squeezing of the output light is predicted. This result was also obtained previously for the case of degenerate mixing in a resonant cavity by Collett and Walls.2 Our current theory does not account for the reduction in squeezing due to the loss present in such a resonator.2 Since the loss is also enhanced by a factor of the resonator finesse, this is of some concern and will limit the maximum useful finesse for quantum noise squeezing. The major source of loss is the single-mode directional coupler, which for currently available technology is of the order of a few percent.
A common strategy for increasing the efficiency of Stimulated and Spontaneous FourWave Mixing (SFWM) in integrated optical devices, is to enhance the intensity of the propagating optical field through nanoscale geometrical engineering. Typically, this is accomplished by confining light into microresonators or into sequences of mutually coupled cavities. Usually these structures are treated as a whole, with tens or hundreds of repeating units. In these structures, long grange periodicity is deliberately sought to tailor the frequency wavevector band diagram, in order to increase the group index while keeping the group velocity dispersion as low as possible. Having to deal with a large number of unit cells inherently precludes the study of the impact of the internal degree of freedom on FWM. The implementation of complex and extended structures precludes the observation of FWM regimes which are in general hidden, or overhung, by the long range periodicity, and that can emerge only by acting at the single resonator level. In this work, we study SFWM in a system made by two Silicon microring resonators (photonic dimer) of radius 7 um, quality factor Q = 10000 and separation 53.1 um, which are indirectly coupled by means of two waveguides with a coupling gap of 160 nm. We independently change the inter-cavity phase f, and the resonator eigenfrequency detuning d, by respectively implementing a Peltier cell and micro-heaters placed on the top of the resonators. We experimentally and theoretically demonstrate that, in the parameter space spanned by (f, d), the efficiency of SFWM can be enhanced, left unchanged or being completely suppressed with the respect to a single uncoupled resonator. This plethora of regimes can not be easily resolved and accomplished in large structures, where the structural periodicity makes slow light to overwhelm any other side effect. Here, a FWM enhancement of 7 dB with respect to each single constituent of the molecule is demonstrated, and attributed to the increase of internal field enhancement of one of the resonator induced by the presence of the other. We theoretically prove that this phenomenon is linked to the excitation of a sub-radiant mode in the structure. FWM suppression arises from the coherent destructive interference between the signal waves generated in the two resonators which are scattered into a common waveguide channel. We find that in the region where SFWM is enhanced, also the efficiency of Spontaneous Four Wave Mixing, the quantum counterpart of the stimulated process, is increased. This opens a plenty of possibilities for the implementation of this device for the generation of correlated photon pairs. We suggest that pairs could be deterministically bunched into a single scattering channel with a brightness that overcomes the one of a critically coupled resonator. This could beat the effective 50% of losses which suffer All-Pass and Add-Drop resonators, and could show superior brightness with respect to asymmetric microrings or dual Mach-Zehnder-microrings devices, whose maximum achievable field enhancement is inherently limited by the level attained at critical coupling.
Quantum Kerr optical frequency combs are generated by pumping a high-Q microresonator with a continuous wave resonant laser. Below threshold, two pump photons are symmetrically up- and down-converted as twin photons via spontaneous four-wave mixing, thereby generating up to a hundred paired channels. Furthermore, these chipscale, high-dimensional and room-temperature systems are expected to play a major role in quantum engineering. However, their theoretical description is still unclear. Here, we present an explicit description of this quantum system via a frequency-bin state and its density operator, and explore the properties of the eigenkets.