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arXiv:2101.03565 · Physical Review A

Improving efficiency of sympathetic cooling in atom-ion and atom-atom confined collisions

Vladimir S. Melezhik

Published May 10, 2021• 13 citations
arXivHTMLPDF

Abstract

We propose a way for sympathetic cooling of ions in an electromagnetic Paul trap: it implies the use for this purpose of cold buffer atoms in the region of atom-ion confinement-induced resonance (CIR). The problem is that the unavoidable micromotion of the ion and the long-range nature of its interaction with the environment of colder atoms in a hybrid atomic-ion trap prevent its sympathetic cooling. We show that the destructive effect of ion micromotion on its sympathetic cooling can, however, be suppressed in the vicinity of the atom-ion CIR. Here, the resonant blocking of the complete approach of an atom with an ion during a collision also blocks the enhancement of its micromotion. We investigate the effect of sympathetic cooling around CIRs in atom-ion and atom-atom confined collisions within the quasiclassical-quantum approach using the $\mathrm{Li}\ensuremath{-}{\mathrm{Yb}}^{+}$ and Li-Yb confined systems as an example. In this approach, the Schr\"odinger equation for a cold light atom is integrated simultaneously with the classical Hamilton equations for a hotter heavy ion or atom during collision. We have found the region near the atom-ion CIR where the sympathetic cooling of the ion by cold atoms is possible in a hybrid atom-ion trap. We also show that it is possible to improve the efficiency of sympathetic cooling in atomic traps by using atomic CIRs.

DOI
10.1103/physreva.103.053109

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We investigate the problem of a single ion in a radio-frequency trap and immersed in an ultracold Bose gas either in condensed or non-condensed phase. We develop master equation formalism describing the sympathetic cooling and we determine the cooling rates and final energies of ions. We show that cold atomic reservoir modifies the stability diagram of the ion in the Paul trap creating the regions where the ion is either cooled or heated due to the energy quanta exchanged with the time-dependent potential. Our calculation indicates that micromotion constitutes an important source of heating limiting the final temperature of ions to values higher than 100$\mu$K for parameters of present experiments.

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We propose a way for sympathetic cooling of ions in an electromagnetic Paul trap: it implies the use for this purpose of cold buffer atoms in the region of atom-ion confinement-induced resonance (CIR). The problem is that the unavoidable micromotion of the ion and the long-range nature of its interaction with the environment of colder atoms in a hybrid atomic-ion trap prevent its sympathetic cooling. We show that the destructive effect of ion micromotion on its sympathetic cooling can, however, be suppressed in the vicinity of the atom-ion CIR. Here, the resonant blocking of the complete approach of an atom with an ion during a collision also blocks the enhancement of its micromotion. We investigate the effect of sympathetic cooling around CIRs in atom-ion and atom-atom confined collisions within the quasiclassical-quantum approach using the Li\ensuremath−Yb+\mathrm{Li}\ensuremath{-}{\mathrm{Yb}}^{+}Li\ensuremath−Yb+ and Li-Yb confined systems as an example. In this approach, the Schr"odinger equation for a cold light atom is integrated simultaneously with the classical Hamilton equations for a hotter heavy ion or atom during collision. We have found the region near the atom-ion CIR where the sympathetic cooling of the ion by cold atoms is possible in a hybrid atom-ion trap. We also show that it is possible to improve the efficiency of sympathetic cooling in atomic traps by using atomic CIRs.
Abstract Sympathetic cooling of a Fermi gas with a buffer gas of bosonic atoms is an efficient way to achieve quantum degeneracy in Fermi systems. However, all attempts to use this method for cooling ions until recently were ineffective because of the unremovable ion “micromotion” in electromagnetic Paul traps, which prevents the realization of a number of hot projects with cold atom-ion systems. In this regard, we propose a new efficient method for sympathetic cooling of ions: the use for this purpose of cold buffer atoms in the region of atom-ion confinement-induced resonances (CIRs) [V.S. Melezhik, Phys. Rev. A103, 53109 (2021)]. We show that the destructive effect of “micromotion” on its sympathetic cooling can, however, be suppressed in the vicinity of the atom-ion CIR. Here, the resonant blocking of a close collision of an atom with an ion also resists its heating due to “micromotion”. We investigate the effect of sympathetic cooling around CIRs in atom-ion, and atom-atom confined collisions within the quantum-quasiclassical approach using the Li–Yb+ and Li–Yb confined systems as an example. In this approach, the Schrödinger equation for a cold light atom is integrated simultaneously with the classical Hamilton equations for a hotter heavy-ion or atom during a collision. We have found the region near the atom-ion CIR where the sympathetic cooling of the ion by cold atoms is possible in a hybrid atom-ion trap. We also show that it is possible to improve the efficiency of sympathetic cooling in atomic traps by using atomic CIRs.
Sympathetic cooling of a Fermi gas with a buffer gas of bosonic atoms is an efficient way to achieve quantum degeneracy in Fermi systems. However, all attempts to use this method for cooling ions until recently were ineffective because of the unremovable ion “micromotion” in electromagnetic Paul traps, which prevents the realization of a number of hot projects with cold atom–ion systems. In this regard, we propose a new efficient method for sympathetic cooling of ions: the use for this purpose of cold buffer atoms in the region of atom–ion confinement-induced resonances (CIRs) (Melezhik V. S. // Phys. Rev. A. 2021. V. 103. P. 53109). We show that the destructive effect of “micromotion” on its sympathetic cooling can, however, be suppressed in the vicinity of the atom–ion CIR. Here, the resonant blocking of a close collision of an atom with an ion also resists its heating due to “micromotion”. We investigate the effect of sympathetic cooling around CIRs in atom–ion and atom–atom confined collisions within the quantum-quasiclassical approach using the Li–Yb+ and Li–Yb confined systems as an example. In this approach, the Schrodinger equation for a cold light atom is integrated simultaneously ¨ with the classical Hamilton equations for a hotter heavy ion or atom during a collision. We have found the region near the atom–ion CIR where the sympathetic cooling of the ion by cold atoms is possible in a hybrid atom–ion trap. We also show that it is possible to improve the efficiency of sympathetic cooling in atomic traps by using atomic CIRs.
We present, and derive analytic expressions for, a fundamental limit to the sympathetic cooling of ions in radio-frequency traps using cold atoms. The limit arises from the work done by the trap electric field during a long-range ion-atom collision and applies even to cooling by a zero-temperature atomic gas in a perfectly compensated trap. We conclude that in current experimental implementations, this collisional heating prevents access to the regimes of single-partial-wave atom-ion interaction or quantized ion motion. We determine conditions on the atom-ion mass ratio and on the trap parameters for reaching the s-wave collision regime and the trap ground state.
Abstract Reaching ultracold temperatures within hybrid atom–ion systems is a major limiting factor for control and exploration of the atom–ion interaction in the quantum regime. In this work, we present results on numerical simulations of trapped ion buffer gas cooling using an ultracold atomic gas in a large number of experimentally realistic scenarios. We explore the suppression of micromotion-induced heating effects through optimization of trap parameters for various radio-frequency (rf) traps and rf driving schemes including linear and octupole traps, digital Paul traps, rotating traps and hybrid optical/rf traps. We find that very similar ion energies can be reached in all of them even when considering experimental imperfections that cause so-called excess micromotion. Moreover we look into a quantum description of the system and show that quantum mechanics cannot save the ion from micromotion-induced heating in an atom–ion collision. The results suggest that buffer gas cooling can be used to reach close to the ion’s groundstate of motion and is even competitive when compared to some sub-Doppler cooling techniques such as Sisyphus cooling. Thus, buffer gas cooling is a viable alternative for ions that are not amenable to laser cooling, a result that may be of interest for studies into cold controlled quantum chemistry and charged impurity physics.
Ultracold atom-ion systems have been a topic of interest for atomic physicists studying chemical reactions and since recently, the cold ion community (ion trap quantum computation and simulation). They have been looking at the possibility of using an ultracold atom gas to sympathetically cool ions since intrinsic motional modulation i.e micromotion is an inherent cause of decoherence in coherent applications of cold ions. Interest is also piqued by the possibility of using this hybrid system for studying impurity physics and to better understand ion-neutral reactions aimed at creation of molecular ions. In this thesis, we aim to study the effect of ion micromotion in atom-ion collision. As a prelude, we treat the 1D collision of a particle in a harmonic trap (ion) and a free particle (atom) using different numerical schemes. This system is of interest in its own right due to the mixed 0D-1D dimensionality. Atom-ion potential is simplified to a zero range potential all through out the work. Next we deal with a similar problem but with the trapped particle in a time dependent harmonic trap identical to an ion Paul trap. Finally we extend the study of micromotion to a model system in 3D with an ion in a 3D spherical Paul trap and a heavy atom at the trap centre. We discuss the effect micromotion has on potential applications of such a system, like a quantum phase gate.
We investigate the problem of a single ion in a radio-frequency trap and immersed in an ultracold Bose gas either in condensed or non-condensed phase. We develop master equation formalism describing the sympathetic cooling and we determine the cooling rates and final energies of ions. We show that cold atomic reservoir modifies the stability diagram of the ion in the Paul trap creating the regions where the ion is either cooled or heated due to the energy quanta exchanged with the time-dependent potential. Our calculation indicates that micromotion constitutes an important source of heating limiting the final temperature of ions to values higher than 100μ\muμK for parameters of present experiments.