Engineering quantum phases using light is a novel route to designing functional materials, where lightinduced superconductivity is a successful example.Although this phenomenon has been realized experimentally, especially for the high-T c cuprates, the underlying mechanism remains mysterious.Using the recently developed variational non-Gaussian exact diagonalization method, we investigate a particular type of photoenhanced superconductivity by suppressing a competing charge order in a strongly correlated electron-electron and electron-phonon system.We find that the d-wave superconductivity pairing correlation can be enhanced by a pulsed laser, consistent with recent experiments based on gap characterizations.However, we also find that the pairing correlation length is heavily suppressed by the pump pulse, indicating that light-enhanced superconductivity may be of fluctuating nature.Our findings also imply a general behavior of nonequilibrium states with competing orders, beyond the description of a mean-field framework.
Engineering quantum phases using light is a novel route to designing functional materials, where lightinduced superconductivity is a successful example.Although this phenomenon has been realized experimentally, especially for the high-T c cuprates, the underlying mechanism remains mysterious.Using the recently developed variational non-Gaussian exact diagonalization method, we investigate a particular type of photoenhanced superconductivity by suppressing a competing charge order in a strongly correlated electron-electron and electron-phonon system.We find that the d-wave superconductivity pairing correlation can be enhanced by a pulsed laser, consistent with recent experiments based on gap characterizations.However, we also find that the pairing correlation length is heavily suppressed by the pump pulse, indicating that light-enhanced superconductivity may be of fluctuating nature.Our findings also imply a general behavior of nonequilibrium states with competing orders, beyond the description of a mean-field framework.
Time-domain techniques have shown the potential of photomanipulating existing orders and inducing new states of matter in strongly correlated materials. Using time-resolved exact diagonalization, we perform numerical studies of pump dynamics in a Mott-Peierls system with competing charge and spin density waves. A light-enhanced d-wave superconductivity is observed when the system resides near a quantum phase boundary. By examining the evolution of spin, charge, and superconducting susceptibilities, we show that a subdominant state in equilibrium can be stabilized by photomanipulating the charge order to allow superconductivity to appear and dominate. This work provides an interpretation of light-induced superconductivity from the perspective of order competition and offers a promising approach for designing novel emergent states out of equilibrium.
Light offers a route to engineer new phases of matter far from equilibrium, including transient states suggestive of superconducting, charge-ordered, and excitonic ordering behavior. Yet it remains unclear how optical excitation can dynamically produce long-range phase coherence-a defining feature of true order such as superconductivity-rather than merely enhancing local pairing. Here we show that impulsively driven low-frequency phonons enhance long-range electronic correlations in a low-dimensional metal. Through numerically exact simulations, we demonstrate that slow phonons suppress dynamical disorder, enabling buildup of coherence and enhancement of charge (and pairing) orders. These findings provide direct evidence that light can mediate enhancement of long-range order and suggest that future experimental strategies-such as the design of selective excitations of narrow phonon distributions to limit dephasing-may offer viable routes to design and stabilize transient superconducting states.
We study the nonequilibrium dynamics of an electronic model of competition between an unconventional charge density wave (a bond density wave) and d-wave superconductivity. In a time-dependent Hartree-Fock+BCS approximation, the dynamics reduces to the equations of motion of operators realizing the generators of SU(4) at each pair of momenta, $(\mathbit{k},\ensuremath{-}\mathbit{k})$, in the Brillouin zone. We also study the nonequilibrium dynamics of a quantum generalization of a O(6) nonlinear $\ensuremath{\sigma}$ model of competing orders in the underdoped cuprates [Hayward et al., Science 343, 1336 (2014)]. We obtain results, in the large N limit of a O(N) model, on the time dependence of correlation functions following a pulse disturbance. We compare our numerical studies with recent picosecond optical experiments. We find that, generically, the oscillatory responses in our models share various qualitative features with the experiments.
The principal purpose of this topical review is to single out some of the universal features of high-temperature (high-Tc) and related strongly-correlated systems, which can be compared with experiment in a quantitative manner. The description starts with the concept of exchange-interaction-mediated (real-space) pairing, combined with strong correlations among narrow band electrons, for which the reference state is that of the Mott–Hubbard insulator. The physical discussion of concrete properties relies on variational approach, starting from generalized renormalized mean-field theory (RMFT) in the form of statistically-consistent Gutzwiller approximation (SGA), and its subsequent generalization, i.e., a systematic Diagrammatic Expansion of the Variational (Gutzwiller-type) Wave Function (DE-GWF). The solution leads to the two energy scales, one involving unconventional quasiparticles close to the Fermi energy, and the other reflecting the fully correlated state, involving electrons deeper below the Fermi surface. Those two regimes are separated by a kink in the dispersion relation, which is observed in photoemission. As a result, one obtains both the doping dependent properties in the correlated state, and effective renormalized quasiparticles. The reviewed ground-state characteristics for high-Tc systems encompass high-Tc superconductivity, nematicity, charge- (and pair-) density-wave effects, as well as non-BCS kinetic energy gain in the paired state. The calculated dynamic properties are: the universal Fermi velocity, the Fermi wave-vector, the effective mass enhancement, the pseudogap; and the d-wave gap magnitude. We discuss that, within the variational approach, the minimal realistic model is represented by the so-called t-J-U Hamiltonian. Inadequacy of the t-J and Hubbard models, particularly of their RMFT versions, is discussed explicitly. For heavy fermion systems, modeled by the Anderson lattice model and with the DE-GWF approach, we discuss the phase diagram, encompassing superconducting, Kondo insulating, ferro- and anti-ferromagnetic states. The superconducting state is then a two-d-wave gap system. If the orbital degeneracy of f-electrons is included, the coexistent ferromagnetic- (spin–triplet) superconducting phases appear and match those observed for UGe2 in a semiquantitative manner. Finally, in the second part, we generalize our approach to the collective spin and charge fluctuations in high-Tc systems, starting from variational approach, defining the saddle-point state, and combining it with 1/N expansion. The present scheme differs essentially from that starting from the saddle-point Hartree–Fock approximation, and incorporating the fluctuations in the random phase approximation (RPA). The spectrum of collective spin and charge excitations is determined for the Hubbard and t-J-U models, and subsequently compared quantitatively with recent experiments. The Appendices provide formal details to make this review self-contained.
We investigate the nonequilibrium dynamics of competing coexisting superconducting (SC) and charge-density wave (CDW) orders in an attractive Hubbard model. A time-periodic laser field A[over →](t) lifts the SC-CDW degeneracy, since the CDW couples linearly to the field (A[over →]), whereas SC couples in second order (A[over →]^{2}) due to gauge invariance. This leads to a striking resonance: When the photon energy is red detuned compared to the equilibrium single-particle energy gap, CDW is enhanced and SC is suppressed, while this behavior is reversed for blue detuning. Both orders oscillate with an emergent slow frequency, which is controlled by the small amplitude of a third induced order, namely η pairing, given by the commutator of the two primary orders. The induced η pairing is shown to control the enhancement and suppression of the dominant orders. Finally, we demonstrate that light-induced superconductivity is possible starting from a predominantly CDW initial state.
Intense time-periodic laser fields can transform the electronic structure of a solid into strongly modified Floquet-Bloch bands. While this suggests multiple pathways to induce electronic orders such as superconductivity or charge density waves, the possibility of preparing low-energy phases of Floquet Hamiltonians remains unclear because of the energy absorption at typical experimentally accessible driving frequencies. Here we investigate a realistic pathway towards laser control of electronic orders, which is the transient enhancement of fluctuating orders. Using a conserving Keldysh Green's function formalism, we simulate the buildup of short range Cooper-pair correlations out of a normal metal in the driven attractive Hubbard model. Even for frequencies only slightly above or within the bandwidth, a substantial enhancement of correlations can be achieved before the system reaches a high electronic temperature. This behavior relies on the nonthermal nature of the driven state. The effective temperature of the electrons at the Fermi surface, which more closely determines the superconducting correlations, remains lower than an estimate from the global energy density. Even though short ranged, the fluctuations can have marked signatures in the electronic spectra.