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arXiv:2011.11481 · Physical Review A

Interatomic interaction of two ground-state atoms in vacuum: Contributions of vacuum fluctuations and radiation reaction

Wenting Zhou, Shijing Cheng, Hongwei Yu

Published Jan 29, 2021• 13 citations
arXivHTMLPDF

Abstract

We generalize the formalism proposed by Dalibard, Dupont-Roc, and Cohen-Tannoudji (the DDC formalism) to the fourth order of the coupling constant, which can be used to study the interatomic interaction of two ground-state atoms coupled with the vacuum scalar fields. We show that the interatomic potential can be attributed to the joint effect of both vacuum fluctuations and the radiation reaction of atoms. Remarkably, the formulas we derived for the contributions of vacuum fluctuations and the radiation reaction to the interatomic potential upon which future research on fourth-order effects in particular circumstances can be based differ from those in the existing literature [Phys. Rev. D 95, 085014 (2017)].

DOI
10.1103/physreva.103.012227

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Abstract We generalize the formalism proposed by Dalibard, Dupont-Roc, and Cohen-Tannoudji (the DDC formalism) in the fourth order for two atoms in interaction with scalar fields in vacuum to a thermal bath at finite temperature T, and then calculate the interatomic interaction energy of two ground-state atoms separately in terms of the contributions of thermal fluctuations and the radiation reaction of the atoms and analyze in detail the thermal corrections to the van der Waals and Casimir–Polder interactions. We discover a particular region, i.e. λ 3 β 4 ≪ L ≪ λ with L, β and λ denoting the interatomic separation, the wavelength of thermal photons and the transition wavelength of the atoms respectively, where the thermal corrections remarkably render the van der Waals force, which is usually attractive, repulsive, leading to an interesting crossover phenomenon of the interatomic interaction from attractive to repulsive as the temperature increases. We also find that the thermal corrections cause significant changes to the Casimir–Polder force when the temperature is sufficiently high, resulting in an attractive force proportional to TL −3 in the λ ≪ β ≪ L region, and a force that can be either attractive or repulsive and even vanishing in the β ≪ λ ≪ L region depending on the interatomic separation.

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We investigate the resonance dipole-dipole interaction energy between two identical atoms, one in the ground state and the other in the excited state, interacting with the electromagnetic field in the presence of a perfectly reflecting plane boundary. The atoms are prepared in a correlated (symmetric or antisymmetric) Bell-type state. Following a procedure due to Dalibard et al. [J. Dalibard et al., J. Phys. (Paris) 43, 1617 (1982); J. Phys. (Paris) 45, 637 (1984)], we separate the contributions of vacuum fluctuations and radiation reaction (source) field to the resonance interaction energy between the two atoms and show that only the source field contributes to the interatomic interaction, while vacuum field fluctuations do not. By considering specific geometric configurations of the two-atom system with respect to the mirror and specific choices of dipole orientations, we show that the presence of the mirror significantly affects the resonance interaction energy and that different features appear with respect to the case of atoms in free space, for example, a change in the spatial dependence of the interaction. Our findings also suggest that the presence of a boundary can be exploited to tailor and control the resonance interaction between two atoms, as well as the related energy transfer process. The possibility of observing these phenomena is also discussed.

arXiv:1711.08249•Physical Review A•Apr 13, 2018•25 citations
We generalize the formalism proposed by Dalibard, Dupont-Roc, and Cohen-Tannoudji (the DDC formalism) to the fourth order of the coupling constant, which can be used to study the interatomic interaction of two ground-state atoms coupled with the vacuum scalar fields. We show that the interatomic potential can be attributed to the joint effect of both vacuum fluctuations and the radiation reaction of atoms. Remarkably, the formulas we derived for the contributions of vacuum fluctuations and the radiation reaction to the interatomic potential upon which future research on fourth-order effects in particular circumstances can be based differ from those in the existing literature [Phys. Rev. D 95, 085014 (2017)].
We give a general derivation of the fourth-order DDC formalism (a formalism proposed by Dalibard, Dupont-Roc, and Cohen-Tannoudji) for calculating the interaction energy between two ground-state multilevel atoms which are coupled to electromagnetic fields in a thermal bath at temperature TTT. Both the contributions of the thermal field fluctuations and the radiation reaction of atoms are separately identified. As an application of the formalism, we revisit the interaction energy of two static ground-state two-level atoms in a free space and discover new behaviors such as the $\ensuremath{\sim}T{L}^{\ensuremath{-}2}$ behavior of the van der Waals interaction energy in the region where ${\ensuremath{\lambda}}^{3/4}{T}^{\ensuremath{-}1/4}\ensuremath{\ll}L\ensuremath{\ll}\ensuremath{\lambda}$, with $\ensuremath{\lambda}$ the transition wavelength of the atoms and LLL the interatomic separation, and an oscillatory behavior of the Casimir-Polder interaction energy as LLL varies which is superimposed on the monotonic $\ensuremath{\sim}T{L}^{\ensuremath{-}6}$ dependence when $L\ensuremath{\gg}\ensuremath{\lambda}\ensuremath{\gg}{T}^{\ensuremath{-}1}$.
Abstract We generalize the formalism proposed by Dalibard, Dupont-Roc, and Cohen-Tannoudji (the DDC formalism) in the fourth order for two atoms in interaction with scalar fields in vacuum to a thermal bath at finite temperature T, and then calculate the interatomic interaction energy of two ground-state atoms separately in terms of the contributions of thermal fluctuations and the radiation reaction of the atoms and analyze in detail the thermal corrections to the van der Waals and Casimir–Polder interactions. We discover a particular region, i.e. λ 3 β 4 ≪ L ≪ λ with L, β and λ denoting the interatomic separation, the wavelength of thermal photons and the transition wavelength of the atoms respectively, where the thermal corrections remarkably render the van der Waals force, which is usually attractive, repulsive, leading to an interesting crossover phenomenon of the interatomic interaction from attractive to repulsive as the temperature increases. We also find that the thermal corrections cause significant changes to the Casimir–Polder force when the temperature is sufficiently high, resulting in an attractive force proportional to TL −3 in the λ ≪ β ≪ L region, and a force that can be either attractive or repulsive and even vanishing in the β ≪ λ ≪ L region depending on the interatomic separation.
We apply the DDC formalism [proposed by Dalibard, Dupont-Roc and Cohen-Tannoudji] to study the average rate of change of energy of two identical two-level atoms interacting with the vacuum massless scalar field in synchronized motion along stationary trajectories. By separating the contributions of vacuum fluctuations and atomic radiation reaction, we first show that for the two-atom system initially prepared in the factorizable eigenstates ∣gAgB⟩|{g}_{A}{g}_{B}⟩∣gA​gB​⟩ and ∣eAeB⟩|{e}_{A}{e}_{B}⟩∣eA​eB​⟩, where ggg and eee represent the ground state and the excited state of a single atom, respectively, both vacuum fluctuations and atomic radiation reaction contribute to the average rate of change of energy of the two-atom system, and the contribution of vacuum fluctuations is independent of the interatomic separation while that of atomic radiation reaction is dependent on it. This is contrary to the existing results in the literature where vacuum fluctuations are interatomic-separation dependent. However, if the two-atom system is initially prepared in the unfactorizable symmetric/antisymmetric entangled state, the average rate of change of energy of the two-atom system is never perturbed by the vacuum fluctuations, but is totally a result of the atomic radiation reaction. We then consider two special cases of motion of the two-atom system, which is initially prepared in the symmetric/antisymmetric entangled state, i.e., synchronized inertial motion and synchronized uniform acceleration. In contrast to the average rate of change of energy of a single uniformly accelerated atom, the average rate of change of energy of the uniformly accelerated two-atom system is nonthermal-like. The effects of noninertial motion on the transitions of states of the two correlated atoms are also discussed.
Abstract We study the interaction potential of two nonidentical ground-state atoms coupled to a scalar field in a vacuum by separately calculating the contributions of vacuum fluctuations and those of the radiation reaction of the atoms. Both cases of atoms in a free space and in parallel or vertical alignment to a reflecting boundary are considered. For the former case, we find that the leading-order interaction potential in the region λ A ≪ L ≪ λ B exhibits the same separation-dependence as that in the region L ≪ λ A ≪ λ B , where L, λ A and λ B are respectively the interatomic separation and the transition wavelengths of two atoms with λ A ≪ λ B . For the latter case, we find that boundary-induced modifications are very remarkable when L ≫ z, with z characterizing the separation between the two-atom system and the boundary. Particularly, when L further satisfies L ≫ λ A and L ≫ λ B , the interaction potential in the parallel- and the vertical-alignment cases respectively scales as z 4 L −7 and z 2 L −5, the L-dependence of which is one order higher than those of two atoms in regions where L ≫ z and meanwhile L ≪ λ A or/and L ≪ λ B . Our results suggest that retardation for the interaction potential of two nonidentical atoms with remarkably distinctive transition frequencies happens only when the interatomic separation is much greater than the transition wavelengths of both atoms.
Dalibard, Dupont-Roc and Cohen-Tannoudji (J. Physique 43 (1982) 1617; 45 (1984) 637) used the Heisenberg picture to show that the atomic transitions, and the stability of the ground state, can only be explained by introducing radiation reaction and vacuum fluctuation forces. Here we consider the simple case of nonrelativistic charged harmonic oscillator, in one dimension, to investigate how to take into account the radiation reaction and vacuum fluctuation forces within the Schrodinger picture. We consider classical vacuum fields and large mass oscillator.
We investigate the resonance dipole-dipole interaction energy between two identical atoms, one in the ground state and the other in the excited state, interacting with the electromagnetic field in the presence of a perfectly reflecting plane boundary. The atoms are prepared in a correlated (symmetric or antisymmetric) Bell-type state. Following a procedure due to Dalibard et al. [J. Dalibard et al., J. Phys. (Paris) 43, 1617 (1982); J. Phys. (Paris) 45, 637 (1984)], we separate the contributions of vacuum fluctuations and radiation reaction (source) field to the resonance interaction energy between the two atoms and show that only the source field contributes to the interatomic interaction, while vacuum field fluctuations do not. By considering specific geometric configurations of the two-atom system with respect to the mirror and specific choices of dipole orientations, we show that the presence of the mirror significantly affects the resonance interaction energy and that different features appear with respect to the case of atoms in free space, for example, a change in the spatial dependence of the interaction. Our findings also suggest that the presence of a boundary can be exploited to tailor and control the resonance interaction between two atoms, as well as the related energy transfer process. The possibility of observing these phenomena is also discussed.