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arXiv:2011.05256 · Physical Review Letters

Spin Susceptibility above the Superfluid Onset in Ultracold Fermi Gases

Yun Long, Feng Xiong, Colin Parker

Published Apr 14, 2021• 12 citations
arXivHTMLPDF

Abstract

Ultracold atomic Fermi gases can be tuned to interact strongly, which produces a display of spectroscopic signatures above the superfluid transition reminiscent of the pseudogap in cuprates. However, the extent of the analogy can be questioned since many thermodynamic quantities in the low temperature spin-imbalanced normal state can be described successfully using Fermi liquid theory. Here we present spin susceptibility measurements across the interaction strength-temperature phase diagram using a novel radio frequency technique with ultracold ^{6}Li gases. For all significant interaction strengths and at all temperatures we find the spin susceptibility is reduced compared to the equivalent value for a noninteracting Fermi gas. At unitarity, we can use the local density approximation to extract the integrated spin susceptibility for the uniform gas as a function of temperature, which at high temperatures is generally less than theoretically predicted. At low temperatures, our data lie within the range of theoretical predictions, although we can also describe the entire curve using a very simple one-parameter mean field model with monotonically increasing spin susceptibility.

DOI
10.1103/physrevlett.126.153402

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Ultracold atomic Fermi gases can be tuned to interact strongly, which produces a display of spectroscopic signatures above the superfluid transition reminiscent of the pseudogap in cuprates. However, the extent of the analogy can be questioned since many thermodynamic quantities in the low temperature spin-imbalanced normal state can be described successfully using Fermi liquid theory. Here we present spin susceptibility measurements across the interaction strength-temperature phase diagram using a novel radio frequency technique with ultracold ^{6}Li gases. For all significant interaction strengths and at all temperatures we find the spin susceptibility is reduced compared to the equivalent value for a noninteracting Fermi gas. At unitarity, we can use the local density approximation to extract the integrated spin susceptibility for the uniform gas as a function of temperature, which at high temperatures is generally less than theoretically predicted. At low temperatures, our data lie within the range of theoretical predictions, although we can also describe the entire curve using a very simple one-parameter mean field model with monotonically increasing spin susceptibility.
We theoretically investigate the uniform spin susceptibility $\ensuremath{\chi}$ in the superfluid phase of an ultracold Fermi gas in the region of the Bardeen-Cooper-Schrieffer--Bose-Einstein-condensate (BCS-BEC) crossover. In our previous paper [H. Tajima et al., Phys. Rev. A 89, 033617 (2014)], including pairing fluctuations within an extended TTT-matrix approximation (ETMA), we showed that strong pairing fluctuations cause the so-called spin-gap phenomenon, where $\ensuremath{\chi}$ is anomalously suppressed even in the normal state near the superfluid phase transition temperature Tc{T}_{\mathrm{c}}Tc​. In this paper, we extend this work to the superfluid phase below Tc{T}_{\mathrm{c}}Tc​, to clarify how this many-body phenomenon is affected by the superfluid order. From the comparison of the ETMA $\ensuremath{\chi}$ with the Yosida function describing the spin susceptibility in a weak-coupling BCS superfluid, we identify the region where pairing fluctuations crucially affect this magnetic quantity below Tc{T}_{\mathrm{c}}Tc​ in the phase diagram with respect to the strength of a pairing interaction and the temperature. This spin-gap regime is found to be consistent with the previous pseudogap regime determined from the pseudogapped density of states. We also compare our results with a recent experiment on a 6Li^{6}\mathrm{Li}6Li Fermi gas. Since the spin susceptibility is sensitive to the formation of spin-singlet preformed pairs, our results would be useful for the study of pseudogap physics in an ultracold Fermi gas on the viewpoint of the spin degrees of freedom.
We will present recent experimental work on the thermodynamics of strongly interacting Fermi gases. We have developed a general method to probe with high precision the Equation of State (EoS) of locally homogeneous ultracold gases. This allows stringent tests of recent many-body theories. First, we focus on the finite-temperature EoS of the unpolarized unitary gas. Precise thermometry is provided by adding to the Fermi gas of 6Li a trace of bosonic 7Li. We show that the low-temperature properties of the strongly interacting normal phase are well described by Fermi liquid theory and we localize the superfluid transition. Second, we address the zero-temperature EoS of the spin-polarized system in the BEC-BCS crossover. Surprisingly, despite strong interactions, the polarized phase behaves as a mixture of two ideal gases: a Fermi gas of majority atoms and a non-interacting gas of dressed quasi-particles, the Fermi polarons. We also obtain the equation of state of the superfluid state as a function of interaction strength, that we compare to Monte Carlo simulations and to the Lee-Huang-Yang corrections for low-density bosonic and fermionic superfluids.
In this paper we present an overview of radio frequency (RF) spectroscopy in the atomic Fermi superfluids. An ultimate goal is to suggest new directions in the cold gas research agenda from the condensed matter perspective.Our focus is on the experimental and theoretical literature of cold gases and photoemission spectroscopy of the cuprates particularly as it pertains to areas of overlap. This paper contains a systematic overview of the theory of RF spectroscopy, both momentum integrated and momentum resolved. We discuss the effects of traps, population imbalance, final state interactions over the entire range of temperatures and compare theory and experiment. We show that this broad range of phenomena can be accomodated within the BCS-Leggett description of BCS-BEC crossover and that this scheme also captures some of the central observations in photoemission experiments in the cuprates. In this last context, we note that the key themes which have emerged in cuprate photoemission studies involve characterization of the fermionic self energy, of the pseudogap and of the effects of superconducting coherence (in passing from above to below the superfluid transition temperature, TcT_cTc​).These issues have a counterpart in the cold Fermi gases and it would be most useful in future to use these atomic systems to address these and the more sweeping question of how to describe that anomalous superfluid phase which forms in the presence of a normal state excitation gap.
We show, using an ab initio approach based on Quantum Monte Carlo technique, that the pseudogap regime emerges in ultracold Fermi gases close to the unitary point. We locate the onset of this regime at a value of the interaction strength corresponding to (k(F)a)(-1)≈-0.05 (a-scattering length). We determine the evolution of the gap as a function of temperature and interaction strength in the Fermi gas around the unitary limit and show that our results exhibit a remarkable agreement with the recent wave-vector resolved radio frequency spectroscopy data. Our results indicate that a finite temperature structure of the Fermi gas around unitarity is more complicated and involves the presence of the phase with preformed Cooper pairs, which, however, do not contribute to the long range order.
We investigate the uniform spin susceptibility ${\ensuremath{\chi}}_{\mathrm{s}}$ in the BCS (Bardeen-Cooper-Schrieffer)-BEC (Bose-Einstein condensation) crossover regime of an ultracold Fermi gas. Including pairing fluctuations within the framework of an extended TTT-matrix approximation, we show that ${\ensuremath{\chi}}_{\mathrm{s}}$ exhibits nonmonotonic temperature dependence in the normal state. In particular, ${\ensuremath{\chi}}_{\mathrm{s}}$ is suppressed near the superfluid phase transition temperature Tc{T}_{\mathrm{c}}Tc​ due to strong pairing fluctuations. To characterize this anomalous behavior, we introduce the spin-gap temperature Ts{T}_{\mathrm{s}}Ts​ as the temperature at which ${\ensuremath{\chi}}_{\mathrm{s}}$ takes a maximum value. Determining Ts{T}_{\mathrm{s}}Ts​ in the whole BCS-BEC crossover region, we identify the spin-gap regime in the phase diagram of a Fermi gas in terms of the temperature and the strength of a pairing interaction. We also clarify how the spin-gap phenomenon is related to the pseudogap phenomenon appearing in the single-particle density of states. Our results indicate that an ultracold Fermi gas in the BCS-BEC crossover region is a very useful system to examine the pseudogap phenomenon and the spin-gap phenomenon in a unified manner.
We investigate magnetic properties of a strongly interacting ultracold Fermi gas. Within the framework of an extended T -matrix approximation, we calculate the spin susceptibility χ in the unitarity limit. We show that effects of pairing fluctuations on this magnetic quantity are quite different in between the normal state and the superfluid phase. In the normal state, pairing fluctuations cause spin-gap phenomenon near the superfluid phase transition temperature T c , where χ is anomalously suppressed. In the superfluid phase, on the other hand, the ordinary suppression of χ by the BCS energy gap is weakened by pairing fluctuations, because they induce finite density of states inside the gap. Our results indicate that the spin susceptibility is a useful quantity for the study of pairing fluctuations in the BCS-BEC crossover regime of an ultracold Fermi gas.