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arXiv:2011.04574

Response to "Comment on Universal Lindblad Equation for open quantum systems"

Frederik Nathan, Mark Spencer Rudner

Published Nov 9, 2020• 1 citation
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Abstract

In a recent comment, Lee and Yeo show that the Gibbs state is not generically an exact steady state of the Universal Lindblad Equation (ULE) that we developed in Phys. Rev. B 102, 115109 (2020). This non-controversial observation is precisely as expected for open quantum systems with finite system-bath coupling, where transition rates may be comparable to or larger than the level spacing of the system, and we made no claim to the contrary in our paper. The comment by Lee and Yeo hence highlights that the ULE captures contributions to the steady state due to finite system-bath coupling that are beyond the reach of master equations that rely on rotating wave approximations. In this response we further clarify the nature of our analytical and numerical results.

DOI
10.48550/arxiv.2011.04574

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In a recent comment, Lee and Yeo show that the Gibbs state is not generically an exact steady state of the Universal Lindblad Equation (ULE) that we developed in Phys. Rev. B 102, 115109 (2020). This non-controversial observation is precisely as expected for open quantum systems with finite system-bath coupling, where transition rates may be comparable to or larger than the level spacing of the system, and we made no claim to the contrary in our paper. The comment by Lee and Yeo hence highlights that the ULE captures contributions to the steady state due to finite system-bath coupling that are beyond the reach of master equations that rely on rotating wave approximations. In this response we further clarify the nature of our analytical and numerical results.
It is very common in the literature to write a Markovian quantum master equation in Lindblad form to describe a system with multiple degrees of freedom and weakly connected to multiple thermal baths which can, in general, be at different temperatures and chemical potentials. However, the microscopically derived quantum master equation up to leading order in a system-bath coupling is of the so-called Redfield form, which is known to not preserve complete positivity in most cases. Additional approximations to the Redfield equation are required to obtain a Lindblad form. We lay down some fundamental requirements for any further approximations to the Redfield equation, which, if violated, leads to physical inconsistencies such as inaccuracies in the leading order populations and coherences in the energy eigenbasis, violation of thermalization, and violation of local conservation laws at the nonequilibrium steady state. We argue that one or more of these conditions will generically be violated in all the weak system-bath-coupling Lindblad descriptions existing in the literature to our knowledge. As an example, we study the recently derived universal Lindblad equation and use these conditions to show the violation of local conservation laws due to inaccurate coherences but accurate populations in the energy eigenbasis. Finally, we exemplify our analytical results numerically in an interacting open quantum spin system.
Away from equilibrium, the properties of open quantum systems depend on the details of their environment. A microscopic derivation of a master equation (ME) is therefore crucial. Of particular interest are Lindblad-type equations, not only because they provide the most general class of Markovian MEs, but also since they are the starting point for efficient quantum trajectory simulations. Lindblad-type MEs are commonly derived from the Born-Markov-Redfield equation via a rotating-wave approximation (RWA). However the RWA is valid only for ultraweak system-bath coupling and often fails to accurately describe nonequilibrium processes. Here we derive an alternative Lindbladian approximation to the Redfield equation, which does not rely on ultraweak system-bath coupling. Applying it to an extended Hubbard model coupled to Ohmic baths, we show that, especially away from equilibrium, it provides a good approximation in large parameter regimes where the RWA fails.
Abstract Quantum master equations are widely used to describe the dynamics of open quantum systems. All these different master equations rely on specific approximations that may or may not be justified. Starting from a microscopic model, applying the standard Born and Markov approximations results in the Redfield equation that does not guarantee to preserve positivity. The latter is typically achieved by additionally applying the secular approximation resulting in a quantum master equation in Lindblad form. There are other ways to obtain an equation in Lindblad form, one of which is the recently proposed universal Lindblad equation (ULE). It has been shown that it is in the same equivalence class of approximations as the Redfield master equation although avoiding the heuristic secular approximation (Nathan and Rudner 2020 Phys. Rev. B 102 115109). In this work, we prove that the solutions of the master equation obtained by applying the secular approximation are also obtained by an approximation of the same order as the one performed to obtain the Redfield equation. We hereby provide a mathematical justification for the secular approximation. We show that the result of applying the secular approximation is obtained naturally by applying a self-consistency argument. This shows that the resulting master equation is also in the same equivalence class of approximations as the Redfield master equation and the ULE. We furthermore give numerical considerations about the accuracy of the secular master equation compared to the ULE.
We investigate the scaling of the fermionic logarithmic negativity (FLN) between complementary intervals in the steady state of a driven-dissipative tight-binding critical chain, coupled to two thermal reservoirs at its edges. We compare the predictions of three different master equations, namely a nonlocal Lindblad equation, the Redfield equation, and the recently proposed universal Lindblad equation (ULE). Within the nonlocal Lindblad equation approach, the FLN grows logarithmically with the subsystem size ℓ\ellℓ, for any value of the system-bath coupling and of the bath parameters. This is consistent with the logarithmic scaling of the mutual information analytically demonstrated in [Phys. Rev. B 106, 235149 (2022)]. In the ultraweak-coupling regime, the Redfield equation and the ULE exhibit the same logarithmic increase; such behavior holds even when moving to moderately weak coupling and intermediate values of ℓ\ellℓ. However, when venturing beyond this regime, the FLN crosses over to superlogarithmic scaling for both equations.
We show that steady-state expectation values predicted by the universal Lindblad equation (ULE) are accurate up to bounded corrections that scale linearly with the effective system-bath coupling $\mathrm{\ensuremath{\Gamma}}$ (second order in the microscopic coupling). We also identify a near-identity, quasilocal ``memory-dressing'' transformation, used during the derivation of the ULE, whose inverse can be applied to achieve relative deviations of observables that generically scale to zero with $\mathrm{\ensuremath{\Gamma}}$, even for nonequilibrium currents whose steady-state values themselves scale to zero with $\mathrm{\ensuremath{\Gamma}}$. This result provides a solution to recently identified limitations on the accuracy of Lindblad equations, which highlighted a potential for significant relative errors in currents of conserved quantities. The transformation we identify allows for high-fidelity computation of currents in the weak-coupling regime, ensuring thermodynamic consistency and local conservation laws, while retaining the stability and physicality of a Lindblad-form master equation.