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arXiv:2010.15536 · Physical Review A

Quantum signatures of chaos in a cavity-QED-based stimulated Raman adiabatic passage

Amit Dey

Published May 11, 2021• 2 citations
arXivHTMLPDF

Abstract

Nonlinear stimulated Raman adiabatic passage (STIRAP) is a fascinating physical process that dynamically explores chaotic and nonchaotic phases. In a recent paper [A. Dey and M. Kulkarni, Phys. Rev. Res. 2, 042004(R) (2020)], such a phenomenon is realized in a cavity-QED platform. There, the emergence of chaos and its impact on STIRAP efficiency are mainly demonstrated in the semiclassical limit. In the present paper we treat the problem in a fully quantum many-body framework. With the aim of extracting quantum signatures of a classically chaotic system, it is shown that an out-of-time-ordered correlator (OTOC) measure precisely captures chaotic and nonchaotic features of the system. The prediction by OTOC is in precise matching with classical chaos quantified by Lyapunov exponent analysis. Furthermore, it is shown that the quantum route corresponding to the semiclassical followed state encounters a dip in single-particle purity within the chaotic phase, depicting a consequence of chaos. A dynamics through the chaotic phase is associated with spreading of the many-body quantum state and an irreversible increase in the number of participating adiabatic eigenstates.

DOI
10.1103/physreva.103.053704

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Nonlinear stimulated Raman adiabatic passage (STIRAP) is a fascinating physical process that dynamically explores chaotic and nonchaotic phases. In a recent paper [A. Dey and M. Kulkarni, Phys. Rev. Res. 2, 042004(R) (2020)], such a phenomenon is realized in a cavity-QED platform. There, the emergence of chaos and its impact on STIRAP efficiency are mainly demonstrated in the semiclassical limit. In the present paper we treat the problem in a fully quantum many-body framework. With the aim of extracting quantum signatures of a classically chaotic system, it is shown that an out-of-time-ordered correlator (OTOC) measure precisely captures chaotic and nonchaotic features of the system. The prediction by OTOC is in precise matching with classical chaos quantified by Lyapunov exponent analysis. Furthermore, it is shown that the quantum route corresponding to the semiclassical followed state encounters a dip in single-particle purity within the chaotic phase, depicting a consequence of chaos. A dynamics through the chaotic phase is associated with spreading of the many-body quantum state and an irreversible increase in the number of participating adiabatic eigenstates.
We study the many-body dynamics of stimulated Raman adiabatic passage in the presence of on-site interactions. In the classical mean-field limit, explored in A. Dey et al. [Phys. Rev. Lett. 121, 250405 (2018)], interaction-induced chaos leads to the breakdown of adiabaticity under the quasistatic variation of the parameters, thus producing low-sweep-rate boundaries on efficient population transfer. We show that for the corresponding many-body system, alternative quantum pathways from the initial to the target state open up at even slower sweep rates. These quantum detours avoid the chaotic classical path and hence allow a robust and efficient population transfer.
A distinct feature of Hermitian quantum chaotic dynamics is the exponential increase of certain out-of-time-order correlation (OTOC) functions around the Ehrenfest time with a rate given by a Lyapunov exponent. Physically, the OTOCs describe the growth of quantum uncertainty that crucially depends on the nature of the quantum motion. Here, we employ the OTOC in order to provide a precise definition of dissipative quantum chaos. For this purpose, we compute analytically the Lyapunov exponent for the vectorized formulation of the large- q limit of a q -body Sachdev-Ye-Kitaev model coupled to a Markovian bath. These analytic results are confirmed by an explicit numerical calculation of the Lyapunov exponent for several values of q ≥ 4 based on the solutions of the Schwinger-Dyson and Bethe-Salpeter equations. We show that the Lyapunov exponent decreases monotonically as the coupling to the bath increases and eventually becomes negative at a critical value of the coupling signaling a transition to a dynamics which is no longer quantum chaotic. Therefore, a positive Lyapunov exponent is a defining feature of dissipative many-body quantum chaos. The observation of the breaking of the exponential growth for sufficiently strong coupling suggests that dissipative quantum chaos may require in certain cases a sufficiently weak coupling to the environment. Published by the American Physical Society 2024
In this work, we show, that relative oscillations in asymptotic times of microcanonical Out-of-Time-Order correlators (OTOCs) are suppressed by chaos with the size of the sys- tem. Therefore they can serve as an indicator of quantum chaos in quantum systems. We demonstrate this phenomenon on numerical results of the Out-of-Time-Order correlators from a model with hamiltonian based on the u(3) algebra. Firstly we prove, that this model can be used not only for the description of molecular vibrations, but also Bose- Einstein condensate. Then we employ several methods for the analysis of both quantum and classical chaos, namely spectral statistics such as Nearest Neighbour Spacing Distri- bution and Brody distribution, Inverse Participation Ratio, Poincaré sections, Lyapunov exponent, and the chaotic fraction of classical phase space. We compare these results with relative oscillations of microcanonical Out-of-Time-Order correlators and show, that their suppression corresponds with the chaoticity of the quantum system and the fraction of chaotic regions of the classical phase space. 1
We study two classes of quantum phenomena associated with classical chaos in a variety of quantum models: (i) dynamical localization and its extension and generalization to interacting few- and many-body systems and (ii) quantum exponential divergences in high-order correlators and other diagnostics of quantum chaos. Dynamical localization (DL) is a subtle phenomenon related to Anderson localization. It hinges on quantum interference and is typically destroyed in presence of interactions. DL often manifests as a failure of a driven system to heat up, violating the foundations of statistical physics. Kicked rotor (KR) is a prototypical chaotic classical model that exhibits linear energy growth with time. The quantum kicked rotor (QKR) features DL instead: its energy saturates. Multiple attempts of many-body generalizations faced difficulties in preserving DL. Recently, DL was shown in a special integrable many-body model. We study non-integrable models of few- and many-body QKR-like systems and provide direct evidence that DL can persist there. In addition, we show how a novel related concept of localization landscape can be applied to study transport in rippled channels. Out-of-time-ordered correlator (OTOC) was proposed as an indicator of quantum chaos, since in the semiclassical limit, this correlator's possible exponential growth rate (CGR) resembles the classical Lyapunov exponent (LE). We show that the CGR in QKR is related, but distinct from the LE in KR. We also show a singularity in the OTOC at the Ehrenfest time tᴱ due to a delay in the onset of quantum interference. Next, we study scaling of OTOC beyond tᴱ. We then explore how the OTOC-based approach to quantum chaos relates to the random-matrix-theoretical description by introducing an operator we dub the Lyapunovian. Its level statistics is calculated for quantum stadium billiard, a seminal model of quantum chaos, and aligns perfectly with the Wigner-Dyson surmise. In the semiclassical limit, the Lyapunovian reduces to the matrix of uncorrelated finite-time Lyapunov exponents, connecting the CGR at early times, when the quantum effects are weak, to universal level repulsion that hinges on strong quantum interference. Finally, we consider quantum polygonal billiards: their classical counterparts are non-chaotic. We show exponential growth of the OTOCs in these systems, sharply contrasted with the classical behavior even before quantum interference develops.
Quantum chaos remains a challenging concept because classical signatures of chaos do not directly transfer to quantum systems. This thesis investigates which indicators of chaos are shared between classical and quantum mechanics and how they can be used to characterise non-integrable many-body systems. We examine ergodicity and thermalisation by means of the Eigenstate Thermalisation Hypothesis (ETH) as signatures of non-integrability, and study the Out-of-Time-Ordered Correlator (OTOC) as a probe of information scrambling and as a measure of sensitivity to initial conditions. We briefly discuss the appearance of chaotic wavefunctions and observations such as quantum scars and quantum ergodicity in individual eigenmodes of the Bunimovich stadium potential. Using the OTOC, we discuss extensions of the Lyapunov exponent to quantum systems and apply these ideas to the Sachdev–Ye–Kitaev (SYK) model. In the large-N limit, and using the AdS/CFT correspondence, we find that the model might potentially be the dual of a black hole and that it is maximally chaotic. We conclude by discussing additional proposed signatures of quantum chaos and prospects for experimental realisations of the SYK model.