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arXiv:2010.09604 · Frontiers of Physics

Nonreciprocal transition between two indirectly coupled energy levels

Xun‐Wei Xu, Hai-Quan Shi, Aixi Chen

Published Dec 24, 2021• 2 citations
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Abstract

We propose a theoretical scheme to realize nonreciprocal transition between two energy levels that can not coupled directly. Suppose they are coupled indirectly by two auxiliary levels with a cyclic four-level configuration, and the four transitions in the cyclic configuration are controlled by external fields. The indirectly transition become nonreciprocal when the time reversal symmetry of the system is broken by the synthetic magnetic flux, i.e., the total phase of the external driving fields through the cyclic four-level configuration. The nonreciprocal transition can be identified by the elimination of a spectral line in the spontaneous emission spectrum. Our work introduces a feasible way to observe nonreciprocal transition in a wide range of multi-level systems, including natural atoms or ions with parity symmetry.

DOI
10.1007/s11467-021-1138-x

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We propose a theoretical scheme to realize nonreciprocal transition between two energy levels that can not coupled directly. Suppose they are coupled indirectly by two auxiliary levels with a cyclic four-level configuration, and the four transitions in the cyclic configuration are controlled by external fields. The indirectly transition become nonreciprocal when the time reversal symmetry of the system is broken by the synthetic magnetic flux, i.e., the total phase of the external driving fields through the cyclic four-level configuration. The nonreciprocal transition can be identified by the elimination of a spectral line in the spontaneous emission spectrum. Our work introduces a feasible way to observe nonreciprocal transition in a wide range of multi-level systems, including natural atoms or ions with parity symmetry.
We propose a theoretical scheme to realize nonreciprocal transition in a multi-level atomic system with cyclic four-level transition. The effective transition between two indirectly coupled energy levels become nonreciprocal, when they are coupled to two auxiliary levels simultaneously, by four strong driving fields with the total phase serving as a synthetic magnetic flux and breaking the time reversal symmetry of the system. The nonreciprocal transition can lead to the elimination of a spectral line in the spontaneous emission spectrum, which provide us a simple approach to measure the phenomenon in steady state. This work provides a feasible approach to observe nonreciprocal transition in a wide range of multi-level systems, including natural atoms with parity symmetry.
Stimulated emission and absorption are two fundamental processes of light–matter interaction, and the coefficients of the two processes should be equal. However, we will describe a generic method to realize the significant difference between the stimulated emission and absorption coefficients of two nondegenerate energy levels, which we refer to as a nonreciprocal transition. As a simple implementation, a cyclic three-level atom system, comprising two nondegenerate energy levels and one auxiliary energy level, is employed to show a nonreciprocal transition via a combination of synthetic magnetism and reservoir engineering. Moreover, a single-photon nonreciprocal transporter is proposed using two one-dimensional semi-infinite coupled-resonator waveguides connected by an atom with nonreciprocal transition effect. Our work opens up a route to design atom-mediated nonreciprocal devices in a wide range of physical systems.
The spontaneous emission spectrum of a multilevel atom or molecule with nonreciprocal transition is investigated. It is shown that the nonreciprocal transition can lead to the elimination of a spectral line in the spontaneous emission spectrum. As an application, we show that nonreciprocal transition arises from the phase-related driving fields in chiral molecules with cyclic three-level transitions, and the elimination of a spectral line induced by nonreciprocal transition provides us a method to determine the enantiomeric excess for the chiral molecules without requiring the enantio-pure samples.
A scheme for magnetic-free optical nonreciprocity in an ensemble of four-level cold atoms is proposed by exploiting the directional four-wave mixing effect. Using experimentally achievable parameters, the nonreciprocal optical responses of the system can be observed and the conversion on nonreciprocal transmission and nonreciprocal phase shift can be implemented. These nonreciprocal phenomena originate from the directional phase matching, which breaks the time-reversal symmetry and dynamic reciprocity of the cold atomic system. Moreover, by embedding the cold atoms into a Mach-Zehnder interferometer and choosing proper parameters, a two-port optical isolator with an isolation ratio of 79.70 dB and an insertion loss of 0.35 dB and a four-port optical circulator with a fidelity of 0.9985 and a photon survival probability of 0.9278 can be realized, which shows the high performance of isolation and circulation. The proposal may enable a new class of optically controllable cavity-free nonreciprocal devices in optical signal processing at the low light level.
We investigate the physics of an open two-component Dicke model, where the light field mediates nonreciprocal interactions between two spin species. We show that the model, which we dub nonreciprocal Dicke model, exhibits a discrete parity-time (PT) symmetry and we characterize the emergence of a nonstationary phase, so far explained in terms of dissipation-induced instability, as spontaneous breaking of PT symmetry. We further show that such PT symmetry breaking embodies an instance of a nonreciprocal phase transition, a concept recently introduced by Fruchart et al. [Nature (London) 592, 363 (2021)NATUAS0028-083610.1038/s41586-021-03375-9]. Remarkably, the phase transition in our model does not necessitate the presence of any underlying broken symmetry or exceptional points in the spectrum, both believed to be essential requirements for nonreciprocal phase transitions. Our results establish driven-dissipative light-matter systems as a new avenue for exploring nonreciprocal phase transitions and contribute to the theory of nonreciprocal collective phenomena.
Active agents are capable of exerting nonreciprocal forces upon one another. For instance, one agent, say A , may attract another agent B while B repels A . These antagonistic nonreciprocal interactions have been extensively studied in classical systems, revealing a wealth of exciting phenomena such as novel phase transitions and traveling-wave states. Whether these phenomena can originate in quantum many-body systems is an open issue, and proposals for their realization are lacking. In this work, we present a model of two species of quantum spins that interact in an antagonistic nonreciprocal way of the attraction-repulsion type. We propose an implementation based on two atomic ensembles coupled via chiral waveguides featuring both braided and nonbraided geometries. The spins are active due to the presence of local gain, which allows them to synchronize. In the thermodynamic limit, we show that nonreciprocal interactions result in a nonreciprocal phase transition to time-crystalline traveling-wave states, associated with spontaneous breaking of parity-time symmetry. We establish how this symmetry emerges from the microscopic quantum model. For a finite number of spins, signatures of the time-crystal phase can still be identified by inspecting equal-time or two-time correlation functions. Remarkably, continuous monitoring of the output field of the waveguides induces a quantum traveling-wave state: a time-crystalline state of a finite-size quantum system, in which parity-time symmetry is spontaneously broken. Our work lays the foundation to explore nonreciprocal interactions in active quantum matter.