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arXiv:2010.09450 · Physical Review Letters

Unraveling Two-Photon Entanglement via the Squeezing Spectrum of Light Traveling through Nanofiber-Coupled Atoms

Jakob Hinney, Adarsh S. Prasad, Sahand Mahmoodian, Klemens Hammerer, Arno Rauschenbeutel, Philipp Schneeweiß, Jürgen Volz, Max Schemmer

Published Sep 14, 2021• 2 citations
arXivHTMLPDF

Abstract

We observe that a weak guided light field transmitted through an ensemble of atoms coupled to an optical nanofiber exhibits quadrature squeezing. From the measured squeezing spectrum we gain direct access to the phase and amplitude of the energy-time entangled part of the two-photon wave function which arises from the strongly correlated transport of photons through the ensemble. For small atomic ensembles we observe a spectrum close to the line shape of the atomic transition, while sidebands are observed for sufficiently large ensembles, in agreement with our theoretical predictions. Furthermore, we vary the detuning of the probe light with respect to the atomic resonance and infer the phase of the entangled two-photon wave function. From the amplitude and the phase of the spectrum, we reconstruct the real and imaginary part of the time-domain wave function. Our characterization of the entangled two-photon component constitutes a diagnostic tool for quantum optics devices.

DOI
10.1103/physrevlett.127.123602

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We observe that a weak guided light field transmitted through an ensemble of atoms coupled to an optical nanofiber exhibits quadrature squeezing. From the measured squeezing spectrum we gain direct access to the phase and amplitude of the energy-time entangled part of the two-photon wave function which arises from the strongly correlated transport of photons through the ensemble. For small atomic ensembles we observe a spectrum close to the line shape of the atomic transition, while sidebands are observed for sufficiently large ensembles, in agreement with our theoretical predictions. Furthermore, we vary the detuning of the probe light with respect to the atomic resonance and infer the phase of the entangled two-photon wave function. From the amplitude and the phase of the spectrum, we reconstruct the real and imaginary part of the time-domain wave function. Our characterization of the entangled two-photon component constitutes a diagnostic tool for quantum optics devices.
We study the strong coupling between photons and atoms that can be achieved in an optical nanofiber geometry when the interaction is dispersive. While the Purcell enhancement factor for spontaneous emission into the guided mode does not reach the strong-coupling regime for individual atoms, one can obtain high cooperativity for ensembles of a few thousand atoms due to the tight confinement of the guided modes and constructive interference over the entire chain of trapped atoms. We calculate the dyadic Green's function, which determines the scattering of light by atoms in the presence of the fiber, and thus the phase shift and polarization rotation induced on the guided light by the trapped atoms. The Green's function is related to a full Heisenberg-Langevin treatment of the dispersive response of the quantized field to tensor polarizable atoms. We apply our formalism to quantum nondemolition (QND) measurement of the atoms via polarimetry. We study shot-noise-limited detection of atom number for atoms in a completely mixed spin state and the squeezing of projection noise for atoms in clock states. Compared with squeezing of atomic ensembles in free space, we capitalize on unique features that arise in the nanofiber geometry including anisotropy of both the intensity and polarization of the guided modes. We use a first principles stochastic master equation to model the squeezing as function of time in the presence of decoherence due to optical pumping. We find a peak metrological squeezing of ~5 dB is achievable with current technology for ~2500 atoms trapped 180 nm from the surface of a nanofiber with radius a=225 nm.
We study the strong coupling between photons and atoms that can be achieved in an optical nanofiber geometry when the interaction is dispersive. While the Purcell enhancement factor for spontaneous emission into the guided mode does not reach the strong-coupling regime for individual atoms, one can obtain high cooperativity for ensembles of a few thousand atoms due to the tight confinement of the guided modes and constructive interference over the entire chain of trapped atoms. We calculate the dyadic Green's function, which determines the scattering of light by atoms in the presence of the fiber, and thus the phase shift and polarization rotation induced on the guided light by the trapped atoms. The Green's function is related to a full Heisenberg-Langevin treatment of the dispersive response of the quantized field to tensor polarizable atoms. We apply our formalism to quantum nondemolition (QND) measurement of the atoms via polarimetry. We study shot-noise-limited detection of atom number for atoms in a completely mixed spin state and the squeezing of projection noise for atoms in clock states. Compared with squeezing of atomic ensembles in free space, we capitalize on unique features that arise in the nanofiber geometry including anisotropy of both the intensity and polarization of the guided modes. We use a first-principles stochastic master equation to model the squeezing as a function of time in the presence of decoherence due to optical pumping. We find a peak metrological squeezing of $\ensuremath{\sim}5$ dB is achievable with current technology for $\ensuremath{\sim}2500$ atoms trapped 180 nm from the surface of a nanofiber with radius a=225a=225a=225 nm.
We study two-photon scattering of a tightly focused weak light beam from a small atomic ensemble of two-level atoms (2LAs). This is similar to the scattering of photons from an atomic ensemble in a one-dimensional waveguide. The scaling of two-photon nonlinearity at single-photon resonance shows a nonmonotonic behavior with an increasing number of few identical 2LAs. The two-photon nonlinearity decays monotonically with an increasing number of atoms for incident photons detuned from single-photon resonance. Single-photon transport in two 2LAs is similar to that in a single VVV-type three-level atom (3LA). However, two-photon transport in these two systems shows very different line shapes. When single-photon transmission is zero in these systems, two transmitted photons are bunched together in a VVV-type 3LA, while their correlation is zero in two 2LAs. The difference in the two-photon line shape persists for few 2LAs and 3LAs. Therefore, the two-photon scattering of a tightly focused weak light beam can be used as a probe to detect atomic level structures of different atoms with similar transition energies.
The time-energy entanglement of down-converted photon pairs is particularly difficult to characterize because direct measurements of photon arrival times are limited by the temporal resolution of photon detection. Here, we explore an alternative possibility of characterizing the temporal coherence of two-photon wave functions using single-photon interference with weak coherent light. Specifically, this method makes use of the fact that down conversion generates a coherent superposition of vacuum and two-photon states, so that the coincidence count rates for photon pairs after interference with weak coherent light are given by a superposition of the two-photon wave function from the down conversion with the product wave function defined by the weak coherent references. By observing the frequency-dependent interference pattern, it is possible to reconstruct the amplitudes and the phases of the two-photon wave function within the bandwidth of the reference pulses used in the single-photon interferences. The correlated single-photon interferences therefore provide a direct map of the entangled two-photon wave function generated in the down-conversion process.
We experimentally and theoretically investigate collective radiative effects in an ensemble of cold atoms coupled to a single-mode optical nanofiber. Our analysis unveils the microscopic dynamics of the system, showing that collective interactions between the atoms and a single guided photon gradually build up along the atomic array in the direction of propagation of light. These results are supported by time-resolved measurements of the light transmitted and reflected by the ensemble after excitation via nanofiber-guided laser pulses, whose rise and fall times are shorter than the atomic lifetime. Superradiant decays more than 1 order of magnitude faster than the single-atom free-space decay rate are observed for emission in the forward-propagating guided mode, while at the same time, no speed-up of the decay rate is measured in the backward direction. In addition, position-resolved measurements of the light that is transmitted past the atoms are performed by inserting the nanofiber-coupled atomic array in a 45-m-long fiber ring resonator, which allow us to experimentally reveal the progressive growth of the collective response of the atomic ensemble. Our results highlight the unique opportunities offered by nanophotonic cold atom systems for the experimental investigation of collective light-matter interaction.
An exciting frontier in quantum information science is the integration of otherwise "simple" quantum elements into complex quantum networks. The laboratory realization of even small quantum networks enables the exploration of physical systems that have not heretofore existed in the natural world. Within this context, there is active research to achieve nanoscale quantum optical circuits, for which atoms are trapped near nano-scopic dielectric structures and "wired" together by photons propagating through the circuit elements. Single atoms and atomic ensembles endow quantum functionality for otherwise linear optical circuits and thereby enable the capability of building quantum networks component by component. Toward these goals, we have experimentally investigated three different systems, from conventional to rather exotic systems : free-space atomic ensembles, optical nano fibers, and photonics crystal waveguides. First, we demonstrate measurement-induced quadripartite entanglement among four quantum memories. Next, following the landmark realization of a nanofiber trap, we demonstrate the implementation of a state-insensitive, compensated nanofiber trap. Finally, we reach more exotic systems based on photonics crystal devices. Beyond conventional topologies of resonators and waveguides, new opportunities emerge from the powerful capabilities of dispersion and modal engineering in photonic crystal waveguides. We have implemented an integrated optical circuit with a photonics crystal waveguide capable of both trapping and interfacing atoms with guided photons, and have observed the collective effect, superradiance, mediated by the guided photons. These advances provide an important capability for engineered light-matter interactions, enabling explorations of novel quantum transport and quantum many-body phenomena.