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arXiv:2010.06811 · Optics Letters

Proposal for noise-free visible-telecom quantum frequency conversion through third-order sum and difference frequency generation

Xiyuan Lu, Gregory T. Moille, Ashutosh Rao, Kartik A. Srinivasan

Published Dec 7, 2020• 11 citations
arXivHTMLPDF

Abstract

Quantum frequency conversion (QFC) between the visible and telecom is a key to connect quantum memories in fiber-based quantum networks. Current methods for linking such widely separated frequencies, such as sum/difference frequency generation and four-wave mixing Bragg scattering, are prone to broadband noise generated by the pump laser(s). To address this issue, we propose to use third-order sum/difference frequency generation (TSFG/TDFG) for an upconversion/downconversion QFC interface. In this process, two long wavelength pump photons combine their energy and momentum to mediate frequency conversion across the large spectral gap between the visible and telecom bands, which is particularly beneficial from the noise perspective. We show that waveguide-coupled silicon nitride microring resonators can be designed for efficient QFC between 606 and 1550 nm via a 1990 nm pump through TSFG/TDFG. We simulate the device dispersion and coupling, and from the simulated parameters, estimate that the frequency conversion can be efficient (${\gt}80 \%$) at 50 mW pump power. Our results suggest that microresonator TSFG/TDFG is promising for compact, scalable, and low-power QFC across large spectral gaps.

DOI
10.1364/ol.412602

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Quantum frequency conversion (QFC) between the visible and telecom is a key to connect quantum memories in fiber-based quantum networks. Current methods for linking such widely separated frequencies, such as sum/difference frequency generation and four-wave mixing Bragg scattering, are prone to broadband noise generated by the pump laser(s). To address this issue, we propose to use third-order sum/difference frequency generation (TSFG/TDFG) for an upconversion/downconversion QFC interface. In this process, two long wavelength pump photons combine their energy and momentum to mediate frequency conversion across the large spectral gap between the visible and telecom bands, which is particularly beneficial from the noise perspective. We show that waveguide-coupled silicon nitride microring resonators can be designed for efficient QFC between 606 and 1550 nm via a 1990 nm pump through TSFG/TDFG. We simulate the device dispersion and coupling, and from the simulated parameters, estimate that the frequency conversion can be efficient (>80%{\gt}80 \%>80%) at 50 mW pump power. Our results suggest that microresonator TSFG/TDFG is promising for compact, scalable, and low-power QFC across large spectral gaps.
We describe a chip-scale, telecommunications-band frequency conversion interface designed for low-noise operation at wavelengths desirable for common single photon emitters. Four-wave-mixing Bragg scattering in silicon nitride waveguides is used to demonstrate frequency upconversion and downconversion between the 980 nm and 1550 nm wavelength regions, with signal-to-background levels > 10 and conversion efficiency of ≈ -60 dB at low continuous wave input pump powers (< 50 mW). Finite element simulations and the split-step Fourier method indicate that increased input powers of ≈ 10 W (produced by amplified nanosecond pulses, for example) will result in a conversion efficiency > 25 % in existing geometries. Finally, we present waveguide designs that can be used to connect shorter wavelength (637 nm to 852 nm) quantum emitters with 1550 nm.
High-efficiency quantum frequency conversion (QFC) for group-IV color centers, such as silicon vacancies (SiV), is required for long-distance quantum networking protocols. Performance of QFC depends on the choices of network and pump wavelengths and the choice between bulk crystal and waveguide, since these directly determine the dominant noise processes. These furthermore lead to fiber-based or free-space, single- or multi-pass setups with different complexities, power requirements, losses, and hence, external efficiencies. Here, we present a QFC device design for SiV QFC with simultaneous state-of-the-art performance and simple setup. Namely, by choosing the C-band pump wavelength of λ p = 1561 nm, which leads to an E-band network wavelength of λ n = 1398 nm, we remain in the anti-Stokes noise regime in a one-stage, single-pass conversion scheme. The high-quality erbium-doped fiber amplifiers in this band aid in maximizing the internal nonlinear process. We measure an external (internal) photon conversion efficiency of 44.5 ± 1.8 % (8.5 ± 1.8 %) at an external (internal) pump power of 1.51 W (0.97 W), limited by fiber coupling efficiencies. This is an increase in efficiency by 9 % (25 %) compared to prior demonstrations for SiV QFC, which were limited by factors such as internal device efficiencies, limited available pump power, and losses. We measure a pump-generated noise spectral density of 4913 counts/s/nm, which can be attributed to the anti-Stokes Raman scattering, in line with other one-stage demonstrations, though higher by an order of magnitude than that obtained in two-stage conversion. Without extra filtering, we expect this to lead to a networking photon signal-to-noise ratio of above 7000 for cavity-integrated SiVs in emission-based schemes.
Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. Practicable QFC interfaces connecting ultraviolet and telecommunication bands are of great significance but have remained elusive, constrained by the dual challenges of a high-performance frequency converter and effective noise suppression in short-wavelength pumping configurations. We address this by demonstrating the phase-matching mechanism with domain defects and differential-tuning behavior of the spontaneous parametric down-conversion noises. Based on a quantitative analysis of performance degradation induced by domain defects, we propose specific fabrication guidelines and experimentally achieve an ultrahigh normalized conversion efficiency of 839%/(W cm^{2}) for the fundamental guided mode in thin-film lithium niobate waveguides. Meanwhile, we reveal a new noise control mechanism for short-wavelength pumping by utilizing the differential-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion processes. Then a single-stage QFC from 393 nm to the telecom C band with a record-high external efficiency of 28.8% and an ultralow noise level of 35 counts per second is achieved experimentally. The proposed mechanisms would enable other QFCs with higher efficiency and lower noise, advancing the development of scalable quantum networks. Furthermore, it holds significant potential for driving progress in both classical and integrated nonlinear photonics.
We report a detailed study of the noise properties of a visible-to-telecom photon frequency converter based on difference frequency generation (DFG). The device converts 580 nm photons to 1541 nm using a strong pump laser at 930 nm, in a periodically poled lithium niobate ridge waveguide. The converter reaches a maximum device efficiency of 46 % (internal efficiency of 67%) at a pump power of 250 mW. The noise produced by the pump laser is investigated in detail by recording the noise spectra both in the telecom and visible regimes and measuring the power dependence of the noise rates. The noise spectrum in the telecom is very broadband, as expected from previous work on similar DFG converters. However, we also observe several narrow dips in the telecom spectrum, with corresponding peaks appearing in the 580 nm noise spectrum. These features are explained by sum frequency generation of the telecom noise at wavelengths given by the phase-matching condition of different spatial modes in the waveguide. The proposed noise model is in good agreement with all the measured data, including the power dependence of the noise rates, both in the visible and telecom regimes. These results are applicable to the class of DFG converters where the pump laser wavelength is in between the input and target wavelength.
Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. In this work, we demonstrate a short-wavelength-pumping QFC with the first-order quasi-phase matching period of 3.07 um on thin-film lithium niobate, converting ultraviolet photons to the telecom C-band. By constructing a theoretical model that correlates the normalized conversion efficiency with domain defects in the short-period phase-matched waveguide, we found the critical tolerance of domain defects along the waveguide should be ≤2\le 2≤2 (excluding the ends). Based on this, we achieved a theoretical limit normalized conversion efficiency of 839%/(W*cm^2) for the fundamental guided mode through fabrication optimization. Furthermore, we propose a robust noise suppression strategy for short-wavelength pumping by utilizing the counter-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion. By combining these advances with ultra-narrowband filtering, we achieve a record-high external efficiency of 28.8% and an ultra-low noise of 35 counts per second. This high-performance QFC connecting ultraviolet and telecom bands satisfies the stringent requirements for long-lived remote ion-ion entanglement in scalable quantum networks [W.-Z. Liu et al., Nature (2026)].
Quantum frequency conversion (QFC) is essential for interfacing quantum systems operating at different wavelengths and for realizing scalable quantum networks. Despite extensive progress, achieving QFC with simultaneous high efficiency, low pump power, minimal noise, broad bandwidth, and pump-wavelength flexibility remains challenging. Here, we demonstrate efficient, low-noise, and bidirectional QFC between the telecom (1550-nm) and visible (780-nm) bands using unpoled indium gallium phosphide (InGaP) χ(2)χ^{(2)}χ(2) nanophotonic waveguides, eliminating the need for a long-wavelength pump. Leveraging the large nonlinear susceptibility of InGaP together with programmable modal-phase-matching control, we obtain record-low pump power (20 mW) -- an order of magnitude lower than that in previous demonstrations using integrated thin-film waveguides -- and record-high loss-inclusive normalized conversion efficiency among non-resonant QFC implementations. The platform maintains quantum coherence and entanglement of input photons with noise well below the single-photon level. These results mark a significant advance in integrated nonlinear photonics for high-performance QFC, facilitating the development of versatile and scalable quantum networks.