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arXiv:2010.00584 · SciPost Physics Community Reports

The future of the correlated electron problem

A. Alexandradinata, N. P. Armitage, Andrey Baydin, Wenli Bi, Yue Cao, Hitesh J. Changlani, Eli Chertkov, Eduardo H. da Silva Neto, Luca V. Delacrétaz, Ismail El Baggari, Michael S. Ferguson, W. J. Gannon, Sayed Ali Akbar Ghorashi, Berit H. Goodge, Olga Goulko, G. Grissonnanche, Alannah Hallas, Ian Hayes, Yu He, Edwin W. Huang, Anshul Kogar, Divine P. Kumah, Jong Yeon Lee, Anaëlle Legros, Fahad Mahmood, Yulia Maximenko, Nick Pellatz, Hryhoriy Polshyn, Tarapada Sarkar, Allen O. Scheie, Kyle Seyler, Zhenzhong Shi, Brian J. Skinner, Lucia Steinke, K. Thirunavukkuarasu, Thaís V. Trevisan, Michael Rudolf Vogl, Pavel A. Volkov, Yao Wang, Yishu Wang, Di Wei, Kaya Wei, Shuolong Yang, Xian Zhang, Ya-Hui Zhang, Liuyan Zhao, Alfred Zong

Published Jun 25, 2025• 11 citations
arXivHTMLPDF

Abstract

A central problem in modern condensed matter physics is the understanding of materials with strong electron correlations. Despite extensive work, the essential physics of many of these systems is not understood and there is very little ability to make predictions in this class of materials. In this manuscript we share our personal views on the major open problems in the field of correlated electron systems. We discuss some possible routes to make progress in this rich and fascinating field. This manuscript is the result of the vigorous discussions and deliberations that took place at Johns Hopkins University during a three-day workshop January 27, 28, and 29, 2020 that brought together six senior scientists and 46 more junior scientists. Our hope, is that the topics we have presented will provide inspiration for others working in this field and motivation for the idea that significant progress can be made on very hard problems if we focus our collective energies.

DOI
10.21468/scipostphyscommrep.8

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In our comment we show that some of the very difficult problems have been successfully solved. We have to focus on the resolved problems, since the authors claims: Our hope, however, is that the topics we have presented will provide inspiration for others working in this field and motivation for the idea that significant progress can be made on very hard problems if we focus our collective energies. Thus, there is no need to mislead potential researchers.

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A central problem in modern condensed matter physics is the understanding of materials with strong electron correlations. Despite extensive work, the essential physics of many of these systems is not understood and there is very little ability to make predictions in this class of materials. In this manuscript we share our personal views on the major open problems in the field of correlated electron systems. We discuss some possible routes to make progress in this rich and fascinating field. This manuscript is the result of the vigorous discussions and deliberations that took place at Johns Hopkins University during a three-day workshop January 27, 28, and 29, 2020 that brought together six senior scientists and 46 more junior scientists. Our hope, is that the topics we have presented will provide inspiration for others working in this field and motivation for the idea that significant progress can be made on very hard problems if we focus our collective energies.
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The study of strongly correlated materials remains one of the most challenging and active frontiers in condensed matter physics. In these systems, the intricate interplay between electrons' kinetic energy and their mutual Coulomb repulsion gives rise to a plethora of exotic phenomena, from high-temperature superconductivity to giant magnetoresistance, which cannot be explained by conventional one-electron theories. This necessitates the development and application of advanced theoretical and computational methods capable of capturing the essential physics of strong electronic correlations. A diverse array of numerical and analytical techniques has been developed to tackle the many-body problem. However, no single method serves as a panacea; each comes with its own set of strengths and weaknesses, and their domains of applicability vary significantly. The choice of an appropriate approximation is therefore highly dependent on the specific physical system and the scientific question at hand. Different problems may benefit from different, and sometimes complementary, methodological perspectives. This thesis focuses primarily on the application and development of local or quasi-local approaches. The rationale for this focus is rooted in the physical reality of many key correlated materials, such as transition metal oxides, heavy-fermion systems or molecular solids like alkali-doped fullerenes, where the local on-site electronic interaction is the dominant energy scale. By prioritizing the accurate treatment of local physics, these methods provide a robust and computationally efficient approximation for understanding a wide range of material properties. Recent experimental and theoretical advancements—spanning the rich physics of multiorbital compounds, the precise control over interactions in ultracold atomic gases, and the complex interplay in electron-phonon coupled systems—have created an urgent need for theoretical frameworks that can deliver reliable and rapid insights. The methods explored in this work are meant to address these challenges, offering a balance between accuracy and computational feasibility. Given the variety of topics addressed, from methodological developments to their application in diverse physical contexts, this thesis will try to be as detailed and self-contained as necessary, providing a clear exposition of the underlying concepts and technical aspects.
Discoveries in quantum materials, which are characterized by the strongly quantum-mechanical nature of electrons and atoms, have revealed exotic properties that arise from correlations. It is the promise of quantum materials for quantum information science superimposed with the potential of new computational quantum algorithms to discover new quantum materials that inspires this Review. We anticipate that quantum materials to be discovered and developed in the next years will transform the areas of quantum information processing including communication, storage, and computing. Simultaneously, efforts toward developing new quantum algorithmic approaches for quantum simulation and advanced calculation methods for many-body quantum systems enable major advances toward functional quantum materials and their deployment. The advent of quantum computing brings new possibilities for eliminating the exponential complexity that has stymied simulation of correlated quantum systems on high-performance classical computers. Here, we review new algorithms and computational approaches to predict and understand the behavior of correlated quantum matter. The strongly interdisciplinary nature of the topics covered necessitates a common language to integrate ideas from these fields. We aim to provide this common language while weaving together fields across electronic structure theory, quantum electrodynamics, algorithm design, and open quantum systems. Our Review is timely in presenting the state-of-the-art in the field toward algorithms with nonexponential complexity for correlated quantum matter with applications in grand-challenge problems. Looking to the future, at the intersection of quantum information science and algorithms for correlated quantum matter, we envision seminal advances in predicting many-body quantum states and describing excitonic quantum matter and large-scale entangled states, a better understanding of high-temperature superconductivity, and quantifying open quantum system dynamics.
The discovery of high-Tc superconductivity in cuprates in 1986 moved strongly correlated systems from exotic worlds interesting only for pure theorists to the focus of solid-state research. In recent decades, the majority of hot topics in condensed matter physics (high-Tc superconductivity, colossal magnetoresistance, multiferroicity, ferromagnetism in diluted magnetic semiconductors, etc.) have been related to strongly correlated transition metal compounds. The highly successful electronic structure calculations based on density functional theory lose their predictive power when applied to such compounds. It is necessary to go beyond the mean field approximation and use the many-body theory. The methods and models that were developed for the description of strongly correlated systems are reviewed together with the examples of response function calculations that are needed for the interpretation of experimental information (inelastic neutron scattering, optical conductivity, resonant inelastic X-ray scattering, electron energy loss spectroscopy, angle-resolved photoemission, electron spin resonance, and magnetic and magnetoelectric properties). The peculiarities of (quasi-) 0-, 1-, 2-, and 3- dimensional systems are discussed.
Quantum many-body theory as a discipline in its own right dates largely from the 1950's. It has developed since then to its current position as one of the cornerstones of modern theoretical physics. The field remains vibrant and active, vigorous and exciting. Indeed, its successes and importance were vividly illustrated prior to the conference by the sharing of the 1998 Nobel Prizes in both Physics and Chemistry by three many-body theorists. Two of those Nobel laureates, Walter Kohn and Bob Laughlin, delivered invited lectures at this meeting, the tenth in the series of International Conferences on Recent Progress in Many-Body Theories. This series is universally recognized as being the premier series of meetings on this subject, and its proceedings have always summarized the current state of the art through the lectures of its leading practitioners. The present volume is no exception. A major aim of this conference series has been to foster the exchange of ideas between physicists working in all the diverse fields of application of quantum many-body theory. These include nuclear and subnuclear physics, quantum fluids, strongly correlated electronic systems, and low-dimensional condensed-matter systems and materials. All of these fields and others are represented in the present volume. Other topical themes covered include density functional theory and its applications to nuclear and electronic systems, quantum dots and chaos, and trapped Bose?Einstein condensates. Through this breadth of applications the reader will get a clear illustration of the power of the tools of modern microscopic quantum many-body theory, and their usefulness both in achieving a commonality of approach and understanding, and in transferring powerful ideas from one field to another.