Abstract An ensemble of excited atoms can synchronize emission of light collectively in a process known as superradiance when its characteristic size is smaller than the wavelength of emitted photons. The underlying superradiance depends strongly on electromagnetic (photon) fields surrounding the atomic ensemble. High mode densities of microwave photons from 300 K blackbody radiation (BBR) significantly enhance decay rates of Rydberg states to neighbouring states, enabling superradiance that is not possible with bare vacuum induced spontaneous decay. Here we report observations of the superradiance of ultracold Rydberg atoms embedded in a bath of room-temperature photons. The temporal evolution of the Rydberg | nD ⟩ to |( n + 1) P ⟩ superradiant decay of Cs atoms ( n the principal quantum number) is measured directly in free space. Theoretical simulations confirm the BBR enhanced superradiance in large Rydberg ensembles. We demonstrate that the van der Waals interactions between Rydberg atoms change the superradiant dynamics and modify the scaling of the superradiance. In the presence of static electric fields, we find that the superradiance becomes slow, potentially due to many-body interaction induced dephasing. Our study provides insights into many-body dynamics of interacting atoms coupled to thermal BBR, and might open a route to the design of blackbody thermometry at microwave frequencies via collective, dissipative photon-atom interactions.
Abstract An ensemble of excited atoms can synchronize emission of light collectively in a process known as superradiance when its characteristic size is smaller than the wavelength of emitted photons. The underlying superradiance depends strongly on electromagnetic (photon) fields surrounding the atomic ensemble. High mode densities of microwave photons from 300 K blackbody radiation (BBR) significantly enhance decay rates of Rydberg states to neighbouring states, enabling superradiance that is not possible with bare vacuum induced spontaneous decay. Here we report observations of the superradiance of ultracold Rydberg atoms embedded in a bath of room-temperature photons. The temporal evolution of the Rydberg | nD ⟩ to |( n + 1) P ⟩ superradiant decay of Cs atoms ( n the principal quantum number) is measured directly in free space. Theoretical simulations confirm the BBR enhanced superradiance in large Rydberg ensembles. We demonstrate that the van der Waals interactions between Rydberg atoms change the superradiant dynamics and modify the scaling of the superradiance. In the presence of static electric fields, we find that the superradiance becomes slow, potentially due to many-body interaction induced dephasing. Our study provides insights into many-body dynamics of interacting atoms coupled to thermal BBR, and might open a route to the design of blackbody thermometry at microwave frequencies via collective, dissipative photon-atom interactions.
Atoms excited to electronically high-lying Rydberg states decay to low-energy states through spontaneous emission processes. We investigate the impact of a static electric field on the superradiant emission process between Rydberg |60 D 5/2 〉 and |61 P 3/2 〉 states in an ultracold Cesium Rydberg atom ensemble. We report experimental observations of a significant slowdown in superradiance upon applying an electric field. To understand the slowing down of superradiance, we employ a master equation in which Stark effects and collective decay are taken into account. We solve the master equation with the discrete truncated Wigner approximation (DTWA) method. Our numerical simulations demonstrate that superradiance decoherence is caused by the Stark shifts of the Rydberg level. Our theoretical simulations qualitatively match the experimental observations. Our work provides new insights into controlling quantum critical behaviors, with implications for quantum many-body dynamics, and the study of quantum phase transitions.
We investigate Rydberg |65D5/2〉 → |66P3/2〉 superradiance in dense ultracold cesium atoms, where the ground atoms are excited to |65D5/2〉 Rydberg states via two-photon excitation in a standard magneto-optical trap. The superradiant spectrum of |65D5/2〉 → |66P3/2〉 is obtained using the state-selective field ionization technique. We observe its dynamic evolution process by varying the delay time of ionization field t d. The results show that the evolution process of |65D5/2〉 → |66P3/2〉 is much shorter than its radiation lifetime at room temperature, which verifies the superradiance effect. The dependence of the superradiance process on Rydberg atoms number N e and principal quantum number n is investigated. The results show that the superradiance becomes faster with increasing N e, while it is suppressed for stronger van der Waals (vdW) interactions. Superradiance has potential applications in quantum technologies, and the Rydberg atom is an ideal medium for superradiance. Our system is effective for studying the strong two-body interaction between Rydberg atoms.
When atoms are excited to high-lying Rydberg states they interact strongly with dipolar forces. The resulting state-dependent level shifts allow us to study many-body systems displaying intriguing nonequilibrium phenomena, such as constrained spin systems, and are at the heart of numerous technological applications, e.g., in quantum simulation and computation platforms. Here, we show that these interactions also have a significant impact on dissipative effects caused by the inevitable coupling of Rydberg atoms to the surrounding electromagnetic field. We demonstrate that their presence modifies the frequency of the photons emitted from the Rydberg atoms, making it dependent on the local neighborhood of the emitting atom. Interactions among Rydberg atoms thus turn spontaneous emission into a many-body process which manifests, in a thermodynamically consistent Markovian setting, in the emergence of collective jump operators in the quantum master equation governing the dynamics. We discuss how this collective dissipation-stemming from a mechanism different from the much studied superradiance and subradiance-accelerates decoherence and affects dissipative phase transitions in Rydberg ensembles.
Rydberg states of alkali-metal atoms are highly sensitive to electromagnetic radiation in the GHz-to-THz regime because their transitions have large electric dipole moments. Consequently, environmental blackbody radiation (BBR) can couple Rydberg states together at µ s timescales. Here, we track the BBR-induced transfer of a prepared Rydberg state to its neighbors and use the evolution of these state populations to characterize the BBR field at the relevant wavelengths, primarily at 130 GHz. We use selective field ionization readout of Rydberg states with principal quantum number n ∼ 30 in Rb 85 and substantiate our ionization signal with a theoretical model. With this detection method, we measure the associated blackbody-radiation-induced time dynamics of these states, reproduce the results with a simple semiclassical population transfer model, and demonstrate that this measurement is temperature sensitive with a statistical sensitivity to the fractional temperature uncertainty of 0.09 Hz − 1 / 2 , corresponding to 26 K Hz − 1 / 2 at room temperature. This represents a calibration-free SI-traceable temperature measurement, for which we calculate a systematic fractional temperature uncertainty of 0.006, corresponding to 2 K at room temperature when used as a primary temperature standard.
Abstract We present a first-principles density-matrix simulation of blackbody-radiation (BBR)-induced decoherence in cesium Rydberg electromagnetically induced transparency (EIT). The model incorporates spontaneous emission, blackbody-stimulated transitions, collisional broadening, transit-time-limited decoherence, and Doppler averaging across a truncated but converged Rydberg manifold within a Lindblad masterequation framework. From the steady-state solution, we extract both the temperaturedependent Rydberg coherence decay rate and the corresponding probe absorption coefficient.We show that the experimentally observed modification of probe transmission reported by Kaur et al. (2026) arises predominantly from BBR-induced decoherence of the Rydberg coherence, rather than from population redistribution among Rydberg levels. The model reproduces the observed temperature-dependent trends in probe absorption with quantitative accuracy. By employing a fully m j -resolved transition network, we establish a direct connection between microscopic decoherence processes and macroscopic optical observables. The decoherence effect on the optical response is sufficiently well-defined to serve as a measurable signal, enabling potential applications in Rydberg-based thermometry and radiometry.These results provide a self-consistent microscopic description of BBR-limited performance in thermal-vapor Rydberg EIT and establish a quantitative link between Rydberg-state decoherence and measurable changes in optical susceptibility, with direct relevance to RF-based sensing platforms.
We have observed the evolution of cold Rydberg gases and ultracold plasmas in an environment that allows for the control of interactions of the blackbody radiation temperature from 4K to 300K. The work in this thesis describes the influence of initial densities, populations, excitation state, evolution time and thermal background temperature on the evolution of cold Rydberg gases as well as directly excited ultracold plasmas. With some initial ionization, cold-Rydberg-atom gases easily develop a positive space charge that traps electrons for times on the order of tens of mus. This acts as a catalyst for electron-Rydberg atom collisions, increasing the collision probabilities by orders of magnitude and profoundly altering the final state of the Rydberg gas. Using state-selective field ionization, we have provided direct proof that these collisions cause changes in l-states, and we have seen the first experimental evidence that they also lead to inelastic n-changing collisions, as predicted by theory. We have also found evidence for Rydberg-Rydberg collisions, enabled by the attractive electric-dipole forces between atoms in high-l states and possibly by van-der-Waal's interactions at very high-n . Thermal interactions are seen to influence the formation of a plasma from a cold Rydberg gas. Plasmas form more easily in the presence of a 300K radiation field than at 4K, due to the contribution of thermal ionization to the plasma formation. The background temperature also appears to affect the electron temperature in both the directly excited plasma and the plasma spontaneously formed from a cold Rydberg gas. In Rydberg atom gases that have undergone partial ionization, electron temperatures were estimated using the dependence of n-changing collisions on the electron temperature.