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arXiv:2009.11908 · Physical Review Letters

Hydrodynamic Stabilization of Self-Organized Criticality in a Driven Rydberg Gas

Kai Klocke, T. M. Wintermantel, G. Lochead, S. Whitlock, Michael Buchhold

Published Mar 23, 2021• 17 citations
arXivHTMLPDF

Abstract

Signatures of self-organized criticality (SOC) have recently been observed in an ultracold atomic gas under continuous laser excitation to strongly interacting Rydberg states [S. Helmrich et al., Nature, 577, 481-486 (2020)]. This creates unique possibilities to study this intriguing dynamical phenomenon under controlled experimental conditions. Here we theoretically and experimentally examine the self-organizing dynamics of a driven ultracold gas and identify an unanticipated feedback mechanism originating from the interaction of the system with a thermal reservoir. Transport of particles from the flanks of the cloud toward the center compensates avalanche-induced atom loss. This mechanism sustains an extended critical region in the trap center for timescales much longer than the initial self-organization dynamics. The characteristic flattop density profile provides an additional experimental signature for SOC while simultaneously enabling studies of SOC under almost homogeneous conditions. We present a hydrodynamic description for the reorganization of the atom density, which very accurately describes the experimentally observed features on intermediate and long timescales, and which is applicable to both collisional hydrodynamic and chaotic ballistic regimes.

DOI
10.1103/physrevlett.126.123401

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Signatures of self-organized criticality (SOC) have recently been observed in an ultracold atomic gas under continuous laser excitation to strongly interacting Rydberg states [S. Helmrich et al., Nature, 577, 481-486 (2020)]. This creates unique possibilities to study this intriguing dynamical phenomenon under controlled experimental conditions. Here we theoretically and experimentally examine the self-organizing dynamics of a driven ultracold gas and identify an unanticipated feedback mechanism originating from the interaction of the system with a thermal reservoir. Transport of particles from the flanks of the cloud toward the center compensates avalanche-induced atom loss. This mechanism sustains an extended critical region in the trap center for timescales much longer than the initial self-organization dynamics. The characteristic flattop density profile provides an additional experimental signature for SOC while simultaneously enabling studies of SOC under almost homogeneous conditions. We present a hydrodynamic description for the reorganization of the atom density, which very accurately describes the experimentally observed features on intermediate and long timescales, and which is applicable to both collisional hydrodynamic and chaotic ballistic regimes.
From financial markets and neuronal activity in the brain to the way forest fires and diseases spread, the dynamics of complex systems are governed by critical events and emergent phenomena that are exceedingly difficult to understand or predict from underlying principles. We recently discovered that a gas of ultracold atoms continuously driven to strongly-interacting Rydberg states by an off-resonant laser field displays all the hallmarks of complex systems dynamics in a highly-controllable experimental system: (i) At early times we observe rapid growth of Rydberg excitations that has a striking correspondence with the spreading of diseases empirically observed in epidemics [1]; (ii) At later times we find that the system evolves toward a self-organised critical (SOC) state [2], a phenomenon that has been conjectured to explain the abundance of scale-invariant systems found in nature. I will discuss how these experiments can be understood in terms of an emergent atomic network that bridges the gap between mathematical models and empirical observations. This provides the opportunity to identify general principles governing non-equilibrium dynamics and to learn how seemingly universal properties emerge from microscopic physical details. References: [1] T. M. Wintermantel et al., Epidemic growth and Griffiths effects on an emergent network of excited atoms. Nature Communications 12, 103 (2021) [2] S. Helmrich et al., Signatures of self-organized criticality in an ultracold atomic gas. Nature 577, 481-486 (2020)
Recent experiments with strongly interacting, driven Rydberg ensembles have introduced a promising setup for the study of self-organized criticality (SOC) in cold atom systems. Based on this setup, we theoretically propose a control mechanism for the paradigmatic avalanche dynamics of SOC in the form of a time-dependent drive amplitude. This gives access to a variety of avalanche dominated, self-organization scenarios, prominently including self-organized criticality, as well as sub- and supercritical dynamics. We analyze the dependence of the dynamics on external scales and spatial dimensionality. It demonstrates the potential of driven Rydberg systems as a playground for the exploration of an extended SOC phenomenology and their relation to other common scenarios of SOC, such as, e.g., in neural networks and on graphs.
Spontaneous avalanche to plasma begins in the core of an ellipsoidal Rydberg gas of nitric oxide. Ambipolar expansion of NO +^++ draws energy from avalanche-heated electrons. Then, cycles of long-range resonant electron transfer from Rydberg molecules to ions equalize their relative velocities. This sequence of steps gives rise to a remarkable mechanics of self-assembly, in which the kinetic energy of initially formed hot electrons and ions drives an observed separation of plasma volumes. These dynamics adiabatically sequester energy in a reservoir of mass transport, starting a process that anneals separating volumes to form an apparent glass of strongly coupled ions and electrons. Short-time electron spectroscopy provides experimental evidence for complete ionization. The long lifetime of this system, particularly its stability with respect to recombination and neutral dissociation, suggests that this transformation affords a robust state of arrested relaxation, far from thermal equilibrium. We see this most directly in the excitation spectrum of transitions to states in the initially selected Rydberg series, detected as the long-lived signal that survives a flight time of 500 μ500\ \mathrm {\mu }500 μ s to reach an imaging detector. The initial density of electrons produced by prompt Penning ionization, which varies with the selected initial principal quantum number and density of the Rydberg gas, determines a balance between the rising density of ions and the falling density of Rydberg molecules. This Penning-regulated ion-Rydberg molecule balance appears necessary as a critical factor in achieving the long ultracold plasma lifetime to produce spectral features detected after very long delays.
Far-from-equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics but also in life, earth, and social sciences.However, it is challenging to find systems with sufficiently controllable parameters that allow quantitatively modeling of emergent properties.Here, we study a nonequilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapor of atoms optically excited to strongly interacting Rydberg states.Electromagnetically induced transparency provides excellent control over the population dynamics and enables highresolution probing of the driven-dissipative dynamics, which also exhibits phase bistability.Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram, including in the vicinity of the critical point.We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population.This case limits the application of generic mean-field models; however, a modified, threshold-dependent approach is in qualitative agreement with experimental data.Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.
Abstract Far-from equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics, but also in life-, earth-, and social sciences. It is challenging however to find systems with sufficiently controllable parameters that allow quantitatively modelling of emergent properties. Here, we study a non-equilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapour of atoms optically excited to strongly interacting Rydberg states. Electromagnetically induced transparency (EIT) provides excellent control over the population dynamics and enables high-resolution probing of the driven-dissipative dynamics, which also exhibits phase bistability. Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram including in the vicinity of the critical point. We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population. This limits the application of generic mean-field models, however a modified, threshold-dependent approach is in qualitative agreement with experimental data. Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.
We report the sudden and spontaneous evolution of an initially correlated gas of repulsively interacting Rydberg atoms to an ultracold plasma. Under continuous laser coupling we create a Rydberg ensemble in the strong blockade regime, which at longer times undergoes an ionization avalanche. By combining optical imaging and ion detection, we access the full information on the dynamical evolution of the system, including the rapid increase in the number of ions and a sudden depletion of the Rydberg and ground state densities. Rydberg-Rydberg interactions are observed to strongly affect the dynamics of plasma formation. Using a coupled rate-equation model to describe our data, we extract the average energy of electrons trapped in the plasma, and an effective cross section for ionizing collisions between Rydberg atoms and atoms in low-lying states. Our results suggest that the initial correlations of the Rydberg ensemble should persist through the avalanche. This would provide the means to overcome disorder-induced heating, and offer a route to enter new strongly coupled regimes.