Quantum spin liquids provide paradigmatic examples of highly entangled quantum states of matter. Frustration is the key mechanism to favor spin liquids over more conventional magnetically ordered states. Here we propose to engineer frustration by exploiting the coupling of quantum magnets to the quantized light of an optical cavity. The interplay between the quantum fluctuations of the electro-magnetic field and the strongly correlated electrons results in a tunable long-range interaction between localized spins. This cavity-induced frustration robustly stabilizes spin liquid states, which occupy an extensive region in the phase diagram spanned by the range and strength of the tailored interaction. This occurs even in originally unfrustrated systems, as we showcase for the Heisenberg model on the square lattice.
Quantum spin liquids provide paradigmatic examples of highly entangled quantum states of matter. Frustration is the key mechanism to favor spin liquids over more conventional magnetically ordered states. Here we propose to engineer frustration by exploiting the coupling of quantum magnets to the quantized light of an optical cavity. The interplay between the quantum fluctuations of the electro-magnetic field and the strongly correlated electrons results in a tunable long-range interaction between localized spins. This cavity-induced frustration robustly stabilizes spin liquid states, which occupy an extensive region in the phase diagram spanned by the range and strength of the tailored interaction. This occurs even in originally unfrustrated systems, as we showcase for the Heisenberg model on the square lattice.
Topological phases in frustrated quantum magnetic systems have captivated researchers for decades, with the chiral spin liquid (CSL) standing out as one of the most compelling examples. Featuring long-range entanglement, topological order, and exotic fractional excitations, the CSL has inspired extensive exploration for practical realizations. In this Letter, we demonstrate that CSLs can emerge in a kagome lattice driven by vacuum quantum fluctuations over the noninteracting vacuum within a single-mode gyrotropic cavity. The gyrotropic cavity imprints quantum fluctuations with time-reversal symmetry breaking and stabilizes a robust CSL phase without external laser excitation. Moreover, we identify experimentally accessible observables-such as average photon number and transport properties-that reveal connections between photon dynamics and the emergent chiral order. Our findings establish a novel pathway for creating, controlling, and probing topological and symmetry-breaking quantum phases in strongly correlated systems.
Quantum systems inside high-Q cavities offer an excellent testbed for the control of emergent symmetries induced by light and their interplay with quantum matter. Recently several developments in cavity experiments with neutral atoms and other quantum objects such as ions motivate the study of their quantum correlated properties and their entanglement to tailor and control the behavior of the system. Using the enhanced coupling between light and interacting matter we explore the properties of emergent superradiant modes using our newly developed Light-Matter DMRG algorithm with strongly interacting spin chains. We explore a experimentally viable generalization of the transverse Ising chain coupled to the cavity light where it is possible to induce multimode structures tailored by the light pumped into the system. We find a plethora of scenarios can be explored with clear and accesible measurable signatures. This allows to study the physics of emergent orders and strong quantum correlations with quantum spins where the local and long range coupling can be efficiently simulated. We find that quantum spin nematic states with long range order and magnon pairs emerge as the transitions to superradiant phases take place. Notably, we show the cavity field allows the optimization of entanglement between spins for different light induced modes which can be used for quantum state engineering of quantum correlated states. Our methods can be used to model other hybrid quantum systems efficiently.
When sizable quantum fluctuations and strong frustration mechanisms act in concert to repel the formation of conventional long-range order in quantum magnets, they can make way for massively entangled spin liquid phases which may imbue the material with extraordinary properties. \nThe search for such curious phases of matter has proceeded for several decades, gaining extra momentum some fifteen years ago when Kitaev proposed an analytically solvable model for a quantum spin liquid with anyonic excitations on the basis of realistic microscopic spin exchange terms [Kitaev, Annals of Physics 321, 2 (2006)]. Attempts to identify different models or materials which harbor quantum spin liquid ground states have kept researchers -- experimentalists and theorists alike -- in suspense ever since. However, the simulation of quantum many-body systems poses a serious challenge even to modern numerical techniques, particularly in the case of frustrated quantum magnetism in three spatial dimensions. Such models evade tractability by many established approaches, leaving a methodological void. \n \nIn this thesis, we report on recent progress in cutting-edge implementations of the pseudo-fermion functional renormalization group (pf-FRG), which has originally been proposed by Reuther and Wölfle in the context of two-dimensional frustrated quantum magnetism with highly symmetric spin interactions [Reuther and Wölfle, Phys. Rev. B 81, 144410 (2010)]. Reflecting the growing interest in models with SU(2) symmetry-breaking spin exchange terms that has followed the unearthing of Kitaev's honeycomb model, we present a generalized implementation of the pf-FRG which is suited to numerically simulate arbitrary microscopic models with diagonal or off-diagonal two-spin interactions, even in three-dimensional frustrated quantum magnets. We provide insight into the inner workings of the method which has emerged over the course of the last couple of years, arguing that the pf-FRG formalism simultaneously combines aspects of a large-S expansion as well as a large-N expansion on equal footing, thus being able to resolve the subtle interplay between magnetic ordering tendencies and disruptive quantum fluctuations. \n \nMoreover, on a case by case basis we explore the stability of quantum spin liquids in paradigmatic models of frustrated quantum magnetism and elucidate the joint action of geometric frustration, exchange frustration, and quantum fluctuations to inhibit the formation of magnetic long-range order. Examples include: (i) a Heisenberg spin model on the three-dimensional diamond lattice where geometric frustration arises from antiferromagnetic next-nearest neighbor interactions. The additional competition with nearest neighbor interactions leads to an unusually large ground state degeneracy already on classical level. The quantum-to-classical transition is studied by systematically varying the spin length and the different roles of quantum fluctuations and thermal fluctuations are discussed. The theory is applied to interpret experiments on the spin-liquid candidate NiRh2O4; (ii) a Heisenberg antiferromagnet on the face centered cubic lattice which is augmented by competing bond-directional interactions, evolving around the concurrent manifestation of geometric frustration and exchange frustration. A situation is identified where both mechanisms collude to give rise to an unusually large degree of frustration over a wide parameter regime. We discuss related experimental findings on the highly frustrated iridate compound Ba2CeIrO6; (iii) a Heisenberg antiferromagnet on the kagome lattice with additional Dzyaloshinskii-Moriya interactions. The robustness of the unperturbed kagome antiferromagnet's spin liquid ground state against low-symmetry Dzyaloshinskii-Moriya interactions is investigated. Implications for the spin-liquid candidate herbertsmithite are discussed.
Quantum matter at ultra-low temperatures offers a testbed for analysing and controlling desired properties in strongly correlated systems. Under typical conditions the nature of the atoms fixes the magnetic character the system can have. Beyond classical light potentials leading to optical lattices and short range interactions, high-Q cavities introduce novel dynamics into the system via the quantumness of light. Here we propose a theoretical model and we analyse via numerically exact simulations, the effect of cavity mediated long range magnetic interactions and optical lattices in ultracold matter. We find that global interactions allow to modify the underlying magnetic character of the system while introducing competition scenarios. Antiferromagnetic correlated bosonic matter emerges, in conditions beyond to what nature typically provides. This allows new alternatives towards the design of robust mechanisms for quantum information purposes, exploiting the properties of magnetic phases of strongly correlated quantum matter.
Quantum matter at ultralow temperatures offers a test bed for analyzing and controlling desired properties in strongly correlated systems. Under typical conditions the nature of the atoms fixes the magnetic character of the system. Beyond classical light potentials leading to optical lattices and short-range interactions, high-Q cavities introduce novel dynamics into the system via the quantumness of light. Here we propose a theoretical model and we analyze it using exact diagonalization and density matrix renormalization group simulations. We explore the effects of cavity mediated long-range magnetic interactions and optical lattices in ultracold matter. We find that global interactions modify the underlying magnetic character of the system while introducing competition scenarios. Antiferromagnetic correlated bosonic matter emerges in conditions beyond what nature typically provides. These allow new alternatives toward the design of robust mechanisms for quantum information purposes, exploiting the properties of magnetic phases of strongly correlated quantum matter.
Quantum spin liquids may be considered 'quantum disordered' ground states of spin systems, in which zero-point fluctuations are so strong that they prevent conventional magnetic long-range order. More interestingly, quantum spin liquids are prototypical examples of ground states with massive many-body entanglement, which is of a degree sufficient to render these states distinct phases of matter. Their highly entangled nature imbues quantum spin liquids with unique physical aspects, such as non-local excitations, topological properties, and more. In this review, we discuss the nature of such phases and their properties based on paradigmatic models and general arguments, and introduce theoretical technology such as gauge theory and partons, which are conveniently used in the study of quantum spin liquids. An overview is given of the different types of quantum spin liquids and the models and theories used to describe them. We also provide a guide to the current status of experiments in relation to study quantum spin liquids, and to the diverse probes used therein.