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arXiv:2009.10946 · Nature Communications

A quantum heat engine driven by atomic collisions

Quentin Bouton, Jens Nettersheim, Sabrina Burgardt, Daniel Adam, Eric Lutz, Artur Widera

Published Apr 6, 2021• 163 citations
arXivHTMLPDF

Abstract

Quantum heat engines are subjected to quantum fluctuations related to their discrete energy spectra. Such fluctuations question the reliable operation of thermal machines in the quantum regime. Here, we realize an endoreversible quantum Otto cycle in the large quasi-spin states of Cesium impurities immersed in an ultracold Rubidium bath. Endoreversible machines are internally reversible and irreversible losses only occur via thermal contact. We employ quantum control to regulate the direction of heat transfer that occurs via inelastic spin-exchange collisions. We further use full-counting statistics of individual atoms to monitor quantized heat exchange between engine and bath at the level of single quanta, and additionally evaluate average and variance of the power output. We optimize the performance as well as the stability of the quantum heat engine, achieving high efficiency, large power output and small power output fluctuations.

DOI
10.1038/s41467-021-22222-z

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arXiv:1803.06021•Physical Review Letters•Dec 9, 2019•374 citations
Quantum heat engines are subjected to quantum fluctuations related to their discrete energy spectra. Such fluctuations question the reliable operation of thermal machines in the quantum regime. Here, we realize an endoreversible quantum Otto cycle in the large quasi-spin states of Cesium impurities immersed in an ultracold Rubidium bath. Endoreversible machines are internally reversible and irreversible losses only occur via thermal contact. We employ quantum control to regulate the direction of heat transfer that occurs via inelastic spin-exchange collisions. We further use full-counting statistics of individual atoms to monitor quantized heat exchange between engine and bath at the level of single quanta, and additionally evaluate average and variance of the power output. We optimize the performance as well as the stability of the quantum heat engine, achieving high efficiency, large power output and small power output fluctuations.
Quantum heat engines are subjected to quantum fluctuations related to their discrete energy spectra. Such fluctuations question the reliable operation of thermal machines in the quantum regime. Here, we realize an endoreversible quantum Otto cycle in the large quasi-spin states of Cesium impurities immersed in an ultracold Rubidium bath. Endoreversible machines are internally reversible and irreversible losses only occur via thermal contact. We employ quantum control to regulate the direction of heat transfer that occurs via inelastic spin-exchange collisions. We further use full-counting statistics of individual atoms to monitor quantized heat exchange between engine and bath at the level of single quanta, and additionally evaluate average and variance of the power output. We optimize the performance as well as the stability of the quantum heat engine, achieving high efficiency, large power output and small power output fluctuations.
Heat engines usually operate by exchanging heat with thermal baths at different (positive) temperatures. Nonthermal baths may, however, lead to a significant performance boost. We here experimentally analyze the power output of a single-atom quantum Otto engine realized in the quasi-spin states of individual Cesium atoms interacting with an atomic Rubidium bath. From measured time-resolved populations of the quasi-spin state, we determine the dynamics during the cycle of both the effective spin temperature and of the quantum fluctuations of the engine, which we quantify with the help of the Shannon entropy. We find that power is enhanced in the negative temperature regime, and that it reaches its maximum value at half the maximum entropy. Quantitatively, operating our engine at negative effective temperatures increases the power by up to 30% compared to operation at positive temperatures, including even the case of infinite temperature. At the same time, entering the negative temperature regime allows for reducing the entropy to values close to zero, offering highly stable operation at high power output. We furthermore numerically investigate the influence of the size of the Hilbert space on the performance of the quantum engine by varying the number of levels of the working medium. Our work thereby paves the way to fluctuation control in the operation of high-power and efficient single-atom quantum engines.
The non-equilibrium properties of open quantum systems are determined by the microscopic laws governing energy exchange with their environment. In particular, an enhancement of the performance of quantum heat engines has been predicted by speeding up the dynamics through control of the system--bath interaction. However, direct microscopic control of heat transfer between the machine and the reservoir has remained elusive so far. Here, we experimentally demonstrate such control in a quantum Otto engine realized with ultracold Cs-133 atoms coupled to an atomic reservoir of ultracold Rb-87 atoms. Heat exchange between the two is mediated by inelastic s-wave collisions whose energy-dependent scattering cross sections lead to an asymmetric equilibration dynamics in the isochoric heating and cooling strokes. By tuning the kinetic temperature of the atomic reservoir, we modify the associated microscopic scattering rates, and thereby the heat transfer law, giving control over the time allocation within the engine cycle through control over the microscopic, multi-exponential relaxation dynamics. This enables power output optimization at fixed efficiency. Our results establish microscopic control of system-reservoir interactions as a tool for manipulating heat flow at the nanoscale and engineering the finite-time performance of quantum thermal machines.
Heat engines usually operate by exchanging heat with thermal baths at different (positive) temperatures. Nonthermal baths may, however, lead to a significant performance boost. We here experimentally analyze the power output of a single-atom quantum Otto engine realized in the quasi-spin states of individual Cesium atoms interacting with an atomic Rubidium bath. From measured time-resolved populations of the quasi-spin state, we determine the dynamics during the cycle of both the effective spin temperature and of the quantum fluctuations of the engine, which we quantify with the help of the Shannon entropy. We find that power is enhanced in the negative temperature regime, and that it reaches its maximum value at half the maximum entropy. Quantitatively, operating our engine at negative effective temperatures increases the power by up to 30% compared to operation at positive temperatures, including even the case of infinite temperature. At the same time, entering the negative temperature regime allows for reducing the entropy to values close to zero, offering highly stable operation at high power output. We furthermore numerically investigate the influence of the size of the Hilbert space on the performance of the quantum engine by varying the number of levels of the working medium. Our work thereby paves the way to fluctuation control in the operation of high-power and efficient single-atom quantum engines.
The fast-developing quantum technology is propelling thermal machine, which lies at the heart of thermodynamics, into a new golden era. Being stochastic because of the non-negligible thermal and quantum fluctuations, the efficiency and power of a finite-time quantum heat engine exhibit a trade-off, preventing the simultaneous achievement of high power and high efficiency. Conventional studies treat the statistics of a heat engine by assuming canonical thermalization, which is valid only under weak-coupling conditions. We here investigate the noncanonical effect on the statistics of the efficiency and power for a finite-time quantum Otto cycle. It is revealed that their average values and variances are highly controllable by engineering the energy spectrum structure of the composite system consisting of the working substance and the bath. Near the quantum critical point induced by the formation of a bound state in the energy spectrum, the average efficiency and power can be boosted simultaneously, meanwhile, both of their variances are decreased. Deepening our understanding of the usefulness of quantum reservoir engineering in thermodynamics, our result lays the foundation for the realization of efficient and stable quantum energy devices.
Developments in the thermodynamics of small quantum systems envisage nonclassical thermal machines. In this scenario, energy fluctuations play a relevant role in the description of irreversibility. We experimentally implement a quantum heat engine based on a spin-1/2 system and nuclear magnetic resonance techniques. Irreversibility at a microscope scale is fully characterized by the assessment of energy fluctuations associated with the work and heat flows. We also investigate the efficiency lag related to the entropy production at finite time. The implemented heat engine operates in a regime where both thermal and quantum fluctuations (associated with transitions among the instantaneous energy eigenstates) are relevant to its description. Performing a quantum Otto cycle at maximum power, the proof-of-concept quantum heat engine is able to reach an efficiency for work extraction (η≈42%) very close to its thermodynamic limit (η=44%).