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arXiv:2009.06164 · Physical Review Letters

Observation of Intensity Squeezing in Resonance Fluorescence from a Solid-State Device

Hui Wang, Jian Qin, Si Chen, Ming-Cheng Chen, Xiang You, Xing Ding, Yong-Heng Huo, Ying Yu, Christian Schneider, Sven Höfling, Marlan O. Scully, Chao‐Yang Lu, Jian-Wei Pan

Published Oct 7, 2020• 24 citations
arXivHTMLPDF

Abstract

Intensity squeezing-i.e., photon number fluctuations below the shot-noise limit-is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that intensity squeezing could be observed in resonance fluorescence from a two-level quantum system. However, its experimental observation in solid states was hindered by inefficiencies in generating, collecting, and detecting resonance fluorescence. Here, we report the intensity squeezing in a single-mode fiber-coupled resonance fluorescence single-photon source based on a quantum dot-micropillar system. We detect pulsed single-photon streams with 22.6% system efficiency, which show sub-shot-noise intensity fluctuation with an intensity squeezing of 0.59 dB. We estimate a corrected squeezing of 3.29 dB at the first lens. The observed intensity squeezing provides the last piece of the fundamental picture of resonance fluorescence, which can be used as a new standard for optical radiation and in scalable quantum metrology with indistinguishable single photons.

DOI
10.1103/physrevlett.125.153601

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Intensity squeezing-i.e., photon number fluctuations below the shot-noise limit-is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that intensity squeezing could be observed in resonance fluorescence from a two-level quantum system. However, its experimental observation in solid states was hindered by inefficiencies in generating, collecting, and detecting resonance fluorescence. Here, we report the intensity squeezing in a single-mode fiber-coupled resonance fluorescence single-photon source based on a quantum dot-micropillar system. We detect pulsed single-photon streams with 22.6% system efficiency, which show sub-shot-noise intensity fluctuation with an intensity squeezing of 0.59 dB. We estimate a corrected squeezing of 3.29 dB at the first lens. The observed intensity squeezing provides the last piece of the fundamental picture of resonance fluorescence, which can be used as a new standard for optical radiation and in scalable quantum metrology with indistinguishable single photons.
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Squeezed states of light enable optical measurements with sensitivity beyond the shot noise limit of detection with classical light. Optical fibers represent a major potential platform for quantum squeezed sensing due to the extremely low loss and perfect single-spatial-mode operation. In this work, we demonstrate two-mode intensity squeezing directly within a commercially available optical fiber, based on a four-wave mixing process. The setup operates in a quasi-continuous-wave mode using 15 ns long pulses and relies on standard laser diode sources, telecommunication electro-optic modulators, and simple photo-detectors. The process is seeded by a coherent signal input, generating bright squeezed output states. Absolute noise reduction by 4 dB below the classical shot-noise limit is detected directly with no post-processing, for output signal and idler pulses of 2.4 × 10 6 photons in average. The results are applicable to quantum interferometry over fiber using simple, readily available components.
We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of (20.7 ± 0.8) % per linear polarization basis. This yields an overall extraction efficiency of (41.4 ± 1.5) % in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical excitation, which enables us to deterministically populate the excited QD state. In this configuration, we probe the single photon statistics of the device yielding g(2)(0) = 0.072 ± 0.011 at a QD-cavity detuning of 75 μeV.
We develop high-efficiency single- and entangled-photons sources that simultaneously combine high purity, efficiency, and indistinguishability. We develop elliptical microcavities to boost the polarized single-photon extraction efficiency over 50%. We coherently excite a quantum dot with a dichromatic pulsed laser to circumvent the 50% loss issue in resonance fluorescence due to the polarization-extinction configuration. We directly observe intensity squeezing of 0.59 dB in resonance fluorescence, and a corrected squeezing of 3.29 dB at the first lens. Quantum interference between quantum-dot single photons and sunlight is also demonstrated in our experiments.
Quantum metrology enables us to estimate optical phase shifts beyond the shot noise limit. Applications include quantum-enhanced biological measurement [1], microscopy [2] and gravitational wave detection[3]. For two-mode N-photon system, the NOON state can achieve the highest possible phase sensitivity where multi-photon coherence between two states significantly contributes to improving the phase sensitivity. Another alternative approach to improve the phase sensitivity by use of squeezed states. Squeezing is usually characterized by reducing the quantum noise of desired observable at the expense of increasing the quantum noise for its non-commute partner. Because shot-noise limits the phase sensitivity of any classical states, the reduced quantum noise can be used for improving the phase sensitivity. Here we experimentally study the phase sensitivity of an optical spin-squeezed state by using linear optics. We generated the optical spin-squeezed state using one photon subtraction from a down converted photon source. To implement the sub-shot noise measurement, we used multiplexed photon number resolving detectors so that we can reconstruct the photon number statistics of the state. In the talk, we will analyse the generated state in terms of both squeezing and phase sensitivity by using Fisher information.
Scalable photonic quantum technologies require on-demand single-photon sources with simultaneously high levels of purity, indistinguishability, and efficiency. These key features, however, have only been demonstrated separately in previous experiments. Here, by s-shell pulsed resonant excitation of a Purcell-enhanced quantum dot-micropillar system, we deterministically generate resonance fluorescence single photons which, at π pulse excitation, have an extraction efficiency of 66%, single-photon purity of 99.1%, and photon indistinguishability of 98.5%. Such a single-photon source for the first time combines the features of high efficiency and near-perfect levels of purity and indistinguishabilty, and thus opens the way to multiphoton experiments with semiconductor quantum dots.