We present a direct mapping between the quantum optomechanical problem of the atoms harmonically trapped in the vicinity of a chiral waveguide and a generalized quantum Rabi model, and we discuss the analogy between the self-organization of atomic chains in photonic structures and Dicke-like quantum phase transitions in the ultrastrong coupling regime. We extend the class of the superradiant phase transitions for the systems possessing Z_{3} rather than parity Z_{2} symmetry and demonstrate the emergence of the multicomponent Schrödinger-cat ground states in these systems.
We present a direct mapping between the quantum optomechanical problem of the atoms harmonically trapped in the vicinity of a chiral waveguide and a generalized quantum Rabi model, and we discuss the analogy between the self-organization of atomic chains in photonic structures and Dicke-like quantum phase transitions in the ultrastrong coupling regime. We extend the class of the superradiant phase transitions for the systems possessing Z_{3} rather than parity Z_{2} symmetry and demonstrate the emergence of the multicomponent Schrödinger-cat ground states in these systems.
We develop a rigorous theoretical framework for interaction-induced phenomena in the waveguide quantum electrodynamics (QED) driven by mechanical oscillations of the qubits. Specifically, we predict that the simplest setup of two qubits, harmonically trapped over an optical waveguide, enables the ultrastrong coupling regime of the quantum optomechanical interaction. Moreover, the combination of the inherent open nature of the system and the strong optomechanical coupling leads to emerging parity-time (PT) symmetry, quite unexpected for a purely quantum system without artificially engineered gain and loss. The PT phase transition drives long-living subradiant states, observable in the state-of-the-art waveguide QED setups.
The Dicke model (DM) serves as a paradigm for understanding collective light-matter interactions. We introduce the chiral Dicke model, a generalization where an atomic ensemble couples to a two-mode cavity via chiral interactions. Unlike the standard DM, the chiral DM is endowed with an inherent continuous U(1) symmetry associated with angular momentum conservation. The ground-state phase diagram and the associated quantum phase transitions are charted out, revealing a U(1)-broken superradiant phase that spans a broad parameter space. We demonstrate that the spectrum of quantum fluctuations is highly tunable in both the symmetric and broken phases. Strikingly, our calculations reveal that the system exhibits `multiversality', where distinct universality classes govern the transition between the same two phases. In particular, along a special line in parameter space, the dynamical critical exponent for the normal-superradiant phase transition changes from zν=1 to zν=1/2. Our work establishes the chiral Dicke model as a powerful platform to realize novel quantum phases and multiversal critical phenomena in light-matter coupled systems.
Quantum optics is the field of physics that studies the interaction between light and matter under a fully quantum mechanical treatment. In recent decades, relentless advances in the technologies used for trapping, cooling, and controlling atoms and molecules have allowed us to finally start exploring experimentally the physics displayed by different cornerstone models of quantum optics originally proposed in the second half of the 20th century. In this thesis, we propose multiple extensions to those fundamental models, expanding the already interesting physics displayed by them into new and exciting directions. More specficially, we study these generalized models in the context of quantum phase transitions both in and out of equilibrium and show how new phases of matter can be unlocked in these extended models. In Chapters 1 and 2 we briefly introduce the reader to the realms of quantum phase transitions and quantum optics. Once the fundamental aspects of both of these fields are covered, we present the superradiant phase transition displayed in the Dicke and Rabi models in Chapter 3. This phase transition will be the central topic we will be orbiting around in the subsequent chapters. In Chapter 4 we propose a generalization of the quantum Rabi model, where N cavities, instead of one, are connected to each other through photon hopping. In this system, named the quantum Rabi ring, interesting chiral superradiant phases can develop as a function of the hopping phase and the geometry of the ring. In particular, we find that geometrical frustration plays a key role in determining the stable phases in equilibrium. Moreover, frustration manifests itself in the quantum Rabi ring through unconventional non-symmetric critical exponents, a phenomenon reported before, but hardly observed in condensed matter materials. Finally, in Chapter 5, we introduce a different extension to the Dicke model where instead of two-level atoms, three-level atoms are considered. In this system, which we have named the tricritical Dicke model, the superradiant phase transition can occur through first-order, second-order, and third-order critical points. We study the critical properties of the system in and out of equilibrium and find that in the open-system description, the tricritical points are still present but are now accompanied by regions of bistability where the final fate depends highly on the initial conditions. These regions of bistability represent potentially interesting environments to investigate dynamical features and steady-state preparation schemes. The critical phenomena displayed by the extended models proposed here, such as multicriticality, geometrically frustrated quantum phases, and chiral phases breaking time-reversal symmetry, are all features that have been observed, although not abundantly, or proposed in condensed matter physics. However, the unmatched tunability and control of atomic and molecular experimental platforms, where the models presented in this thesis are proposed to be realized, causes these extended models to become promising candidates for investigating these features in parameter regimes and conditions never explored before.
This study investigates phase-driven symmetry breaking leading to superradiance phase transitions in cascaded non-Hermitian quantum Rabi cavities. Non-Hermiticity is introduced via the phase coupling $\ensuremath{\varphi}$ between the atom and the optical field. In the thermodynamic limit of the quantum harmonic oscillator, we analytically derive the superradiance phase boundary, validated by observables. An unconventional quantum phase transition without a Hermitian analog arises when $|\ensuremath{\varphi}|=\frac{\ensuremath{\pi}}{4}$ or $\frac{3\ensuremath{\pi}}{4}$, where the phase boundary is uniquely determined by the cavity coupling, at J=21 (J is the ratio of the cavity coupling strength J to the optical field frequency ${\ensuremath{\omega}}_{p}$, and $\mathcal{J}=\frac{J}{{\ensuremath{\omega}}_{p}}$), independent of the atom-photon coupling strength g. For other $\ensuremath{\varphi}$, the phase boundary relies on both J and g, similar to the scenario observed in Hermitian systems. Furthermore, we identify phase-driven first- and second-order superradiance phase transitions, focusing on the quantum criticality of the second-order transition by determining the critical exponents and the universality class. The feasibility of experimental realization is also discussed, aiming to inspire further studies on non-Hermitian superradiance quantum phase transitions.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.
Recent experiments on a one-dimensional chain of trapped alkali-metal atoms [Bernien et al., Nature (London) 551, 579 (2017)] have observed a quantum transition associated with the onset of period-3 ordering of pumped Rydberg states. This spontaneous Z3 symmetry breaking is described by a constrained model of hard-core bosons proposed by Fendley et al. [Phys. Rev. B 69, 075106 (2004)]. By symmetry arguments, the transition is expected to be in the universality class of the Z3 chiral clock model with parameters preserving both time-reversal and spatial-inversion symmetries. We study the nature of the order--disorder transition in these models and numerically calculate its critical exponents with exact diagonalization and density-matrix renormalization-group techniques. We use finite-size scaling to determine the dynamical critical exponent z and the correlation length exponent $\ensuremath{\nu}$. Our analysis presents the only known instance of a strongly coupled generic transition between gapped states with $z\ensuremath{\ne}1$, implying an underlying nonconformal critical-field theory.