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arXiv:2008.12307 · Physical review. B./Physical review. B

Destabilization of U(1) Dirac spin liquids on two-dimensional nonbipartite lattices by quenched disorder

Santanu Dey

Published Dec 30, 2020• 3 citations
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Abstract

The stability of the Dirac spin liquid on two-dimensional lattices has long been debated. It was recently demonstrated [Nat. Commun. 10, 4254 (2019) and Phys. Rev. B 93, 144411 (2016)] that the staggered $\ensuremath{\pi}$-flux Dirac spin-liquid phase on the nonbipartite triangular lattice may be stable in the clean limit. However, quenched disorder plays a crucial role in determining whether such a phase is experimentally viable. For SU(2) spin systems, the effective zero-temperature low-energy description of Dirac spin liquids in $(2+1)$ dimensions is given by the compact quantum electrodynamics $({\mathrm{cQED}}_{2+1})$ which admits monopoles. It is already known that generic quenched random perturbations to the noncompact version of ${\mathrm{QED}}_{2+1}$ (where monopoles are absent) lead to strong-coupling instabilities. In this paper we study ${\mathrm{cQED}}_{2+1}$ in the presence of a class of time-reversal invariant quenched disorder perturbations. We show that in this model, random non-Abelian vector potentials make the symmetry-allowed monopole operators more relevant. The disorder-induced underscreening of monopoles, thus, generically makes the gapless spin-liquid phase fragile.

DOI
10.1103/physrevb.102.235165

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The stability of the Dirac spin liquid on two-dimensional lattices has long been debated. It was recently demonstrated [Nat. Commun. 10, 4254 (2019) and Phys. Rev. B 93, 144411 (2016)] that the staggered \ensuremathπ\ensuremath{\pi}\ensuremathπ-flux Dirac spin-liquid phase on the nonbipartite triangular lattice may be stable in the clean limit. However, quenched disorder plays a crucial role in determining whether such a phase is experimentally viable. For SU(2) spin systems, the effective zero-temperature low-energy description of Dirac spin liquids in (2+1)(2+1)(2+1) dimensions is given by the compact quantum electrodynamics (cQED2+1)({\mathrm{cQED}}_{2+1})(cQED2+1​) which admits monopoles. It is already known that generic quenched random perturbations to the noncompact version of QED2+1{\mathrm{QED}}_{2+1}QED2+1​ (where monopoles are absent) lead to strong-coupling instabilities. In this paper we study cQED2+1{\mathrm{cQED}}_{2+1}cQED2+1​ in the presence of a class of time-reversal invariant quenched disorder perturbations. We show that in this model, random non-Abelian vector potentials make the symmetry-allowed monopole operators more relevant. The disorder-induced underscreening of monopoles, thus, generically makes the gapless spin-liquid phase fragile.
It has been recently demonstrated [Song et al., Nature Comm. 10, 4254 (2019), Iqbal et al., Phys. Rev. B 93, 144411 (2016)] that the staggered π\piπ-flux Dirac spin liquid phase on the non-bipartite triangular lattice may be stable in the clean limit. However, quenched disorder plays a crucial role in determining whether such a phase can be experimentally viable. The effective low-energy description of Dirac spin liquids in (2+1)(2+1)(2+1) dimensions is given by the compact quantum electrodynamics (cQED2+1\rm cQED_{2+1}cQED2+1​) which admits monopoles. It is already known that generic quenched random perturbations to the non-compact version of QED2+1\rm QED_{2+1}QED2+1​ (where monopoles are absent) lead to strong-coupling instabilities. In this work we study cQED2+1\rm cQED_{2+1}cQED2+1​ in the presence of a class of time-reversal invariant quenched disorder perturbations. We show that in this model, random non-abelian vector potentials make the symmetry-allowed monopole operators more relevant. The disorder induced under-screening of monopoles thus generically makes the gapless spin liquid phase fragile.
The U(1)U(1)U(1) Dirac spin liquid might realize an exotic phase of matter whose low-energy properties are described by quantum electrodynamics in 2+12+12+1 dimensions, where gapless modes exist but spinons and gauge fields are strongly coupled. Its existence was proposed in frustrated Heisenberg models in the presence of frustrating superexchange interactions by the (Abrikosov) fermionic representation of the spin operators [Wen, Phys. Rev. B 65, 165113 (2002)], supplemented by the Gutzwiller projection. Here, we construct charge-QQQ monopole excitations in the Heisenberg model on the triangular lattice with nearest-neighbor (J1{J}_{1}J1​) and next-nearest-neighbor (J2{J}_{2}J2​) couplings. In the highly frustrated regime, singlet and triplet monopoles with Q=1Q=1Q=1 become gapless in the thermodynamic limit; in addition, the energies for generic QQQ agree with field-theoretical predictions, obtained for a large number of gapless fermion modes. Finally, we consider localized gauge excitations, in which magnetic $\ensuremath{\pi}$ fluxes are concentrated in the triangular plaquettes (in analogy with Z2{\mathbb{Z}}_{2}Z2​ visons), showing that these kinds of states do not play a relevant role at low energies. All our findings lend support to a stable U(1)U(1)U(1) Dirac spin liquid in the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ Heisenberg model on the triangular lattice.
A complicating factor in the realization and observation of quantum spin liquids in materials is the ubiquitous presence of other degrees of freedom, in particular lattice distortion modes (phonons). These provide additional routes for relieving magnetic frustration, thereby possibly destabilizing spin-liquid ground states. In this work, we focus on triangular-lattice Heisenberg antiferromagnets, where recent numerical evidence suggests the presence of an extended U(1) Dirac spin liquid phase which is described by compact quantum electrodynamics in 2+1 dimensions (QED3_33​), featuring gapless spinons and monopoles as gauge excitations, and believed to flow to a strongly-coupled fixed point with conformal symmetry. Using complementary perturbation theory and scaling arguments, we show that a symmetry-allowed coupling between (classical) finite-wavevector lattice distortions and monopole operators of the U(1) Dirac spin liquid generally induces a spin-Peierls instability towards a (confining) 12-site valence-bond solid state. We support our theoretical analysis with state-of-the-art density matrix renormalization group simulations. Away from the limit of static distortions, we demonstrate that the phonon energy gap establishes a parameter regime where the spin liquid is expected to be stable, and show that the monopole-lattice coupling leads to softening of the phonon in analogy to the Kohn anomaly. We discuss the applicability of our results to similar systems, in particular the Dirac spin liquid on the Kagome lattice.
When two layers of two-dimensional materials are assembled with a relative twist, moir\'e patterns arise, inducing a tremendous wealth of exotic phenomena. In this work, we consider twisting two triangular lattices hosting Dirac quantum spin liquids. A single decoupled layer is described by compact quantum electrodynamics in 2+12+12+1 dimensions (QED3{\mathrm{QED}}_{3}QED3​) with an emergent U(1)\mathrm{U}(1)U(1) gauge field, which is assumed to flow to a strongly interacting fixed point in the IR with conformal symmetry. We use recent results for the quantum numbers of monopole operators, which tunnel $2\ensuremath{\pi}$ fluxes of the compact gauge field. It is found that, in the bilayer system, interlayer monopole tunneling is a symmetry-allowed relevant perturbation which induces an (ordering) instability. We show using perturbation theory that upon twisting the two layers the system remains unstable under the interlayer interaction, but any finite twist angle softens this instability compared to the untwisted case. To analyze the resulting phase induced by the (twisted) interlayer tunneling, we use ``conformal mean-field theory'', which reduces the interacting bilayer system to two copies of QED3{\mathrm{QED}}_{3}QED3​ coupled to background fields which are to be determined self-consistently. In the weak-coupling regime, where the interlayer coupling is weak compared to the energy scale set by the moir\'e lattice constant, we solve the self-consistency equations perturbatively. In the limit of strongly coupled layers, a local scaling approximation is used, and we find that the magnetically ordered state exhibits a lattice of magnetic vortices, with the lattice constant tunable through the twisting angle.
Theory of Dirac Spin-Orbital Liquids: monopoles, anomalies, and applications to SU(4)SU(4)SU(4) honeycomb models
Dirac spin liquids represent a class of highly-entangled quantum phases in two dimensional Mott insulators, featuring exotic properties such as critical correlation functions and absence of well-defined low energy quasi-particles. Existing numerical works suggest that the spin-orbital SU(4)SU(4)SU(4) symmetric Kugel-Khomskii model of Mott insulators on the honeycomb lattice realizes a Dirac spin-orbital liquid, described at low energy by (2+1)d(2+1)d(2+1)d quantum electrodynamics (QED3_33​) with Nf=8N_f=8Nf​=8 Dirac fermions. We generalize methods previously developed for SU(2)SU(2)SU(2) spin systems to analyze the symmetry properties and stability of the Dirac spin-orbital liquid. We conclude that the standard Dirac state in the SU(4)SU(4)SU(4) honeycomb system, based on a simple parton mean-field ansatz, is intrinsically unstable at low energy due to the existence of a monopole perturbation that is allowed by physical symmetries and relevant under renormalization group flow. We propose two plausible alternative scenarios compatible with existing numerics. In the first scenario, we propose an alternative U(1)U(1)U(1) Dirac spin-orbital liquid, which is similar to the standard one except for its monopole symmetry quantum numbers. This alternative U(1)U(1)U(1) state represents a stable gapless phase. In the second scenario, we start from the standard U(1)U(1)U(1) Dirac liquid and Higgs the U(1)U(1)U(1) gauge symmetry down to Z4\mathbb{Z}_4Z4​. The resulting Z4\mathbb{Z}_4Z4​ Dirac spin-orbital liquid is stable. We also discuss the continuous quantum phase transitions from the Z4\mathbb{Z}_4Z4​ Dirac liquids to conventional symmetry-breaking orders, described by the QED3_33​ theory with Nf=8N_f=8Nf​=8 supplemented with a critical charge-444 Higgs field. We discuss possible ways to distinguish these scenarios in numerics. We also extend previous calculations of the quantum anomalies of QED3_33​ and match with generalized lattice Lieb-Schultz-Mattis constraints.
Algebraic spin liquids are quantum disordered phases of insulating magnets that exhibit fractionalized gapless excitations and power-law correlations. Quantum spin liquids in this category include the experimentally established one-dimensional (1D) Luttinger liquid, as well as the U(1) Dirac spin liquid (DSL) that has been a focus of recent candidate materials searches. Most notably, several exchange-frustrated Heisenberg materials on the triangular lattice have shown evidence of the U(1) DSL. In this work, we measure the algebraic correlations of spin-singlet excitations in the J 1 − J 2 antiferromagnetic Heisenberg model on the triangular lattice, prompting a detailed investigation of this model’s stability under spin-lattice coupling with dynamical phonons using variational Monte Carlo. As seen before in 1D spin chains, we observe a low-temperature transition from a U(1) DSL to valence bond order and predict the parameter regime where the model realizes a stable DSL ground state. To achieve this, we employ a series of finite-size scaling Ansätze inspired by the low-energy DSL’s conformal description in terms of quantum electrodynamics and show that emergent monopole operators drive the instability. We compare the physics of this transition to the 1D Luttinger liquid throughout our analysis. We derive the regime of stability against spin-Peierls ordering and argue that the DSL ground state might still be achievable in candidate materials, despite its tendency to valence bond solid ordering.