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arXiv:2008.11740

Imbalanced Fermi systems and exotic superconducting phases

Madhuparna Karmakar

Published Aug 26, 2020• 0 citations
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Abstract

Quantum many body phases, in competition or coexistence has always been a fascinating area of research in condensed matter physics. One of the most widely investigated scenario of phase competition is that between superconductivity and magnetism, which in spite of several decades of research continues to bring up new surprises till date. While superconductivity and magnetism are naively considered to be antagonists, there are several circumstances where these many body phases can be found to be cooperating, coexisting and even promoting each other. The results of such cooperative behavior are found to show up as exotic quantum phases. In this chapter we discuss about such an exotic superconducting phase, which comes to life when a particular class of superconducting material viz. "Pauli limited superconductors" are subjected to an imbalance between the population of the fermionic species undergoing pairing. The consequence of such an imbalance is the emergence of a non-trivial spatially modulated superconducting phase, popularly known as the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. Characterized by a finite momentum pairing between the fermionic species the FFLO phase hosts a non zero magnetization, leading to an unconventional coexistent phase of superconductivity and magnetism.

DOI
10.48550/arxiv.2008.11740

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Quantum many body phases, in competition or coexistence has always been a fascinating area of research in condensed matter physics. One of the most widely investigated scenario of phase competition is that between superconductivity and magnetism, which in spite of several decades of research continues to bring up new surprises till date. While superconductivity and magnetism are naively considered to be antagonists, there are several circumstances where these many body phases can be found to be cooperating, coexisting and even promoting each other. The results of such cooperative behavior are found to show up as exotic quantum phases. In this chapter we discuss about such an exotic superconducting phase, which comes to life when a particular class of superconducting material viz. "Pauli limited superconductors" are subjected to an imbalance between the population of the fermionic species undergoing pairing. The consequence of such an imbalance is the emergence of a non-trivial spatially modulated superconducting phase, popularly known as the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. Characterized by a finite momentum pairing between the fermionic species the FFLO phase hosts a non zero magnetization, leading to an unconventional coexistent phase of superconductivity and magnetism.
Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconductivity, Cooper pairing at finite-momentum driven by spin imbalance, remains difficult to study numerically in two dimensions. The fermion sign problem in the spin-imbalanced attractive Hubbard model severely limits quantum Monte Carlo access to the low temperatures where pairing correlations are most pronounced. We show that the Holstein model, in which the effective attraction is retarded by phonon dynamics, strongly suppresses sign fluctuations under spin imbalance, enabling unbiased determinant quantum Monte Carlo simulations deep in this regime. With increasing magnetization, zero-momentum pairing evolves into finite-momentum FFLO pairing, evidenced by oscillating real-space pair correlations and a shift of the pairing susceptibility peak to finite Q⃗\vec{Q}Q​. The finite-momentum susceptibility substantially exceeds its zero-momentum value. At high density n∼0.875n \sim 0.875n∼0.875, near magnetization m≈1−nm \approx 1-nm≈1−n where the majority-spin density approaches half filling, FFLO pairing coexists with checkerboard charge-density-wave order at short range, while staggered longitudinal spin correlations emerge as a magnetic halo at larger distances. These spatial textures provide experimentally accessible signatures of finite-momentum pairing and motivate cold-atom realizations of FFLO physics.
We report a quantum phase transition in Pauli limited d-wave superconductors and give the mean field estimates of the associated quantum critical point. For a population imbalanced d-wave superconductor a stable ground state phase viz quantum breached pair phase has been identified which comprises of spatial coexistence of gapless superconductivity and nonzero magnetization. Based on the thermodynamic and quasiparticle indicators we for the first time analyze this phase, discuss the thermal behavior of Pauli limited d-wave superconductor, give accurate estimates of the thermal scales associated with such systems and map out the pseudogap regime. Our work shows that while the Pauli limited superconductors are known to exhibit exotic modulated superconducting phase at large imbalance of fermion populations; in the regime of weak imbalance an intriguing phase of competing orders is realized. We have established that rather than the superconducting pairing field, it is the average magnetization of the system that quantifies this quantum phase transition. Given that the existing Pauli limited superconductors possess unconventional pairing state symmetry of the superconducting order, our work promises to open up new avenues in the experimental research of these materials. We have also demonstrated an alternate scenario wherein the quantum breached pair phase is a natural outcome for a d-wave superconductor with unequal effective masses of the fermion species.
Abstract Ultracold two-component Fermi gases with a tunable population imbalance have provided an excellent opportunity for studying the exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states, which have been of great interest in condensed matter physics. However, the FFLO states have not been observed experimentally in Fermi gases in three dimensions (3D), possibly due to their small phase space volume and extremely low temperature required for an equal-mass Fermi gas. Here we explore possible effects of mass imbalance, mainly in a 6Li–40K mixture, on the one-plane-wave FFLO phases for a 3D homogeneous case at the mean-field level. We present various phase diagrams related to the FFLO states at both zero and finite temperatures, throughout the BCS-BEC crossover, and show that a large mass ratio may enhance substantially FFLO type of pairing.
The ground-state phase diagram of attractively interacting Fermi gases in two dimensions with a population imbalance is investigated. We find the regime of stability for the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase, in which pairing occurs at a finite wave vector, and determine the magnitude of the pairing amplitude $\mathrm{\ensuremath{\Delta}}$ and FFLO wave vector qqq in the ordered phase, finding that $\mathrm{\ensuremath{\Delta}}$ can be of the order of the two-body binding energy. Our results rely on a careful analysis of the zero-temperature gap equation for the FFLO state, which possesses nonanalyticities as a function of $\mathrm{\ensuremath{\Delta}}$ and qqq, invalidating a Ginzburg-Landau expansion in small $\mathrm{\ensuremath{\Delta}}$.
ddd-wave FFLO state and charge-2e supersolidity in the ttt-t′t't′-JJJ model under Zeeman fields
Unconventional superconductivity under strong Zeeman fields--particularly beyond the Pauli paramagnetic limit--remains a central challenge in condensed matter physics. The exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, in particular, remains in need of definitive study within fundamental electronic models. Here we employ state-of-the-art finite-temperature and ground-state tensor network approaches to systematically explore the superconducting (SC) phase diagram of the ttt-t′t't′-JJJ model subjected to Zeeman fields. We find that zero-momentum ddd-wave superconductivity persists until the spin gap closes, coexisting with charge density waves. A novel ddd-wave FFLO phase emerges under a higher Zeeman field even above the Pauli limit, concomitant with a field-enhanced spin density waves. We identify these phases, characterized by the simultaneous presence of pairing condensate and density wave orders, as charge-2e supersolids. Analysis of Matsubara Green's function reveals that the FFLO pairing momentum is locked to the underlying Fermi surface. Our results provide microscopic insights into field-induced unconventional pairing mechanisms and reveal the long-sought FFLO state in a fundamental correlated electron model, offering a promising route for its realization in ultracold atom optical lattice.
We theoretically explore a promising route to achieve the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state in a spin-imbalanced ultracold Fermi gas. In the current stage of cold atom physics, search for this exotic Fermi superfluid is facing two serious difficulties: One is the desperate destruction of the FFLO long-range order by FFLO pairing fluctuations, which precludes entering the phase through a second-order transition, even in three dimension. The other is the fierce competition with the phase separation into the BCS (Bardeen-Cooper-Schrieffer) state and the spin-polarized normal state. By including strong FFLO pairing fluctuations within the framework of the strong-coupling theory developed by Nozi\`eres and Schmitt-Rink, we show that the anisotropy of Fermi surface introduced by an optical lattice makes the FFLO state stable against the paring fluctuations. This stabilized FFLO state is also found to be able to overcome the competition with the phase separation under a certain condition. Since the realization of unconventional Fermi superfluids is one of the most exciting challenges in cold atom physics, our results would contribute to the further development of this field.