The advent of the quantum gas microscope allowed for the in situ probing of ultracold gaseous matter on an unprecedented level of spatial resolution.However, the study of phenomena on ever smaller length scales, as well as the probing of three-dimensional systems, is fundamentally limited by the wavelength of the imaging light for all techniques based on linear optics.Here, we report on a high-resolution ion microscope as a versatile and powerful experimental tool to investigate quantum gases.The instrument clearly resolves atoms in an optical lattice with a spacing of 532 nm over a field of view of 50 sites and offers an extremely large depth of field on the order of at least 70 μm.With a simple model, we extract an upper limit for the achievable resolution of approximately 200 nm from our data.We demonstrate a pulsed operation mode enabling 3D imaging and allowing for the study of ionic impurities and Rydberg physics.
The advent of the quantum gas microscope allowed for the in situ probing of ultracold gaseous matter on an unprecedented level of spatial resolution.However, the study of phenomena on ever smaller length scales, as well as the probing of three-dimensional systems, is fundamentally limited by the wavelength of the imaging light for all techniques based on linear optics.Here, we report on a high-resolution ion microscope as a versatile and powerful experimental tool to investigate quantum gases.The instrument clearly resolves atoms in an optical lattice with a spacing of 532 nm over a field of view of 50 sites and offers an extremely large depth of field on the order of at least 70 μm.With a simple model, we extract an upper limit for the achievable resolution of approximately 200 nm from our data.We demonstrate a pulsed operation mode enabling 3D imaging and allowing for the study of ionic impurities and Rydberg physics.
Imagine a new generation of computers that dramatically surpasses the most powerful supercomputers, being able to tackle the most challenging of computational problems. These problems arise, for example, in quantum physics where the computational power required to model a many-particle system increases exponentially with the number of its constituents, and as a consequence the calculations become prohibitively time-consuming. Nobel laureate Richard Feynman proposed this new type of computer in the early 1980s: ‘Let the computer itself be built of quantum mechanical elements which obey quantum mechanical laws.’ Such a quantum simulator would allow researchers to tackle challenging problems in condensed-matter physics. In particular many-body fermionic quantum systems are very difficult to compute due to the antisymmetric nature of the wave function, and the resulting sign problem for quantum Monte Carlo methods. This is why a quantum simulator will be an excellent test bed to investigate phenomena and properties of strongly correlated fermionic quantum systems. A powerful experimental platform to realize a quantum simulator is laser-cooled atoms [1] held in an artificial crystal of light, generated by superimposing laser beams. The atoms are kept in this optical lattice similar to marbles in the hollows of an egg carton, and they can mimic the behaviour of electrons in a real crystal. These systems interface atomic physics with condensed matter physics in a new way, as the tools of atomic physics allow for exquisite control of many experimental parameters, which are often inaccessible in solid state experiments. In-situ imaging techniques [2] using ‘quantum-gas microscopes’ constitute a new approach to the study of many-body quantum systems in an optical lattice with unprecedented resolution at the single-particle and single-site level [3,4]. This new method is complementary to earlier optical lattice experiments measuring distributions in momentum space after a time-of-flight expansion. A quantum-gas microscope uses an optical imaging system (Fig. 1a) for collecting the fluorescence light of ultracold atoms in an optical lattice with high spatial resolution comparable to the lattice spacing of ≈ 500 nm. (a) Atoms in optical lattice atoms are imaged with a high-resolution microscope objective [4]. (b) Single-site addressing is achieved by focussing a laser beam through the microscope onto selected atoms, bringing them into resonance with microwave radiation which produces spin flips [12]. (c) and (d) Single-atom-resolved fluorescence images of bosonic Mottinsulators [4,9]. (e) Deterministically prepared atom distribution using single-site addressing [12]. (f) Direct observation of single-atom quantum walks [15]. Fluorescence imaging of atoms in a quantum-gas microscope has made it possible to directly observe bosonic Mott insulators with single-atom resolution [4–6], giving access to in-situ measurements of temperature and entropy distributions. Subsequently, ground-breaking experiments in many-body quantum dynamics have been performed, such as the first direct observation of correlation spreading after quenches of the system to lower lattice depths [7]. Other experiments include the quantum simulation of an antiferromagnetic spin-1/2 chain [8], the realization of algorithmic cooling [9], the direct measurement of correlations across the superfluid-to-Mott-insulator transition [10], or the observation of the ‘Higgs’ amplitude mode [11]. The high-resolution imaging system is also capable of optically addressing individual atoms with sub-diffraction-limited resolution. For this purpose, a laser beam is focussed though the microscope objective onto selected lattice sites, bringing the atoms into resonance with microwave radiation which produces spin flips [12,13]. The preparation of arbitrary atom distributions in the lattice not only opens perspectives for neutral-atom quantum information processing, but also allows the deterministic creation of specific out-of-equilibrium situations, and their ensuing system dynamics can be studied with single-atom resolution. Examples include the creation of spin impurities and the study of their dynamics in a many-body system [14], the observation of quantum walks [15] and magnon-bound states [16], and the measurement of entanglement entropy [17]. The technique used for single-site-resolved detection of individual atoms in the optical lattice is fluorescence imaging. It requires laser cooling of the atoms to sub-Doppler temperatures while detecting the fluorescence photons emitted during this process. A challenge is to achieve a low particle loss rate and to prevent the atoms from hopping between lattice sites. In the case of the first quantum-gas microscopes, this has been implemented with bosonic rubidium-87 atoms, and also recently for ytterbium-174. However, it has proven more challenging for fermionic alkaline species such as potassium-40 and lithium-6, as their low mass and small excited state hyperfine splitting-prevented standard sub-Doppler cooling from working. As a result, it took several years to extend the quantum-gas microscope technique to fermionic species, and in 2015 several groups have demonstrated single-atom-resolved imaging of fermions [18]. In these setups, the direct observation of band insulators [19], fermionic Mott insulators [20,21] and even antiferromagnetic correlations [22] has been reported most recently. These developments provide fascinating opportunities to study many-body fermionic quantum systems with single-particle access. The fermionic nature of the electron is vital to understanding a range of phenomena within solid-state physics, such as electron pairing in superconductivity, and quantum magnetism. In this context, the quantum simulator will allow, e.g. for direct measurement of ordered quantum phases and out-of-equilibrium dynamics, with access to quantities such as spin--spin correlation functions and the growth of many-body entanglement. The high-resolution imaging systems could also be used to project tailored time-varying light fields onto the atoms, allowing the removal of high-entropy regions by locally modifying the confining potential to attain very low-entropy states. Attaining these low-entropy many-particle states is one of the key challenges in our field. In summary, quantum-gas microscopes offer unprecedented access to many-body quantum systems, and they will allow us to gain an even deeper insight into the intriguing world of quantum physics that governs the properties of strongly correlated materials. Using a well-controlled quantum system to simulate other quantum systems could help resolve some of the most challenging problems scientists face in condensed matter physics and materials science, but it will also provide new insights in quantum chemistry, high-energy physics and biology. SK acknowledges funding from the EU (ERC FERMILATT, SIQS, QuProCs) and SUPA.
Quantum Gases
Quantum microscopes have been used for more than a decade now to image the many-body states of quantum gases in optical lattices. However, their resolution is limited to optical wavelengths, and they can typically image only a single layer of atoms. As a complementary technique for imaging quantum gases, Veit et al. developed an ion microscope. Atoms were first ionized by laser light, and the resulting ions were controlled using electrostatic lenses and imaged. Although the technique was demonstrated on rubidium atoms in their ground state, it is expected that it will also work on highly excited Rydberg atoms and will enable three-dimensional and time-dependent imaging.
Phys. Rev. X 11 , 011036 (2021).
We report on an ion-optical system that serves as a microscope for ultracold ground state and Rydberg atoms. The system is designed to achieve a magnification of up to 1000 and a spatial resolution in the 100 nm range, thereby surpassing many standard imaging techniques for cold atoms. The microscope consists of four electrostatic lenses and a microchannel plate in conjunction with a delay line detector in order to achieve single particle sensitivity with high temporal and spatial resolution. We describe the design process of the microscope including ion-optical simulations of the imaging system and characterize aberrations and the resolution limit. Furthermore, we present the experimental realization of the microscope in a cold atom setup and investigate its performance by patterned ionization with a structure size down to 2.7 μ m. The microscope meets the requirements for studying various many-body effects, ranging from correlations in cold quantum gases up to Rydberg molecule formation.
Abstract Imaging is central to gaining microscopic insight into physical systems, and new microscopy methods have always led to the discovery of new phenomena and a deeper understanding of them. Ultracold atoms in optical lattices provide a quantum simulation platform, featuring a variety of advanced detection tools including direct optical imaging while pinning the atoms in the lattice1,2. However, this approach suffers from the diffraction limit, high optical density and small depth of focus, limiting it to two-dimensional (2D) systems. Here we introduce an imaging approach where matter wave optics magnifies the density distribution before optical imaging, allowing 2D sub-lattice-spacing resolution in three-dimensional (3D) systems. By combining the site-resolved imaging with magnetic resonance techniques for local addressing of individual lattice sites, we demonstrate full accessibility to 2D local information and manipulation in 3D systems. We employ the high-resolution images for precision thermodynamics of Bose–Einstein condensates in optical lattices as well as studies of thermalization dynamics driven by thermal hopping. The sub-lattice resolution is demonstrated via quench dynamics within the lattice sites. The method opens the path for spatially resolved studies of new quantum many-body regimes, including exotic lattice geometries or sub-wavelength lattices3–6, and paves the way for single-atom-resolved imaging of atomic species, where efficient laser cooling or deep optical traps are not available, but which substantially enrich the toolbox of quantum simulation of many-body systems.
The development of quantum-gas microscopes has brought novel ways of probing quantum degenerate many-body systems at the single-atom level. Until now, most of these setups have focused on alkali atoms. Expanding quantum-gas microscopy to alkaline-earth elements will provide new tools, such as SU( N )-symmetric fermionic isotopes or ultranarrow optical transitions, to the field of quantum simulation. Here we demonstrate the site-resolved imaging of a 84 Sr bosonic quantum gas in a Hubbard-regime optical lattice. The quantum gas is confined by a two-dimensional in-plane lattice and a light-sheet potential, which operate at the strontium clock-magic wavelength of 813.4 nm. We realize fluorescence imaging using the broad 461-nm transition, which provides high spatial resolution. Simultaneously, we perform attractive Sisyphus cooling with the narrow 689-nm intercombination line. We reconstruct the atomic occupation from the fluorescence images, obtaining imaging fidelities above 94 % . Finally, we realize a 84 Sr superfluid in the Bose-Hubbard regime. We observe its interference pattern upon expansion, a probe of phase coherence, with single-atom resolution. Our strontium quantum-gas microscope provides a new platform to study dissipative Hubbard models, quantum optics in atomic arrays, and SU( N ) fermions at the microscopic level. Published by the American Physical Society 2024
Our knowledge on ultracold quantum gases is strongly influenced by our ability to probe these objects. In situ imaging combined with single atom sensitivity is an especially appealing scenario as it can provide direct information on the structure and the correlations of such systems. For a precise characterization a high spatial resolution is mandatory. In particular, the perspective to study quantum gases in optical lattices makes a resolution well below one micrometer highly desirable. Here, we report on a novel microscopy technique which is based on scanning electron microscopy and allows for the detection of single atoms inside a quantum gas with a spatial resolution of better than 150 nm. Imaging a Bose-Einstein condensate in a one-dimensional optical lattice with 600 nm period we demonstrate single site addressability in a sub-um optical lattice. The technique offers exciting possibilities for the preparation, manipulation and analysis of quantum gases.