Experimental setup for the production of ultracold strongly correlated fermionic superfluids of 6Li
Diego Hernández-Rajkov, J. E. Padilla‐Castillo, Manuel Mendoza-Lopez, Ricardo Colín‐Rodríguez, Andrés Gutiérrez-Valdés, Sebastián A. Morales-Ramírez, R. A. Gutiérrez-Arenas, Carlos Gardea-Flores, Rocío Jáuregui, Jorge Amin Seman, Freddy Jackson Poveda-Cuevas, G. Roati
We present our experimental setup to produce ultracold strongly correlated fermionic superfluids made of a two-component spin-mixture of 6Li atoms. Employing standard cooling techniques, we achieve quantum degeneracy in a single-beam optical dipole trap. Our setup is capable of generating spin-balanced samples at temperatures as low as T/TF = 0.1 containing up to 5 × 10^4 atomic pairs. We can access different superfluid regimes by tuning the interparticle interactions close to a broad magnetic Feshbach resonance. In particular, we are able to explore the crossover from the molecular Bose-Einstein condensate (BEC) to the Bardeen-Cooper-Schrieffer (BCS) superfluid regimes. In the near future, we plan to study different collective excitations in these superfluid samples.
We present our experimental setup to produce ultracold strongly correlated fermionic superfluids made of a two-component spin-mixture of 6Li atoms. Employing standard cooling techniques, we achieve quantum degeneracy in a single-beam optical dipole trap. Our setup is capable of generating spin-balanced samples at temperatures as low as T/TF = 0.1 containing up to 5 × 10^4 atomic pairs. We can access different superfluid regimes by tuning the interparticle interactions close to a broad magnetic Feshbach resonance. In particular, we are able to explore the crossover from the molecular Bose-Einstein condensate (BEC) to the Bardeen-Cooper-Schrieffer (BCS) superfluid regimes. In the near future, we plan to study different collective excitations in these superfluid samples.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
The work described in this thesis can be divided into two parts. The first part is concerned with the production of degenerate Fermi gases and Bose-Fermi mixtures. The second part of the thesis describes studies of strongly interacting spin-mixtures of ultracold fermions. We have cooled a magnetically trapped spin-polarized 6Li Fermi gas into quantum degeneracy by sympathetic cooling with bosonic 23Na. In order to do this, we have converted our previously developed apparatus for Bose-Einstein condensation of 23Na into a two-species cooling facility. We have produced 6Li samples with up to 7 × 107 atoms at temperatures below 0.5TF , and up to 3× 107 atoms at temperatures as low as 0.05TF . Further, we have also produced stable quantum degenerate mixtures of 23Na and 6Li, with several million atoms of each species. In a second set of experiments, we have studied strongly interacting spin-mixtures of 6Li. The strength of interactions was resonantly controlled by applying a magnetic field and tuning to “Feshbach resonances”, which occur when the total energy of the colliding particles coincides with the energy of a bound molecular state. These studies are relevant for the continuing quest for a superfluid transition in a Fermi gas. By studying the inelastic decay of the cloud, we have experimentally identified two Feshbach resonances for the inter-state interactions of the two lowest ground states of 6Li. Most importantly, we found that the lifetime of the strongly interacting system is long enough to observe a superfluid transition in the future. The effects of the coherent collisions in 6Li spin-mixtures were studied using radiofrequency (RF) spectroscopy. We demonstrated the absence of mean field “clock shifts” in a two-state mixture of fermions, and have introduced a three-level method to observe the interaction energy shifts. In the strongly interacting regime, near a Feshbach resonance, we have observed universal behavior of the interaction energy, independent of the value of the scattering length. Finally, we have theoretically studied the effects of Pauli blocking during a free expansion of a degenerate Fermi gas. We have concluded that a strongly interacting normal gas will undergo a hydrodynamic expansion even at zero temperature, due to inefficiency of the Pauli suppression of collisions. Therefore, the already observed hydrodynamic expansion cannot be conclusively interpreted as a signature of superfluidity. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacArthur Professor of Physics
We present an overview of our recent measurements on the crossover from a Bose‐Einstein condensate of molecules to a Bardeen‐Cooper‐Schrieffer superfluid. The experiments are performed on a two‐component spin‐mixture of 6Li atoms, where a Feshbach resonance serves as the experimental key to tune the s‐wave scattering length and thus to explore the various interaction regimes. In the BEC‐BCS crossover, we have characterized the interaction energy by measuring the size of the trapped gas, we have studied collective excitation modes, and we have observed the pairing gap. Our observations provide strong evidence for superfluidity in the strongly interacting Fermi gas.
In this habilitation-thesis a collection of 14 experiments is presented. In these experiments we have developed and used novel techniques to control ultracold gases on the quantum level. In brief, Bose-Einstein condensates (BEC) and degenerate Fermi gases of laser-cooled alkali atoms are subjected to specially designed optical and magnetic fields. The fields influence in a coherent way the behavior, properties and dynamics of the gases. On this basis we developed tools to prepare, coherently manipulate, and analyze pre-defined quantum states. With this high level of control, it was possible to investigate interesting physics phenomena, and we were able to achieve several breakthroughs in the field of ultracold atoms. Highlights of our experimental results include the demonstration of phase engineering of a BEC wavefunction where we created solitons in a BEC and studied their propagation. In another experiment we constructed a spatially resolved matter wave interferometer with which we mapped out the phase distribution on a condensate. Illuminating the BEC with a periodic pattern, i.e. an optical lattice, allowed us to study solid states physics phenomena. In a second set of experiments we demonstrated optically tuning of the interaction between atoms with optical Feshbach resonances. Employing either magnetically tunable Feshbach resonances or laser radiation, we were able to produce ground state molecules in well defined quantum states. This led to the production of the first molecular BEC. By tuning the coupling of atom pairs in a Fermi gas of atoms, we could for the first time investigate the so-called BEC-BCS crossover which describes the continuous change from a BEC superfluid to a Bardeen-Cooper Schrieffer (BCS) superfluid. Due to the excellent control on the quantum level, the developed cold atom techniques open up intriguing prospects for future applications and experiments. They represent a general tool box to investigate fundamental physical phenomena in a pure and undisturbed environment. In the future, cold atoms might serve as a testing ground for fundamental theories or as quantum simulators for complex systems.
Ultracold mixture experiments hold the promise of providing new insights into many-body quantum systems as well as ultracold chemistry and few-body phenomena. The work presented in this thesis dealt with the construction of a new apparatus for the production and study of ultracold gases of fermionic lithium-6 and bosonic caesium-133. These isotopes offer a wide tunability in their interaction strength, both in inter-species and intra-species collisions, through magnetic Feshbach resonances. Additionally, the widely different resonance frequencies of lithium and caesium enables independent control of each of the species. With this apparatus, Bose-Einstein condensates (BEC) containing 10^4 lithium Feshbach molecules are routinely produced. The cooling system for caesium has been developed in parallel and important steps towards producing ultracold caesium gases have been made. An optical dipole trap has been loaded with 2x10^6 caesium atoms and evaporative cooling towards quantum degeneracy can now be pursued. Laser, vacuum, magnetic and control systems have been developed for the implementation of this experiment. Light produced with this laser system was used to laser cool atoms, create conservative dipole traps as well as to provide means of imaging atomic clouds. Additionally, a system to produce strong magnetic fields of up to 1400 G has been established in order to exploit the wide tunability in the atomic interactions. Software that was developed for the computerised control system facilitated the coordination of all the components involved in the experimental sequence. Measurements and calculations that showcase the functionality of relevant parts of the setup are presented in this thesis. In this experiment, lithium and caesium atoms are obtained from a novel type of Zeeman slower and are loaded into a magneto-optical trap (MOT). The system is capable of doing this independently for each of the atomic species as well as sequentially. After the MOT has been loaded with atoms, they are transferred into a conservative far-off-resonance optical dipole trap. By adjusting the interactions between atoms and lowering the depth of the dipole trap, efficient evaporative cooling of lithium was carried out from which a molecular BEC was obtained. Time-of-flight measurements were used to characterise the condensate and study its expansion dynamics.