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arXiv:2008.02257 · Nano Letters

Signature of Many-Body Localization of Phonons in Strongly Disordered Superlattices

Thanh Nguyen, Nina Andrejevic, Hoi Chun Po, Qichen Song, Yoichiro Tsurimaki, Nathan C. Drucker, Ahmet Alatas, Esen E. Alp, Bogdan M. Leu, Alessandro Cunsolo, Yong Qiang Cai, Lijun Wu, Joseph A. Garlow, Yimei Zhu, Hong Lü, Arthur C. Gossard, Alexander A. Puretzky, David B. Geohegan, Shengxi Huang, Mingda Li

Published Jul 27, 2021• 6 citations
arXivHTMLPDF

Abstract

Many-body localization (MBL) has attracted significant attention because of its immunity to thermalization, role in logarithmic entanglement entropy growth, and opportunities to reach exotic quantum orders. However, experimental realization of MBL in solid-state systems has remained challenging. Here, we report evidence of a possible phonon MBL phase in disordered GaAs/AlAs superlattices. Through grazing-incidence inelastic X-ray scattering, we observe a strong deviation of the phonon population from equilibrium in samples doped with ErAs nanodots at low temperature, signaling a departure from thermalization. This behavior occurs within finite phonon energy and wavevector windows, suggesting a localization-thermalization crossover. We support our observation by proposing a theoretical model for the effective phonon Hamiltonian in disordered superlattices, and showing that it can be mapped exactly to a disordered 1D Bose-Hubbard model with a known MBL phase. Our work provides momentum-resolved experimental evidence of phonon localization, extending the scope of MBL to disordered solid-state systems.

DOI
10.1021/acs.nanolett.1c01905

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Many-body localization (MBL) has attracted significant attention because of its immunity to thermalization, role in logarithmic entanglement entropy growth, and opportunities to reach exotic quantum orders. However, experimental realization of MBL in solid-state systems has remained challenging. Here, we report evidence of a possible phonon MBL phase in disordered GaAs/AlAs superlattices. Through grazing-incidence inelastic X-ray scattering, we observe a strong deviation of the phonon population from equilibrium in samples doped with ErAs nanodots at low temperature, signaling a departure from thermalization. This behavior occurs within finite phonon energy and wavevector windows, suggesting a localization-thermalization crossover. We support our observation by proposing a theoretical model for the effective phonon Hamiltonian in disordered superlattices, and showing that it can be mapped exactly to a disordered 1D Bose-Hubbard model with a known MBL phase. Our work provides momentum-resolved experimental evidence of phonon localization, extending the scope of MBL to disordered solid-state systems.
When a system thermalizes it loses all memory of its initial conditions. Even within a closed quantum system, subsystems usually thermalize using the rest of the system as a heat bath. Exceptions to quantum thermalization have been observed, but typically require inherent symmetries or noninteracting particles in the presence of static disorder. The prediction of many-body localization (MBL), in which disordered quantum systems can fail to thermalize despite strong interactions and high excitation energy, was therefore surprising and has attracted considerable theoretical attention. We experimentally generate MBL states by applying an Ising Hamiltonian with long-range interactions and programmably random disorder to ten spins initialized far from equilibrium with respect to the Hamiltonian. Using experimental and numerical methods we observe the essential signatures of MBL: initial state memory retention, Poissonian distributed many-body energy level spacings, and evidence of long-time entanglement growth. Our platform can be scaled to more spins, where detailed modeling of MBL becomes impossible.
Because of the presence of phonons, many-body localization (MBL) does not occur in disordered solids, even if disorder is strong. Local conservation laws characterizing an underlying MBL phase decay due to the coupling to phonons. We show that this decay can be compensated when the system is driven out of equilibrium. The resulting variations of the local temperature provide characteristic fingerprints of an underlying MBL phase. We consider a one-dimensional disordered spin chain, which is weakly coupled to a phonon bath and weakly irradiated by white light. The irradiation has weak effects in the ergodic phase. However, if the system is in the MBL phase, irradiation induces strong temperature variations despite the coupling to phonons. Temperature variations can be used similar to an order parameter to detect MBL phases, the phase transition, and a MBL correlation length.
Recently it has been suggested that many-body localization (MBL) can occur in translationally-invariant systems, and candidate 1D models have been proposed. We find that such models typically exhibit strong finite-size effects due to the presence of two or more vastly different energy scales, including an artificial separation of density of states into bands separated by large energy gaps. By carefully choosing the parameters of the models such that finite-size effects are minimized, we perform extensive numerical studies of small systems using exact diagonalization. Based on the variety of diagnostics, including entanglement properties and the behavior of local observables, we find the systems exhibit thermal (ergodic), rather than MBL-like behavior. Our results suggest that MBL in translationally-invariant systems with two very different energy scales is less robust than perturbative arguments suggest, possibly pointing to the importance of non-perturbative effects which induce delocalization in the thermodynamic limit.
We investigate the non-equilibrium dynamics of the disordered one-dimensional Fermi-Hubbard model with a focus on many-body localization. The system is initialized in a charge-density-wave-state, and its time evolution is analyzed through sublattice imbalance (spin and charge), and bipartite entanglement entropy. A clear crossover from ergodic to non-ergodic behavior is observed with increasing disorder strength. In the weak disorder regime, rapid decay of imbalance and the fast growth of entanglement indicate efficient thermalization. In contrast, a strong disorder leads to persistent imbalance and slow dynamics, signaling the breakdown of ergodicity. The charge and spin sectors exhibit distinct relaxation behavior, providing evidence for partial decoupling between these degrees of freedom. Furthermore, in the interacting regime, the entanglement entropy shows slow logarithmic growth, reflecting the dephasing-driven dynamics characteristic of the many-body localized phase. These results highlight the interplay between disorder and interactions in determining the dynamical properties of the system and establish robust signatures of many-body localization in the Fermi-Hubbard model.
Disorder in one-dimensional (1D) many-body systems facilitates abundant phases such as many-body localization (MBL) and thermalization. However, it remains unclear regarding their existence and behavior within hybrid quantum systems. Here, based on a simple bosonic-spin hybrid model, known as the Jaynes-Cummings-Hubbard (JCH) array, we investigate the effect of disorder compared to the phenomena in the clean system with the variation of atom-photon coupling strength. By using the level-spacing ratio, entanglement entropy, and the properties of observable diagonal and off-diagonal matrix elements, we find that strong disorder results in the appearance of a MBL phase in the JCH model that strongly violates the eigenstate thermalization hypothesis (ETH), while a conditional prethermal behavior can exist in the weak disorder regime. The conditional prethermal dynamics is based on the choice of initial product states. This work systematically reveals abundant many-body phases in the 1D JCH model and clarifies the discrepancies in the thermalization properties of systems with and without disorder.
Characterizing the many-body localization (MBL) transition in strongly disordered and interacting quantum systems is an important issue in the field of condensed matter physics. We study the single-particle Green's functions for a disordered interacting system in one dimension using exact diagnonalization in the infinite temperature limit and provide strong evidence that single-particle excitations carry signatures of delocalization to MBL transition. In the delocalized phase, the typical values of the local density of states and the scattering rate are finite while in the MBL phase, the typical values for both the quantities become vanishingly small. The probability distribution functions of the local density of states and the scattering rate are broad log-normal distributions in the delocalized phase while the distributions become very narrow and sharply peaked close to zero in the MBL phase. We also study the eigenstate Green's function for all the many-body eigenstates and demonstrate that both, the energy-resolved typical scattering rate and the typical local density of states, can track the many-body mobility edges.