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arXiv:2008.00535 · Physical Review A

Bright, continuous beams of cold free radicals

Jamie Shaw, Daniel McCarron

Published Oct 21, 2020• 19 citations
arXivHTMLPDF

Abstract

We demonstrate a cryogenic buffer gas-cooled molecular beam source capable of producing bright, continuous beams of cold and slow free radicals via laser ablation over durations of up to 60 seconds. The source design uses a closed liquid helium reservoir as a large thermal mass to minimize heating and ensure reproducible beam properties during operation. Under typical conditions, the source produces beams of our test species SrF, containing $5\ifmmode\times\else\texttimes\fi{}{10}^{12}$ molecules per steradian per second in the $X{\phantom{\rule{0.16em}{0ex}}}^{2}\mathrm{\ensuremath{\Sigma}}(v=0,N=1)$ state with a rotational temperature of 1.0(2) K and a forward velocity of $140\phantom{\rule{0.28em}{0ex}}\mathrm{m}/\mathrm{s}$. The beam properties are robust and unchanged for multiple cell exit geometries, but depend critically on the helium buffer gas flow rate, which must be $\ensuremath{\ge}10$ standard cubic centimeters per minute to produce bright, continuous beams of molecules for an ablation repetition rate of 55 Hz.

DOI
10.1103/physreva.102.041302

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•Jan 1, 2011•34 citations
We demonstrate a cryogenic buffer gas-cooled molecular beam source capable of producing bright, continuous beams of cold and slow free radicals via laser ablation over durations of up to 60 seconds. The source design uses a closed liquid helium reservoir as a large thermal mass to minimize heating and ensure reproducible beam properties during operation. Under typical conditions, the source produces beams of our test species SrF, containing 5\ifmmode×\else\texttimes\fi10125\ifmmode\times\else\texttimes\fi{}{10}^{12}5\ifmmode×\else\texttimes\fi1012 molecules per steradian per second in the X2\ensuremathΣ(v=0,N=1)X{\phantom{\rule{0.16em}{0ex}}}^{2}\mathrm{\ensuremath{\Sigma}}(v=0,N=1)X2\ensuremathΣ(v=0,N=1) state with a rotational temperature of 1.0(2) K and a forward velocity of 140m/s140\phantom{\rule{0.28em}{0ex}}\mathrm{m}/\mathrm{s}140m/s. The beam properties are robust and unchanged for multiple cell exit geometries, but depend critically on the helium buffer gas flow rate, which must be \ensuremath≥10\ensuremath{\ge}10\ensuremath≥10 standard cubic centimeters per minute to produce bright, continuous beams of molecules for an ablation repetition rate of 55 Hz.
We demonstrate and characterize a cryogenic buffer gas-cooled molecular beam source capable of producing bright beams of free radicals and refractory species. Details of the beam properties (brightness, forward velocity distribution, transverse velocity spread, rotational and vibrational temperatures) are measured under varying conditions for the molecular species SrF. Under typical conditions we produce a beam of brightness 1.2 × 10(11) molecules/sr/pulse in the X(2)Σ(+)(v = 0, N(rot) = 0) state, with 140(m/s) forward velocity and a rotational temperature of ≈ 1 K. This source compares favorably to other methods for producing beams of free radicals and refractory species for many types of experiments. We provide details of construction that may be helpful for others attempting to use this method.
We study the properties of a cryogenic buffer gas source that uses a low-temperature two-stage buffer gas cell to produce very slow beams of ytterbium monofluoride molecules. The molecules are produced by laser ablation inside the cell and extracted into a beam by a flow of cold helium. We measure the flux and velocity distribution of the beam as a function of ablation energy, helium flow rate, cell temperature, and the size of the gap between the first and second stages of the cell. We also compare the velocity distributions from one-stage and two-stage cells. The one-stage cell emits a beam with a speed of about 82 m s − 1 and a translational temperature of 0.63 K. The slowest beams are obtained using the two-stage cell at the lowest achievable cell temperature of 1.8 K. This beam has a peak velocity of 56 m s − 1 and a flux of 9 × 10 9 ground-state molecules per steradian per pulse, with a substantial fraction at speeds below 40 m s − 1 . These slow molecules can be decelerated further by radiation pressure slowing and then captured in a magneto-optical trap. Published by the American Physical Society 2024
We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. The beam is formed by particles exiting a hole in the buffer gas cell. We characterize the properties of the beam (flux, forward velocity, temperature) for both an atom (Na) and a molecule (PbO) under varying buffer gas density, and discuss conditions for optimizing these beam parameters. Our source compares favorably to existing techniques of beam formation, for a variety of applications.
We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. The beam is formed by particles exiting a hole in the buffer gas cell. We characterize the properties of the beam (flux, forward velocity, temperature) for both an atom (Na) and a molecule (PbO) under varying buffer gas density, and discuss conditions for optimizing these beam parameters. Our source compares favorably to existing techniques of beam formation, for a variety of applications.
A novel cryogenic MgF molecular beam, characterized by high flux and exceptional stability, has been successfully generated within a helium buffer gas environment. This achievement is facilitated by the innovative use of an in-cell stepper motor, which continuously rotates the sample rod during laser ablation. Through meticulous optimization of the ablation laser energy, the position of the ablation spot, and the gas flow rate, among other critical parameters, the resulting MgF beam exhibits a remarkable forward velocity of 209 m/s and an impressive brightness of approximately 1.36 × 1012 molecules per pulse per steradian per internal state. Subsequent attempts at one-dimensional Doppler cooling of the MgF beam have been made, with theoretical calculations closely aligning with experimental outcomes. These findings demonstrate a significant compression in the transverse spatial distribution of the molecular beam, from 7.8 to 6.5 mm, and a substantial cooling of the transverse temperature, from 8.1 to 5.6 mK. This work lays a crucial foundation for the advancement of molecular slowing and magneto-optical trapping techniques for MgF molecules.
Cryogenically cooled buffer gas beam sources of the molecule thorium monoxide (ThO) are optimized and characterized. Both helium and neon buffer gas sources are shown to produce ThO beams with high flux, low divergence, low forward velocity, and cold internal temperature for a variety of stagnation densities and nozzle diameters. The beam operates with a buffer gas stagnation density of \\(\\sim 10^{15}-10^{16}\\) cm\\(^{-3}\\) (Reynolds number \\(\\sim 1-100\\)), resulting in expansion cooling of the internal temperature of the ThO to as low as 2 K. For the neon (helium) based source, this represents cooling by a factor of about 10 (2) from the initial nozzle temperature of about 20 K (4 K). These sources deliver \\(\\sim 10^{11}\\) ThO molecules in a single quantum state within a 1-3 ms long pulse at 10 Hz repetition rate. Under conditions optimized for a future precision spectroscopy application [A C Vutha et al 2010 J. Phys. B: At. Mol. Opt. Phys. 43 074007], the neon-based beam has the following characteristics: forward velocity of 170 m/s, internal temperature of 3.4 K, and brightness of \\(3 \\times 10^{11}\\) ground state molecules per steradian per pulse. Compared to typical supersonic sources, the relatively low stagnation density of this source, and the fact that the cooling mechanism relies only on collisions with an inert buffer gas, make it widely applicable to many atomic and molecular species, including those which are chemically reactive, such as ThO.