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arXiv:2007.12220 · Physical Review A

Superradiance from nonideal initial states: A quantum trajectory approach

Sebastian Fuchs, András Vukics, Stefan Yoshi Buhmann

Published Apr 15, 2021• 4 citations
arXivHTMLPDF

Abstract

Collective emission behavior is usually described by the decay dynamics of the completely symmetric Dicke states. To study a more realistic scenario, we investigate alternative initial states inducing a more complex time evolution. Superposition states of the fully inverted Dicke state and the Dicke ground state with unequal mutual weights are studied as examples as well as superradiance stemming from atoms in clusters separated by more than one wavelength. The Monte Carlo wave function method serves as a framework to study the dynamics of quantum states, which is determined by quantum jumps, on the one hand, and continuous evolution dynamics, on the other hand. We compare this method with the classical picture of a system of rate equations written for the diagonal components of the density matrix.

DOI
10.1103/physreva.103.043712

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Collective emission behavior is usually described by the decay dynamics of the completely symmetric Dicke states. To study a more realistic scenario, we investigate alternative initial states inducing a more complex time evolution. Superposition states of the fully inverted Dicke state and the Dicke ground state with unequal mutual weights are studied as examples as well as superradiance stemming from atoms in clusters separated by more than one wavelength. The Monte Carlo wave function method serves as a framework to study the dynamics of quantum states, which is determined by quantum jumps, on the one hand, and continuous evolution dynamics, on the other hand. We compare this method with the classical picture of a system of rate equations written for the diagonal components of the density matrix.
We present several analytical approaches to the Dicke superradiance problem, which involves determining the time evolution of the density operator for an initially inverted ensemble of NNN identical two-level systems undergoing collective spontaneous emission. This serves as one of the simplest cases of open quantum system dynamics that allows for a fully analytical solution. We explore multiple methods to tackle this problem, yielding a solution valid for any time and any number of spins. These approaches range from solving coupled rate equations and identifying exceptional points in non-Hermitian evolution to employing combinatorial and probabilistic techniques, as well as utilizing a quantum jump unraveling of the master equation. The analytical solution is expressed as a residue sum obtained from a contour integral in the complex plane, suggesting the possibility of fully analytical solutions for a broader class of open quantum system dynamics problems.
We simulate the superradiant dynamics of ensembles of atoms in the presence of collective and individual atomic decay processes. We apply the Monte-Carlo wave-function method and identify quantum jumps in a reduced Dicke state basis, which reflects the permutation symmetry of the system. While the number of density matrix elements in the Dicke representation increases polynomially with atom number, the quantum jump dynamics populates only a single Dicke state at the time and thus efficient simulations can be carried out for tens of thousands of atoms. The superradiant pulses from initially excited atoms agree quantitatively with recent experimental results of strontium atoms but rapid atom loss in these experiments does not permit steady-state superradiance. By introducing an incident flux of new atoms to maintain a large average atom number, our theoretical calculations predict lasing with a millihertz linewidth despite rapid atom number fluctuations.
Fully-excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954. The burst is characterized by a maximum intensity scaling with the square of the number of atoms NNN and a temporal width reduced by NNN compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength λλλ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of non-interacting atoms with mutual separations much larger than λλλ. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.
We solve Dicke superradiance with two or more competing collective decay channels of tunable rates using a symbolic quantum-trajectory construction. The method yields closed time-domain populations and observables as finite combinations of exponential terms for arbitrary numbers of emitters and arbitrary decay rates. For two channels, the behavior of the stationary ground-state distribution resembles a first-order phase transition at the point where the channel-rate ratio is equal to unity. For balanced ddd-channel decay, we obtain scaling laws for the superradiant peak time and intensity. These results unify and extend single-channel Dicke dynamics to multilevel emitters and provide a compact tool for cavity and waveguide experiments, where permutation-symmetric reservoirs engineer multiple collective decay paths.
Fully excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954 [Phys. Rev. 93, 99 (1954)]. The burst is characterized by a maximum intensity scaling with the square of the number of atoms NNN and a temporal width reduced by NNN compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength $\ensuremath{\lambda}$ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of distant noninteracting atoms with mutual separations much larger than $\ensuremath{\lambda}$. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.
Determining the peak photon emission time and rate for an ensemble of NNN quantum systems undergoing collective superradiant decay typically requires tracking the time evolution of the density operator. Generally, the dimension of the density operator grows exponentially (∼ ⁣2N\sim \! 2^N∼2N) with the number of emitters, in the absence of any symmetries such as in Dicke superradiance with full or partial permutational symmetry. We present a detailed study of the superradiant peak emission rate and time for initially fully excited quantum emitter ensembles, for one-, two- and three-dimensional arrays in free-space and emitter chains coupled to waveguide reservoirs. For few emitters (N≲14N\lesssim 14N≲14) we utilize the full quantum master equation, and for mesoscopic emitter numbers (N≲400N\lesssim 400N≲400) we use a second- and third-order cumulant expansion of the operator averages to track the time evolution of the system.