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arXiv:2007.06752 · Physical Review A

Speeding up particle slowing using shortcuts to adiabaticity

John P. Bartolotta, J. Reilly, Murray Holland

Published Oct 16, 2020• 9 citations
arXivHTMLPDF

Abstract

We propose a method for slowing particles by laser fields that potentially has the ability to generate large forces without the associated momentum diffusion that results from the random directions of spontaneously scattered photons. In this method, time-resolved laser pulses with periodically modified detunings address an ultranarrow electronic transition to reduce the particle momentum through repeated absorption and stimulated emission cycles. We implement a shortcut to adiabaticity approach that is based on Lewis-Riesenfeld invariant theory. This affords our scheme the advantages of adiabatic transfer, where there can be an intrinsic insensitivity to the precise strength and detuning characteristics of the applied field, with the advantages of rapid transfer that are necessary for obtaining a short slowing distance. For typical parameters of a thermal oven source that generates a particle beam with a central velocity on the order of meters per second, this could result in slowing the particles to near stationary in less than a millimeter. We compare the slowing scheme to widely implemented slowing techniques that rely on radiation pressure forces and show the advantages that potentially arise when the excited-state decay rate is small. Thus, this scheme is a particularly promising candidate to slow narrow-linewidth systems that lack closed cycling transitions, such as occurs in certain molecules.

DOI
10.1103/physreva.102.043107

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We propose a method for slowing particles by laser fields that potentially has the ability to generate large forces without the associated momentum diffusion that results from the random directions of spontaneously scattered photons. In this method, time-resolved laser pulses with periodically modified detunings address an ultranarrow electronic transition to reduce the particle momentum through repeated absorption and stimulated emission cycles. We implement a shortcut to adiabaticity approach that is based on Lewis-Riesenfeld invariant theory. This affords our scheme the advantages of adiabatic transfer, where there can be an intrinsic insensitivity to the precise strength and detuning characteristics of the applied field, with the advantages of rapid transfer that are necessary for obtaining a short slowing distance. For typical parameters of a thermal oven source that generates a particle beam with a central velocity on the order of meters per second, this could result in slowing the particles to near stationary in less than a millimeter. We compare the slowing scheme to widely implemented slowing techniques that rely on radiation pressure forces and show the advantages that potentially arise when the excited-state decay rate is small. Thus, this scheme is a particularly promising candidate to slow narrow-linewidth systems that lack closed cycling transitions, such as occurs in certain molecules.
We propose and demonstrate a novel laser cooling mechanism applicable to particles with narrow-linewidth optical transitions. By sweeping the frequency of counter-propagating laser beams in a sawtooth manner, we cause adiabatic transfer back and forth between the ground state and a long-lived optically excited state. The time-ordering of these adiabatic transfers is determined by Doppler shifts, which ensures that the associated photon recoils are in the opposite direction to the particle's motion. This ultimately leads to a robust cooling mechanism capable of exerting large forces via a weak transition and with reduced reliance on spontaneous emission. We present a simple intuitive model for the resulting frictional force, and directly demonstrate its efficacy for increasing the total phase-space density of an atomic ensemble. We rely on both simulation and experimental studies using the 7.5 kHz linewidth 1 S 0 to 3 P 1 transition in 88 Sr. The reduced reliance on spontaneous emission may allow this adiabatic sweep method to be a useful tool for cooling particles that lack closed cycling transitions, such as molecules.
We provide a theoretical analysis for a recently demonstrated cooling method. Two-level particles undergo successive adiabatic transfers upon interaction with counterpropagating laser beams that are repeatedly swept over the transition frequency. We show that particles with narrow linewidth transitions can be cooled to near the recoil limit. This cooling mechanism has a reduced reliance on spontaneous emission compared to Doppler cooling, and hence shows promise for application to systems lacking closed cycling transitions, such as molecules.
Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We apply this technique to accelerate atoms, demonstrating up to an average of 19ℏk momentum transfers per spontaneous emission event. This represents more than an order of magnitude improvement in suppression of spontaneous emission compared to radiative scattering forces. For molecular beam slowing, this technique is capable of delivering a many-fold increase in the achievable time-averaged force to significantly reduce both the slowing distance and detrimental losses to dark vibrational states.
Optical cooling is a key technique for preparing ultracold atoms in quantum technologies and precision experiments. We employ shortcut-to-adiabaticity (STA) techniques to accelerate and stabilize laser-based atomic cooling protocols. This approach improves the performance of conventional adiabatic momentum transfer schemes by addressing key limitations such as Doppler shifts, laser intensity fluctuations, and spontaneous emission. We first examine two- and three-level atomic systems subjected to counter-propagating laser pulses that induce momentum reduction through photon recoil. STA methods are then employed to construct pulse sequences that are robust against detuning errors and amplitude noise, outperforming standard π-pulse schemes in resilience. Meanwhile, we analyze the dissipative dynamics during the momentum transfer and demonstrate the superiority of the STA protocol in enhancing momentum transfer efficiency via accelerated control. The results demonstrate that STA can significantly improve both the efficiency and robustness of cooling. These findings have implications for applications in atomic physics, quantum information processing, and precision metrology.
We report radiation pressure slowing of YbF molecules to low velocity. In YbF, laser slowing is hindered by leaks out of the optical cycle attributed to low-lying metastable electronic states arising from inner-shell excitation. We bring this population back into the optical cycle once it has decayed to the electronic ground state using microwaves to couple the relevant rotational levels. We measure the scattering rate and closure of the optical cycle as repumps are added, and study the destabilization of dark states by a magnetic field and by polarization modulation, finding that both are helpful for maximizing the scattering rate. Starting from a beam with a mean speed of 80 m/s, and using frequency-broadened slowing light, we reduce the mean speed of the beam and produce a substantial flux in the low-velocity tail of the distribution. Slowing increases the fraction of molecules below 40 m/s from 0.4(1)% to 7.0(2)%, and the fraction below 30 m/s from zero to 3.2(1)%. The establishment of a nearly closed optical cycle and the production of molecules at low velocity are important steps toward trapping YbF molecules for future measurements of the electron's electric dipole moment.
By definition, quantum adiabatic process means a slow process which allows the state to follow the instantaneous eigenstates of time-dependent Hamiltonian. For some reasons, for example, to avoid the decoherence effects, or to implement large-scale quantum information processing, we may want to speed up the adiabatic process, that is, to achieve the adiabatic-like control but in very short time. In this talk, we present new methods to speeded-up expansion and transport of cold atoms in a harmonic trap. Such shortcuts to adiabaticity provide the fast expansion or transport, in which the final atomic state is the same as in the adiabatic process, but in arbitrarily short time, keeping the same populations of vibrational levels in the initial and final trap. These methods can also be generalized to Bose-Einstein Condensates. Moreover, we present shortcuts to adiabatic passage from one internal atomic state to another in twoor three-level atoms. In detail, we can apply Berry’s transitionless quantum driving method and invariant-based inverse engineering method to accelerate the Rapid Adiabatic Passage (RAP) and Stimulated Raman Adiabatic Passage (STIRAP) in twoand three-level atomic systems, respectively. We also examine and compare the stability of different schemes concerning different types of noise and system errors. Finally, we show that the technique of shortcuts to adiabaticity in two-level system can be applied in fast and robust spin flip in a quantum dot, to avoid the decoherent effects.